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Journal of Physics B Atomic Molecular and Optical Physics

Theoretical model and novel numerical approach of a broadband optically pumped three-level alkali vapour laser

Zining Yang, Hongyan Wang, Qisheng Lu, Liang Liu, Yuandong Li, Weihong Hua, Xiaojun Xu, Jinbao Chen

Published Apr 11, 2011• 30 citations
Publisher

Abstract

A model for an end-pumped double-pass alkali vapour laser is set up which has considered all the main physical features, including the fine-structure mixing rate that represents the three-level nature of this kind of laser, the spectral dependence of pump light absorption for broadband pumping, the longitudinal population variation and the distributed intra-cavity losses. To solve this model, we have proposed a searching algorithm for a single-pass configuration and developed a novel iterative algorithm for a double-pass case which has taken the single-pass solution as an initial value. The calculation process demonstrates a fast rate of convergence and high degree of accuracy. By this algorithm, some special cases, for example, the non-uniform longitudinal distribution of alkali atom concentration, can also be solved well. The model and the numerical approach described in this paper demonstrate a new method to simulate the CW end-pumped quasi-three- or three-level lasers. In this way, no significant assumptions or simplifications are needed in the model, and both the detailed intra-cavity information and pump power distribution can be obtained. To ensure the correctness of our model, a comparison between our model and Beach et al 's model is made. The result shows that when the non-uniformity of the longitudinal population distribution is less than 20% or the pump intensity is far beyond the threshold, the assumption of longitudinal population average is valid and the two models are equivalent. When the pump intensity is near the threshold, this assumption may be invalid due to the large longitudinal population variation. If this case happens or more detailed laser information is required, we could use this model to obtain a more accurate solution.

