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Physical Review A

Correlation-function hierarchies in nonlinear quantum optics

Christopher J. Mertens, Jeff Hasty, H. H. Roark, D. Nowakowski, T. A. B. Kennedy

Published Jul 1, 1995• 8 citations
Publisher

Abstract

A correlation-function hierarchy for intracavity quantum optical systems has been derived using nonequilibrium Green function methods. A specific truncation is applied to study nonlinear quantum fluctuations in an optical parametric oscillator near threshold. An analysis of the limitations of the truncation and comparison of its efficiency and accuracy relative to coherent state phase space methods and wave-function simulation methods is made.

DOI
10.1103/physreva.52.742

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A correlation-function hierarchy for intracavity quantum optical systems has been derived using nonequilibrium Green function methods. A specific truncation is applied to study nonlinear quantum fluctuations in an optical parametric oscillator near threshold. An analysis of the limitations of the truncation and comparison of its efficiency and accuracy relative to coherent state phase space methods and wave-function simulation methods is made.
A method for the the derivation and truncation of correlation function hierarchies for Markovian damped quantum-optical systems is presented. The theory enables the inclusion of multiphoton scattering processes which are ignored in conventional semiclassical theories. These produce observable dynamical signatures which depend on characteristic scales of photon number. Applications of the theory to intracavity optical parametric oscillation and second-harmonic generation are given. \textcopyright{} 1996 The American Physical Society.
Quantum properties of intracavity nonlinear optical processes such as parametric oscillation and second harmonic generation are limited to a linearized analytical treatment except for certain special cases. Perfect squeezing in one quadrature and the divergence in fluctuations of the conjugate quadrature predicted at threshold in parametric oscillation are a consequence of the approximate linearized analysis. We investigate nonlinear quantum fluctuation corrections by using nonequilibrium Green’s function methods1,2 in concert with quantum master equations, to assess when these system-size effects may be observable in the laboratory.
We develop a systematic theory of quantum fluctuations in the driven optical parametric oscillator, including the region near threshold. This allows us to treat the limits imposed by nonlinearities to quantum squeezing and noise reduction in this nonequilibrium quantum phase transition. In particular, we compute the squeezing spectrum near threshold and calculate the optimum value. We find that the optimal noise reduction occurs at different driving fields, depending on the ratio of damping rates. The largest spectral noise reductions are predicted to occur with a very high-QQQ second-harmonic cavity. Our analytic results agree well with stochastic numerical simulations. We also compare the results obtained in the positive-PPP representation, as a fully quantum-mechanical calculation, with the truncated Wigner phase-space equation, also known as the semiclassical theory.
We present a fully quantum mechanical treatment of the nondegenerate optical parametric oscillator both below and near threshold. This is a nonequilibrium quantum system with a critical point phase transition, that is also known to exhibit strong yet easily observed squeezing and quantum entanglement. Our treatment makes use of the positive PPP representation and goes beyond the usual linearized theory. We compare our analytical results with numerical simulations and find excellent agreement. We also carry out a detailed comparison of our results with those obtained from stochastic electrodynamics, a theory obtained by truncating the equation of motion for the Wigner function, with a view to locating regions of agreement and disagreement between the two. We calculate commonly used measures of quantum behavior including entanglement, squeezing, and Einstein-Podolsky-Rosen (EPR) correlations as well as higher order tripartite correlations, and show how these are modified as the critical point is approached. These results are compared with those obtained using two degenerate parametric oscillators, and we find that in the near-critical region the nondegenerate oscillator has stronger EPR correlations. In general, the critical fluctuations represent an ultimate limit to the possible entanglement that can be achieved in a nondegenerate parametric oscillator.
We present a method to describe driven-dissipative multi-mode systems by considering a truncated hierarchy of equations for the correlation functions. We consider two hierarchy truncation schemes with a global cutoff on the correlation order, which is the sum of the exponents of the operators involved in the correlation functions: a 'hard' cutoff corresponding to an expansion around the vacuum, which applies to a regime where the number of excitations per site is small; a 'soft' cutoff which corresponds to an expansion around coherent states, which can be applied for large excitation numbers per site. This approach is applied to describe the bunching-antibunching crossover in the driven-dissipative Bose–Hubbard model for photonic systems. The results have been successfully benchmarked by comparison with calculations based on the corner-space renormalization method in 1D and 2D systems. The regime of validity and strengths of the present truncation methods are critically discussed.
Abstract We present a method to describe driven-dissipative multi-mode systems by considering a truncated hierarchy of equations for the correlation functions. We consider two hierarchy truncation schemes with a global cutoff on the correlation order, which is the sum of the exponents of the operators involved in the correlation functions: a ‘hard’ cutoff corresponding to an expansion around the vacuum, which applies to a regime where the number of excitations per site is small; a ‘soft’ cutoff which corresponds to an expansion around coherent states, which can be applied for large excitation numbers per site. This approach is applied to describe the bunching-antibunching crossover in the driven-dissipative Bose–Hubbard model for photonic systems. The results have been successfully benchmarked by comparison with calculations based on the corner-space renormalization method in 1D and 2D systems. The regime of validity and strengths of the present truncation methods are critically discussed.