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Physical Review A

Propagation of Small-Area Pulses of Coherent Light through a Resonant Medium

Michael D. Crisp

Published Nov 1, 1970• 85 citations
Publisher

Abstract

This article presents a study of the propagation of small-area pulses of coherent light through matter. It is found that the small-area pulses exactly obey an area theorem which, in the case of an attenuating medium, requires that the pulse area decay to zero exponentially with increasing distance of propagation. This, however, does not necessarily imply that the pulse energy decays exponentially. Instead, it is found that pulses of duration comparable to or shorter than the transverse relaxation time of the medium ${T}_{2}$ (including both homogeneous and inhomogeneous broadening) propagate with low energy loss. The results are explained in terms of simple physical arguments which indicate that the pulse envelope should oscillate between positive and negative values, causing the area to decrease without a comparable decrease in the pulse energy. Analytic solutions are presented for the case of a pulse whose envelope varies as ${t}^{k}{e}^{\ensuremath{-}t}$ for $tg0$, a rectangular pulse, an ultrashort pulse (i.e., pulse width much less than ${T}_{2}$), and the leading portion of a step-function pulse. The propagation of a small-area Gaussian pulse is studied numerically.

DOI
10.1103/physreva.2.2172.2

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Propagation of Small-Area Pulses of Coherent Light through a Resonant Medium

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This article presents a study of the propagation of small-area pulses of coherent light through matter. It is found that the small-area pulses exactly obey an area theorem which, in the case of an attenuating medium, requires that the pulse area decay to zero exponentially with increasing distance of propagation. This, however, does not necessarily imply that the pulse energy decays exponentially. Instead, it is found that pulses of duration comparable to or shorter than the transverse relaxation time of the medium ${T}_{2}$ (including both homogeneous and inhomogeneous broadening) propagate with low energy loss. The results are explained in terms of simple physical arguments which indicate that the pulse envelope should oscillate between positive and negative values, causing the area to decrease without a comparable decrease in the pulse energy. Analytic solutions are presented for the case of a pulse whose envelope varies as ${t}^{k}{e}^{\ensuremath{-}t}$ for $t>0$, a rectangular pulse, an ultrashort pulse (i.e., pulse width much less than ${T}_{2}$), and the leading portion of a step-function pulse. The propagation of a small-area Gaussian pulse is studied numerically.

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Ultrashort x-ray pulse propagation through resonant attenuating media

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A theoretical model for the propagation of coherent light pulses in resonant media where a large number of atoms cooperate in spontaneous emission (superradiance) is discussed. The medium is supposedly free of inhomogeneous broadening, and no lossy relaxation mechanisms are taken into account. The conditions for the emission of all spontaneous radiation in the direction of pulse propagation are described. A semi-classical model is used and, at each point in the medium, the propagation field and the spontaneous damping field are considered separately. The equation governing the evolution of a superradiant system in the presence of an applied pulse is derived. A mechanism of energy transfer from the traveling pulse to the medium is described which includes superradiant spontaneous emission effects. As a result of the neglect of all lossy relaxation processes, all energy stored in the medium is eventually returned to the pulse by coherent spontaneous emission. Therefore, in this theory, all pulses travel through the medium without energy loss. Numerical results for square input pulses are discussed which show two possible types of propagation behavior: (a) Low input intensities produce a negative tail to the input (positive) pulse and sharpening of the tail with the advance in the medium; (b) higher input intensities produce, after sufficient penetration, a steady-state pulse envelope somewhat similar to the $2\ensuremath{\pi}$ pulses of self-induced transparency. The steady-state solutions of the equations of motion are found numerically and the pulse shapes are computed for different degrees of superradiance. In the limit of strong superradiance, very asymmetric pulse envelopes of large area are found. For negligible superradiance, approximately $2\ensuremath{\pi}$ hyperbolic-secant pulses are obtained. The effects of inhomogeneous broadening are briefly considered, and the consequences of important superradiant damping in photon-echo experiments are qualitatively discussed.

