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European Quantum Electronics Conference (EQEC)

Four-Wave Mixing at a Glass-Dense Cesium Vapor Interface Using Bichromatic Excitation

Vladimir A. Sautenkov, R. Gamidov

Published Jan 1, 1996• 0 citations
Publisher
DOI
10.1109/eqec.1996.561631

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Observation of narrow resonances inside homogeneously self-broadened lines in pump-probe reflection experiments

Vladimir A. Sautenkov, R. Gamidov, Antoine Weis

We report the experimental investigation of spectral hole burning and four-wave mixing at the interface of glass and a dense cesium vapor using two tunable diode lasers in a pump-probe experiment. Narrow spectral features were observed in the center of the strongly self-broadened ${\mathrm{D}}_{2}$ line at Cs number density from 9\ifmmode\times\else\texttimes\fi{}${10}^{15}$ to 2.8\ifmmode\times\else\texttimes\fi{}${10}^{16}$${\mathrm{ncm}}^{\mathrm{\ensuremath{-}}3}$. The origin of the resonances is associated with the coherent scattering of laser beams at a self-induced population grating, and their spectral widths reflect the relaxation rate of the population difference. A simple asymptotic expression is used to fit the spectral line shapes and to infer a population relaxation time of 3.7(2) ns, which is almost an order of magnitude shorter than natural lifetime of the excited state.

Physical Review A•Apr 1, 1997•14 citations
We report the experimental investigation of spectral hole burning and four-wave mixing at the interface of glass and a dense cesium vapor using two tunable diode lasers in a pump-probe experiment. Narrow spectral features were observed in the center of the strongly self-broadened D2{\mathrm{D}}_{2}D2​ line at Cs number density from 9\ifmmode\times\else\texttimes\fi{}1015{10}^{15}1015 to 2.8\ifmmode\times\else\texttimes\fi{}1016{10}^{16}1016${\mathrm{ncm}}^{\mathrm{\ensuremath{-}}3}$. The origin of the resonances is associated with the coherent scattering of laser beams at a self-induced population grating, and their spectral widths reflect the relaxation rate of the population difference. A simple asymptotic expression is used to fit the spectral line shapes and to infer a population relaxation time of 3.7(2) ns, which is almost an order of magnitude shorter than natural lifetime of the excited state.