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Lasers, Sources, and Related Photonic Devices

Remote backwards emission in air via stimulated emission in atomic oxygen

Arthur Dogariu, James Michael, Richard B. Miles

Published Jan 1, 2012• 1 citation
Publisher

Abstract

We demonstrate and investigate coherent stimulated emission in the forward and backward direction form a remotely induced gain region created by an ultraviolet laser which dissociates molecular oxygen and excites atomic oxygen.
DOI
10.1364/lacsea.2012.lt2b.2

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The physical nature of the backward-stimulated emission can be understood by considering the angular distribution of the total radiation from a set of atomic dipoles driven by an intense laser beam. From the classical point of view, the backward-stimulated emission is simply a reflection from the interface between a dielectric and a gain medium from the mismatch in the imaginary parts of their indices of refraction. For bulk gain structure, backward-stimulated emission is usually too weak to be noticed. However, in the case of a gain layer much thinner than a wavelength or a periodic thin gain structure with a spacing of λ/2, the backward-stimulated emission is enhanced and can be as large as the forward stimulated emission in terms of the amplitude of radiation field.1
We have studied coherent emission from ambient air and demonstrated efficient generation of laser-like beams directed both forward and backward with respect to a nanosecond ultraviolet pumping laser beam. The generated optical gain is a result of two-photon photolysis of atmospheric O(2), followed by two-photon excitation of atomic oxygen. We have analyzed the temporal shapes of the emitted pulses and have observed very short duration intensity spikes as well as a large Rabi frequency that corresponds to the emitted field. Our results suggest that the emission process exhibits nonadiabatic atomic coherence, which is similar in nature to Dicke superradiance where atomic coherence is large and can be contrasted with ordinary lasing where atomic coherence is negligible. This atomic coherence in oxygen adds insight to the optical emission physics and holds promise for remote sensing techniques employing nonlinear spectroscopy.
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There is nothing so practical as a good theory. As a case in point, the compelling need for standoff detection of hazardous gases and vapor indicators of explosives has motivated the development of remotely pumped, scheme(s) which produce radiation in the backward direction [1,2]. Moving from conceptualization to theoretical analysis and experimental verification, we demonstrate that high gain can be achieved in air. Backward air lasing provides possibilities for remote detection [3] as will be discussed.