Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical Review A

Coherent-incoherent transition and relaxation in condensed-phase tunneling systems

Chi H. Mak, David Chandler

Published Aug 1, 1991• 132 citations
Publisher

Abstract

The tunneling dynamics of the spin-boson problem has been computed using discretized path-integral simulations for temperatures T and couplings, i.e., the Kondo parameter \ensuremath{\alpha}, spanning the entire T-\ensuremath{\alpha} plane. The inherent problem of alternating weights has been solved using a combination of the stationary-phase Monte Carlo method and contour-distortion techniques. A transition from coherent to purely incoherent relaxation was observed for the spin correlation function. The time correlation functions and the location of the coherent-incoherent boundary on the T-\ensuremath{\alpha} plane are well described by the noninteracting-blip approximation. In the deep-tunneling limit of large \ensuremath{\alpha}, low T, and high bath frequency, the system relaxes exponentially, with its relaxation time constant following a power-law temperature dependence, in accord with perturbation theory. At higher T and low bath frequency, the relaxation time crosses over to a classical Arrhenius temperature dependence, reflecting the onset of activated processes. For a narrow region within 1/21, numerical results suggest that the system undergoes incoherent relaxation, with a short-time exponential decay, followed by a long-time tail of the power-law type. The short-time exponential relaxation time follows a peculiar power-law temperature dependence, with the relaxation rate increasing as a function of decreasing temperature.

DOI
10.1103/physreva.44.2352

Related papers

From coherent motion to localization: dynamics of the spin-boson model at zero temperature

Haobin Wang, Michael Thoss

The dynamics of the spin-boson model at zero temperature is investigated using the multilayer multiconfiguration time-dependent Hartree (ML-MCTDH) method.This method allows a numerically exact description of the dynamics of the spin-boson model in a broad range of coupling strengths.The results show the transition of the dynamics from weakly damped coherent motion to incoherent decay and finally to localization upon increase of the system-bath coupling strength.A detailed analysis of the incoherent decay for stronger coupling reveals that multiple timescales are involved in the dynamics.Furthermore, the applicability of the scaling limit for large characteristic frequencies of the bath as well as the validity of the non-interacting blip approximation are studied in some detail.

New Journal of Physics•Nov 20, 2008•145 citations

Dissipative tunneling in a bath of two-level systems

Kelsey M. Forsythe, Nancy Makri

The dynamical behavior of a two-level system coupled linearly to a dissipative bath of two-level systems whose tunneling splittings and coupling parameters are distributed according to an Ohmic spectrum is studied using numerical path integral methods as well as the noninteracting blip approximation for an equivalent harmonic environment characterized by a scaled spectral density. Comparisons with the behaviors of the conventional spin-boson model of similar coupling strength reveal a weaker quenching of coherence in the present case. Finally, the boundary in parameter space between coherent and incoherent dynamics is mapped.

Physical review. B, Condensed matter•Jul 1, 1999•42 citations

Observation of incoherent relaxation by tunneling in a macroscopic two-state system

Siyuan Han, J. Lapointe, James E. Lukens

The dynamics of a dissipative, quantized macroscopic two-state system have been experimentally investigated through the measurement of tunneling transitions between the adjacent, equal-energy fluxoid states of a superconducting loop containing Josephson junctions. The tunneling rate \ensuremath{\Gamma} has been observed to approach zero as a power law in the temperature, giving a damping parameter \ensuremath{\alpha}=1.44, in the incoherent relaxation regime. The predicted exponential dependence of \ensuremath{\Gamma} on barrier height has been quantitatively confirmed.