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ULTRASHORT PULSE SHAPING IN LINEAR RESONANT ABSORBERS

Gazi Habiba Akter

Pulse shaping is the technique which controls the ultra-short pulse shape, and it became of great technological interest because of its potential applications in laser pulse compression, digital communications, microscopy etc. We demonstrate the idea of pulse-shaping technique and pulse propagation with low energy losses in a resonant linear absorbing medium. This thesis presents the results of a study of the propagation of Gaussian and hyperbolic secant ultrashort chirped and chirp-free pulses in homogeneously and inhomogeneously broadened resonant linear absorbers. Changes to the pulse shape and energy loss factor are presented as the pulse propagates in the absorber. The Fast Fourier method is used to numerically determine both the normalized intensity profile and the pulse spectrum. Our results show that, for pulse durations shorter than the relaxation time, chirped pulses in absorbing media obey the area theorem, with their shape changing with the propagation distance. Simulation results of the spectra of chirped pulses clearly show the burning of a spectral ’hole’ as the pulse propagates, with the pulse energy pushed away towards the wings. When compared to chirp-free pulses, chirped pulses reshape faster and develop wings in their tail due to initial phase modulation. Simulation results of the energy loss factor show that chirped pulses propagating in resonant linear absorbers sustain less energy losses than do chirp-free pulses. A comparison of chirped secant and Gaussian pulses shows that secant pulses propagate with lower energy losses. Analytic solutions are presented for long-distance asymptotic expressions of initial rms spectral bandwidth as well as for the attenuation factor of chirped Gaussian pulses. These analytical results are in agreement with numerical simulations. The comparison of energy losses of short chirped Gaussian pulses and long pulses of any profile in linear absorbers is also discussed in the thesis.