DOI
10.1088/0953-4075/44/8/085401

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A model for an end-pumped double-pass alkali vapour laser is set up which has considered all the main physical features, including the fine-structure mixing rate that represents the three-level nature of this kind of laser, the spectral dependence of pump light absorption for broadband pumping, the longitudinal population variation and the distributed intra-cavity losses. To solve this model, we have proposed a searching algorithm for a single-pass configuration and developed a novel iterative algorithm for a double-pass case which has taken the single-pass solution as an initial value. The calculation process demonstrates a fast rate of convergence and high degree of accuracy. By this algorithm, some special cases, for example, the non-uniform longitudinal distribution of alkali atom concentration, can also be solved well. The model and the numerical approach described in this paper demonstrate a new method to simulate the CW end-pumped quasi-three- or three-level lasers. In this way, no significant assumptions or simplifications are needed in the model, and both the detailed intra-cavity information and pump power distribution can be obtained. To ensure the correctness of our model, a comparison between our model and Beach et al 's model is made. The result shows that when the non-uniformity of the longitudinal population distribution is less than 20% or the pump intensity is far beyond the threshold, the assumption of longitudinal population average is valid and the two models are equivalent. When the pump intensity is near the threshold, this assumption may be invalid due to the large longitudinal population variation. If this case happens or more detailed laser information is required, we could use this model to obtain a more accurate solution.
A three level model for optically pumped alkali metal vapor lasers is developed by considering the steady state rate equations for the longitudinally averaged number densities of the ground 2 S1/2 and first excited 2 P3/2, and 2 P1/2 states. For efficient operation, the collisional relaxation between the two upper levels should be fast relative to stimulated emission. By assuming a statistical distribution between the upper two levels, the limiting analytic solution for the quasi-two level system is achieved. A second limiting solution is identified for strongly bleached conditions where the atom recycle rate, limited by spin-orbit relaxation, fully specifies the output power. Performance in the intermediate regime depends significantly on pump laser bandwidth and requires numerical simulation. The ratio of populations for the two excited, 2 P3/2,1/2 states completes an analytic solution and depends primarily on pump laser bandwidth, threshold and alkali concentration.
An analytic model for the cw diode pumped alkali laser is developed by considering the longitudinally averaged number densities of the ground 2S1/2 and first excited 2P3/2, and 2P1/2 states. The pump intensity to reach threshold requires fully bleaching the pump transition and exceeding optical losses, typically about 200 Watts/cm2. Slope efficiency depends critically on the fraction of incident photons absorbed and the overlap of pump and resonator modes, approaching the quantum efficiency of 0.95 - 0.98. For marginal cavity transmission losses, peak performance is achieved for low output coupling. For efficient operation, the collisional relaxation between the two upper levels should be fast to prevent bottlenecking. By assuming a statistical distribution between the upper two levels, the limiting analytic solution for the quasitwo level system is achieved. For properly designed gain conditions, the quasi two level solution is usually achievable and represents ideal performance.
Comprehensive analysis of kinetic and fluid dynamic processes in flowing-gas diode-pumped alkali vapor amplifiers is reported. Taking into account effects of the temperature, the amplified spontaneous emission, the saturation power, the excitation of the alkali atoms to high electronic levels and the ionization, a detailed physical model is established to simulate the output performance of flowing-gas diode-pumped alkali vapor amplifiers. Influences of the flow velocity and the pump power on the amplified power are calculated and analyzed. Comparisons between single and double amplifier, longitudinal and transverse flow are made. Results show that end-pumped cascaded amplifier can provide higher output power under the same total pump power and the cell length, while output powers achieved by single- and double-end pumped, double-side pumped amplifiers with longitudinal or transverse flow have a complicated but valuable relation. Thus the model is extremely helpful for designing high-power flowing-gas diode-pumped alkali vapor amplifiers.
In the recent years, alkali vapor lasers have become the most promising candidates for realization of a light source with both good beam quality and high output power because of their excellent performances. A rubidium laser is a typical kind of alkali vapor lasers. In this study, we developed a theoretical mode to evaluate the population densities of three levels as well as mode-matching efficiency of a rubidium laser pumped by a narrow-linewidth Ti:Sapphire laser under two different focal conditions. In the evaluation, at least two values of the output power of a rubidium laser must be known, which are usually obtained from the experiment. We performed a series of experiments by using two pump lenses with two focal lengths of 150 and 200 mm, and acquired two corresponding values of the laser output power. Then, we applied the experimental results in the theoretical calculation and then obtained the population densities of three levels and mode-matching efficiency of the rubidium laser. The study demonstrates that the outputted pump power can be used for evaluation of the population densities of three levels and mode-matching efficiency of an alkali laser under the different experimental conditions. The study might be valuable to better understand the physical features of an alkali vapor laser and to optimize the configuration of a high-powered alkali laser in the future.
A numerical model has been developed, which is well suited to describe the kinetics of a laser-pumped barium vapour. The numerous processes essential for the temporal evolution in the population of the various barium levels are outlined in detail. A number of approximations and simplifications have to be introduced to adapt the complex problem to a numerical solution at an economical expense. Since the authors consider all substantial features of the laser-pumped barium vapour like the population development of low-lying levels, the ionisation of the vapour, stimulated infrared emission and radiative transfer, the requirement for a quantitative interpretation of experimental data is fulfilled.
The optimal detuning of the pump light at the rubidium D2 line is calculated and experimentally validated. A three-level optically end-pumped model in a hot rubidium vapor cell is demonstrated, which takes into account the hyperfine structure of the ground state, various collisional processes, and the nonlinear absorption of the pump light along the cell length. By developing a constrained optimization model, we calculate the optimal detuning of the pump light that maximizes the average excited state atom concentration in the cell. Experimentally, a 1529 nm probe light at higher levels, which is attenuated to the weak-probe limit, is introduced to accurately characterize the excited state atom concentration. Coupling with the experimental results, the variation of the pump light optimal detuning with the temperature and the pump light intensity at the unsaturated pumping is analyzed. At the optimal detuning point, the theoretical decay function of the pump light percentage along the vapor cell length almost coincides regardless of the temperature and the pump light intensity changes. Moreover, the theoretical fitted pump light decay function at optimal detuning is predicted. The fitted pump light percentage exiting the vapor cell is 4.75%. A fast implementation method to achieve the maximal average excited state atom concentration in the experiment is demonstrated.