Physical Review Letters•Feb 11, 1991•70 citations

Influence of temperature on coherent dynamics of a two-level system immersed in a dissipative spin bath

Zhiguo Lü, Hang Zheng

The quantum dynamics of a two-level system coupled to an Ohmic spin bath is studied by means of the perturbation approach based on a unitary transformation. A scattering function xi(k) is introduced in the transformation to take into account quantum fluctuations. By the master equation within the Born approximation, nonequilibrium dynamics quantities are calculated. The method works well for the coupling constant 0<alpha<alpha(c) and a finite bare tunneling Delta. It is found that (i) only at zero temperature with small coupling or moderate one does the spin-spin-bath model display identical behavior as the well-known spin-boson-bath model; (ii) in comparison with the known results of spin-boson-bath model, the coherence-incoherence transition point, which occurs at alpha(c)=12[1+etaDelta/omega(c)], is temperature independent; and (iii) the nonequilibrium correlation function P(t)=tau(z)(t), evolves without temperature dependence, while tau(x)(t) depends on temperature. Both P(t) and tau(x)(t) not only satisfy their initial conditions, respectively, and also have correct long time limits. Besides, the Shiba relation and sum rule are exactly satisfied in the coherent regime for this method. Our results show that increasing temperature does not help the system suppress decoherence in the coherent regime, i.e., finite temperature does not favor the coherent dynamics in this regime. Thus, the finite-temperature dynamics induced by two kinds of baths (spin-bath and boson-bath) exhibit distinctly different physics.

arXiv:1104.1751•The Journal of Chemical Physics•Oct 5, 2009•13 citations

Dynamics of the dissipative two-state system

A. J. Leggett, Sudip Chakravarty, Alan T. Dorsey +3 more

This paper presents the results of a functional-integral approach to the dynamics of a two-state system coupled to a dissipative environment. It is primarily an extended account of results obtained over the last four years by the authors; while they try to provide some background for orientation, it is emphatically not intended as a comprehensive review of the literature on the subject. Its contents include (1) an exact and general prescription for the reduction, under appropriate circumstances, of the problem of a system tunneling between two wells in the presence of a dissipative environment to the "spin-boson" problem; (2) the derivation of an exact formula for the dynamics of the latter problem; (3) the demonstration that there exists a simple approximation to this exact formula which is controlled, in the sense that we can put explicit bounds on the errors incurred in it, and that for almost all regions of the parameter space these errors are either very small in the limit of interest to us (the "slow-tunneling" limit) or can themselves be evaluated with satisfactory accuracy; (4) use of these results to obtain quantitative expressions for the dynamics of the system as a function of the spectral density $J(\ensuremath{\omega})$ of its coupling to the environment. If $J(\ensuremath{\omega})$ behaves as ${\ensuremath{\omega}}^{s}$ for frequencies of the order of the tunneling frequency or smaller, the authors find for the "unbiased" case the following results: For $s<1$ the system is localized at zero temperature, and at finite $T$ relaxes incoherently at a rate proportional to $\mathrm{exp}\ensuremath{-}{(\frac{{T}_{0}}{T})}^{1\ensuremath{-}s}$. For $s>2$ it undergoes underdamped coherent oscillations for all relevant temperatures, while for $1<s<2$ there is a crossover from coherent oscillation to overdamped relaxation as $T$ increases. Exact expressions for the oscillation and/or relaxation rates are presented in all these cases. For the "ohmic" case, $s=1$, the qualitative nature of the behavior depends critically on the dimensionless coupling strength $\ensuremath{\alpha}$ as well as the temperature $T$: over most of the ($\ensuremath{\alpha}$,$T$) plane (including the whole region $\ensuremath{\alpha}>1$) the behavior is an incoherent relaxation at a rate proportional to ${T}^{2\ensuremath{\alpha}\ensuremath{-}1}$, but for low $T$ and $0<\ensuremath{\alpha}<\frac{1}{2}$ the authors predict a combination of damped coherent oscillation and incoherent background which appears to disagree with the results of all previous approximations. The case of finite bias is also discussed.