•Dec 14, 2011•0 citations
This article presents a study of the propagation of small-area pulses of coherent light through matter. It is found that the small-area pulses exactly obey an area theorem which, in the case of an attenuating medium, requires that the pulse area decay to zero exponentially with increasing distance of propagation. This, however, does not necessarily imply that the pulse energy decays exponentially. Instead, it is found that pulses of duration comparable to or shorter than the transverse relaxation time of the medium T2{T}_{2}T2​ (including both homogeneous and inhomogeneous broadening) propagate with low energy loss. The results are explained in terms of simple physical arguments which indicate that the pulse envelope should oscillate between positive and negative values, causing the area to decrease without a comparable decrease in the pulse energy. Analytic solutions are presented for the case of a pulse whose envelope varies as tke\ensuremath−t{t}^{k}{e}^{\ensuremath{-}t}tke\ensuremath−t for tg0tg0tg0, a rectangular pulse, an ultrashort pulse (i.e., pulse width much less than T2{T}_{2}T2​), and the leading portion of a step-function pulse. The propagation of a small-area Gaussian pulse is studied numerically.
This article presents a study of the propagation of small-area pulses of coherent light through matter. It is found that the small-area pulses exactly obey an area theorem which, in the case of an attenuating medium, requires that the pulse area decay to zero exponentially with increasing distance of propagation. This, however, does not necessarily imply that the pulse energy decays exponentially. Instead, it is found that pulses of duration comparable to or shorter than the transverse relaxation time of the medium T2{T}_{2}T2​ (including both homogeneous and inhomogeneous broadening) propagate with low energy loss. The results are explained in terms of simple physical arguments which indicate that the pulse envelope should oscillate between positive and negative values, causing the area to decrease without a comparable decrease in the pulse energy. Analytic solutions are presented for the case of a pulse whose envelope varies as ${t}^{k}{e}^{\ensuremath{-}t}$ for t>0t>0t>0, a rectangular pulse, an ultrashort pulse (i.e., pulse width much less than T2{T}_{2}T2​), and the leading portion of a step-function pulse. The propagation of a small-area Gaussian pulse is studied numerically.
The propagation of ultrashort x-ray pulses through a resonant attenuating two-level atom medium is investigated on the basis of the temporal point-source (the Green-function) formalism. A general case of the small-area pulse (SAP) approximation of a traveling coherent wave is considered. The patterns of the SAP envelope E(t,z) and energy U(z) evolution within the medium are calculated in the cases of incident Lorentzian and exponential pulses and their dependence on the temporal bandwidth ${\mathrm{\ensuremath{\tau}}}_{\mathrm{band}}$ in comparison with the total dissipative relaxation time (lifetime) T2{\mathrm{T}}_{2}T2​ . It is shown that if ${\mathrm{\ensuremath{\tau}}}_{\mathrm{band}}$ is the same order or smaller than T2{\mathrm{T}}_{2}T2​ , the reshaping (oscillations) of the pulse envelope and/or low energy-loss effects occur in accord with the general conclusions pointed out by Crisp [Phys. Rev. A 1, 1604 (1970)] in the case of the SAP for coherent light traveling through a resonant medium. The experimental conditions for the observation of penetration effects of the SAP of x rays are discussed. Based on the theoretical study, it is found that an ultrashort x-ray pulse emitted by an ultrashort laser-produced plasma propagates through thin resonant medium foils with low energy loss.
A theoretical model for the propagation of coherent light pulses in resonant media where a large number of atoms cooperate in spontaneous emission (superradiance) is discussed. The medium is supposedly free of inhomogeneous broadening, and no lossy relaxation mechanisms are taken into account. The conditions for the emission of all spontaneous radiation in the direction of pulse propagation are described. A semi-classical model is used and, at each point in the medium, the propagation field and the spontaneous damping field are considered separately. The equation governing the evolution of a superradiant system in the presence of an applied pulse is derived. A mechanism of energy transfer from the traveling pulse to the medium is described which includes superradiant spontaneous emission effects. As a result of the neglect of all lossy relaxation processes, all energy stored in the medium is eventually returned to the pulse by coherent spontaneous emission. Therefore, in this theory, all pulses travel through the medium without energy loss. Numerical results for square input pulses are discussed which show two possible types of propagation behavior: (a) Low input intensities produce a negative tail to the input (positive) pulse and sharpening of the tail with the advance in the medium; (b) higher input intensities produce, after sufficient penetration, a steady-state pulse envelope somewhat similar to the $2\ensuremath{\pi}$ pulses of self-induced transparency. The steady-state solutions of the equations of motion are found numerically and the pulse shapes are computed for different degrees of superradiance. In the limit of strong superradiance, very asymmetric pulse envelopes of large area are found. For negligible superradiance, approximately $2\ensuremath{\pi}$ hyperbolic-secant pulses are obtained. The effects of inhomogeneous broadening are briefly considered, and the consequences of important superradiant damping in photon-echo experiments are qualitatively discussed.
By solving the Maxwell-Bloch equations, we study the area evolution of a few-cycle pulse laser propagating in a resonant two-level-atom medium. We find that in short propagation distance, the pulse envelope, obtained within the slowly varying envelope approximation and the rotating-wave approximation, agrees nicely with the carrier field. In this case, the area theorem can still predict the profile of the area evolution of a few-cycle optical pulse. However, contrary to the long-pulse case, the variation of the few-cycle pulse area is caused by the pulse splitting but not by the pulse broadening or the pulse compression. Furthermore, the negative area occurs when the pulse area decreases. As a result, a pulse with area less than $\ensuremath{\pi}$ is not absorbed rapidly according to the usual Beer's law of absorption but evolves to nonvanishing zero $\ensuremath{\pi}$ pulse.
Propagation of an ultrashort, small-area (circularly polarized) pulse through a gas medium of three-level atoms near one-photon resonance is studied. The expression for the propagating pulse shape is obtained within the rotating wave and dipole approximations. Results are compared, both analytically and numerically, with those for two-level model. Sinusoidal and Gaussian shapes of input pulses are compared, and a high sensitivity of modulation of the light pulse for envelope to its input shape is revealed.
Pulse shaping is the technique which controls the ultra-short pulse shape, and it became of great technological interest because of its potential applications in laser pulse compression, digital communications, microscopy etc. We demonstrate the idea of pulse-shaping technique and pulse propagation with low energy losses in a resonant linear absorbing medium. This thesis presents the results of a study of the propagation of Gaussian and hyperbolic secant ultrashort chirped and chirp-free pulses in homogeneously and inhomogeneously broadened resonant linear absorbers. Changes to the pulse shape and energy loss factor are presented as the pulse propagates in the absorber. The Fast Fourier method is used to numerically determine both the normalized intensity profile and the pulse spectrum. Our results show that, for pulse durations shorter than the relaxation time, chirped pulses in absorbing media obey the area theorem, with their shape changing with the propagation distance. Simulation results of the spectra of chirped pulses clearly show the burning of a spectral ’hole’ as the pulse propagates, with the pulse energy pushed away towards the wings. When compared to chirp-free pulses, chirped pulses reshape faster and develop wings in their tail due to initial phase modulation. Simulation results of the energy loss factor show that chirped pulses propagating in resonant linear absorbers sustain less energy losses than do chirp-free pulses. A comparison of chirped secant and Gaussian pulses shows that secant pulses propagate with lower energy losses. Analytic solutions are presented for long-distance asymptotic expressions of initial rms spectral bandwidth as well as for the attenuation factor of chirped Gaussian pulses. These analytical results are in agreement with numerical simulations. The comparison of energy losses of short chirped Gaussian pulses and long pulses of any profile in linear absorbers is also discussed in the thesis.