Reviews of Modern Physics•Jan 1, 1987•5,104 citations

Coherent-incoherent transition in the sub-Ohmic spin-boson model

Alex W. Chin, Misha Turlakov

We study the spin-boson model with a sub-Ohmic bath using a variational method. The transition from coherent dynamics to incoherent tunneling is found to be abrupt as a function of the coupling strength $\ensuremath{\alpha}$ and to exist for any power $0<s<1$, where the bath coupling is described by $J(\ensuremath{\omega})\ensuremath{\sim}\ensuremath{\alpha}{\ensuremath{\omega}}^{s}$. We find nonmonotonic temperature dependence of the two-level gap $\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{K}$ and a reentrance regime close to the transition due to nonadiabatic low-frequency bath modes. Differences between thermodynamic and dynamic conditions for the transition as well as the limitations of the simplified bath description are discussed.

arXiv:cond-mat/0511285•Physical Review B•Feb 7, 2006•54 citations
The tunneling dynamics of the spin-boson problem has been computed using discretized path-integral simulations for temperatures T and couplings, i.e., the Kondo parameter \ensuremath{\alpha}, spanning the entire T-\ensuremath{\alpha} plane. The inherent problem of alternating weights has been solved using a combination of the stationary-phase Monte Carlo method and contour-distortion techniques. A transition from coherent to purely incoherent relaxation was observed for the spin correlation function. The time correlation functions and the location of the coherent-incoherent boundary on the T-\ensuremath{\alpha} plane are well described by the noninteracting-blip approximation. In the deep-tunneling limit of large \ensuremath{\alpha}, low T, and high bath frequency, the system relaxes exponentially, with its relaxation time constant following a power-law temperature dependence, in accord with perturbation theory. At higher T and low bath frequency, the relaxation time crosses over to a classical Arrhenius temperature dependence, reflecting the onset of activated processes. For a narrow region within 1/21, numerical results suggest that the system undergoes incoherent relaxation, with a short-time exponential decay, followed by a long-time tail of the power-law type. The short-time exponential relaxation time follows a peculiar power-law temperature dependence, with the relaxation rate increasing as a function of decreasing temperature.
The dynamics of the spin-boson model at zero temperature is investigated using the multilayer multiconfiguration time-dependent Hartree (ML-MCTDH) method.This method allows a numerically exact description of the dynamics of the spin-boson model in a broad range of coupling strengths.The results show the transition of the dynamics from weakly damped coherent motion to incoherent decay and finally to localization upon increase of the system-bath coupling strength.A detailed analysis of the incoherent decay for stronger coupling reveals that multiple timescales are involved in the dynamics.Furthermore, the applicability of the scaling limit for large characteristic frequencies of the bath as well as the validity of the non-interacting blip approximation are studied in some detail.
The dynamical behavior of a two-level system coupled linearly to a dissipative bath of two-level systems whose tunneling splittings and coupling parameters are distributed according to an Ohmic spectrum is studied using numerical path integral methods as well as the noninteracting blip approximation for an equivalent harmonic environment characterized by a scaled spectral density. Comparisons with the behaviors of the conventional spin-boson model of similar coupling strength reveal a weaker quenching of coherence in the present case. Finally, the boundary in parameter space between coherent and incoherent dynamics is mapped.
The dynamics of a dissipative, quantized macroscopic two-state system have been experimentally investigated through the measurement of tunneling transitions between the adjacent, equal-energy fluxoid states of a superconducting loop containing Josephson junctions. The tunneling rate \ensuremath{\Gamma} has been observed to approach zero as a power law in the temperature, giving a damping parameter \ensuremath{\alpha}=1.44, in the incoherent relaxation regime. The predicted exponential dependence of \ensuremath{\Gamma} on barrier height has been quantitatively confirmed.
The quantum dynamics of a two-level system coupled to an Ohmic spin bath is studied by means of the perturbation approach based on a unitary transformation. A scattering function xi(k) is introduced in the transformation to take into account quantum fluctuations. By the master equation within the Born approximation, nonequilibrium dynamics quantities are calculated. The method works well for the coupling constant 0<alpha<alpha(c) and a finite bare tunneling Delta. It is found that (i) only at zero temperature with small coupling or moderate one does the spin-spin-bath model display identical behavior as the well-known spin-boson-bath model; (ii) in comparison with the known results of spin-boson-bath model, the coherence-incoherence transition point, which occurs at alpha(c)=12[1+etaDelta/omega(c)], is temperature independent; and (iii) the nonequilibrium correlation function P(t)=tau(z)(t), evolves without temperature dependence, while tau(x)(t) depends on temperature. Both P(t) and tau(x)(t) not only satisfy their initial conditions, respectively, and also have correct long time limits. Besides, the Shiba relation and sum rule are exactly satisfied in the coherent regime for this method. Our results show that increasing temperature does not help the system suppress decoherence in the coherent regime, i.e., finite temperature does not favor the coherent dynamics in this regime. Thus, the finite-temperature dynamics induced by two kinds of baths (spin-bath and boson-bath) exhibit distinctly different physics.
This paper presents the results of a functional-integral approach to the dynamics of a two-state system coupled to a dissipative environment. It is primarily an extended account of results obtained over the last four years by the authors; while they try to provide some background for orientation, it is emphatically not intended as a comprehensive review of the literature on the subject. Its contents include (1) an exact and general prescription for the reduction, under appropriate circumstances, of the problem of a system tunneling between two wells in the presence of a dissipative environment to the "spin-boson" problem; (2) the derivation of an exact formula for the dynamics of the latter problem; (3) the demonstration that there exists a simple approximation to this exact formula which is controlled, in the sense that we can put explicit bounds on the errors incurred in it, and that for almost all regions of the parameter space these errors are either very small in the limit of interest to us (the "slow-tunneling" limit) or can themselves be evaluated with satisfactory accuracy; (4) use of these results to obtain quantitative expressions for the dynamics of the system as a function of the spectral density $J(\ensuremath{\omega})$ of its coupling to the environment. If $J(\ensuremath{\omega})$ behaves as ${\ensuremath{\omega}}^{s}$ for frequencies of the order of the tunneling frequency or smaller, the authors find for the "unbiased" case the following results: For s<1s<1s<1 the system is localized at zero temperature, and at finite TTT relaxes incoherently at a rate proportional to $\mathrm{exp}\ensuremath{-}{(\frac{{T}_{0}}{T})}^{1\ensuremath{-}s}$. For s>2s>2s>2 it undergoes underdamped coherent oscillations for all relevant temperatures, while for 1<s<21<s<21<s<2 there is a crossover from coherent oscillation to overdamped relaxation as TTT increases. Exact expressions for the oscillation and/or relaxation rates are presented in all these cases. For the "ohmic" case, s=1s=1s=1, the qualitative nature of the behavior depends critically on the dimensionless coupling strength $\ensuremath{\alpha}$ as well as the temperature TTT: over most of the ($\ensuremath{\alpha}$,TTT) plane (including the whole region $\ensuremath{\alpha}>1$) the behavior is an incoherent relaxation at a rate proportional to ${T}^{2\ensuremath{\alpha}\ensuremath{-}1}$, but for low TTT and $0<\ensuremath{\alpha}<\frac{1}{2}$ the authors predict a combination of damped coherent oscillation and incoherent background which appears to disagree with the results of all previous approximations. The case of finite bias is also discussed.
We study the spin-boson model with a sub-Ohmic bath using a variational method. The transition from coherent dynamics to incoherent tunneling is found to be abrupt as a function of the coupling strength $\ensuremath{\alpha}$ and to exist for any power 0<s<10<s<10<s<1, where the bath coupling is described by $J(\ensuremath{\omega})\ensuremath{\sim}\ensuremath{\alpha}{\ensuremath{\omega}}^{s}$. We find nonmonotonic temperature dependence of the two-level gap $\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{K}$ and a reentrance regime close to the transition due to nonadiabatic low-frequency bath modes. Differences between thermodynamic and dynamic conditions for the transition as well as the limitations of the simplified bath description are discussed.