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Physical Review A

Theory of parametric frequency down conversion of light

C. K. Hong, L. Mandeļ

Published Apr 1, 1985• 464 citations
Publisher

Abstract

A theoretical study is made of the process in which incident pump photons that interact with a nonlinear medium (such as a crystal lacking inversion symmetry) are spontaneously split into lower-frequency signal and idler photons. The down-converted fields are quantized and described by a continuum of modes, a subset of which interacts with each photodetector. It is shown that when two ideal photodetectors are appropriately located so that they receive the conjugate signal and idler photons, then the joint probability of two-photon detection by the two detectors can equal the single-photon detection probability. The time correlation between the two detected photons is shown to be limited either by the resolving time of the detectors, or by the bandwidth of the down-converted light, and to be independent of the coherence time of the pump field or of the length of the nonlinear medium. These conclusions are compared with the results of recent experiments.

DOI
10.1103/physreva.31.2409

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jan 19, 2006•1 citation
A theoretical study is made of the process in which incident pump photons that interact with a nonlinear medium (such as a crystal lacking inversion symmetry) are spontaneously split into lower-frequency signal and idler photons. The down-converted fields are quantized and described by a continuum of modes, a subset of which interacts with each photodetector. It is shown that when two ideal photodetectors are appropriately located so that they receive the conjugate signal and idler photons, then the joint probability of two-photon detection by the two detectors can equal the single-photon detection probability. The time correlation between the two detected photons is shown to be limited either by the resolving time of the detectors, or by the bandwidth of the down-converted light, and to be independent of the coherence time of the pump field or of the length of the nonlinear medium. These conclusions are compared with the results of recent experiments.
When a laser beam interacts with a nonlinear crystal, some of the incident photons fission into two lower frequency signal and idler photons through the process of spontaneous parametric downconversion. It is shown that, as a result of the strong positive correlation between signal and idler photons, the normalized intensity cross-correlation function λ12(τ) should be inversely proportional to the downconverted light intensity and ideally should be given by the inverse of the mean number of photons counted in the resolving time. This unusual relationship, which is a reflection of the quantum mechanical character of the downconverted optical field, has been confirmed in photoelectric counting measurements. The experiment makes use of the light from an argon-ion laser oscillating at 351.1 nm interacting with an 8-cm long crystal of KDP. The downconverted light is extracted at 633.5 and 788.0 nm in two directions that satisfy the phase-matching condition and is allowed to fall on two counting photomultipliers. The output pulses are fed to a time-to-digital converter that yields the cross-correlation function.
A concept for an ultra-broad-band optical parametric amplifier or oscillator has emerged as a by-product of a theoretical study in fundamental quantum optics. The study was originally intended to address the question of whether the two-photon temporal correlation function of light [in particular, light produced by spontaneous parametric down conversion (SPDC)] can be considerably narrower than the inverse of the spectral width (bandwidth) of the light. The answer to the question was found to be negative. More specifically, on the basis of the universal integral relations between the quantum two-photon temporal correlation and the classical spectrum of light, it was found that the lower limit of two-photon correlation time is set approximately by the inverse of the bandwidth. The mathematical solution for the minimum two-photon correlation time also provides the minimum relative frequency dispersion of the down-converted light components; in turn, the minimum relative frequency dispersion translates to the maximum bandwidth, which is important for the design of an ultra-broad-band optical parametric oscillator or amplifier. In the study, results of an analysis of the general integral relations were applied in the case of an optically nonlinear, frequency-dispersive crystal in which SPDC produces collinear photons. Equations were found for the crystal orientation and pump wavelength, specific for each parametric-down-converting crystal, that eliminate the relative frequency dispersion of collinear degenerate (equal-frequency) signal and idler components up to the fourth order in the frequency-detuning parameter
A theoretical treatment is given of the situation in which two photons produced in the parametric frequency splitting of light in a nonlinear medium are allowed to interfere. It is shown that there is no interference pattern in the usual sense of quantities that are of the second order in the field, but that fourth-order interference effects are present. These could be demonstrated by placing two photodetectors at positions x,x′ in the interference plane and measuring the joint probability of two detections as a function of x – x′. The probability is predicted to exhibit a cosine modulation with separation x – x′ of close to 100% visibility, even when the integration time in the experiment greatly exceeds the reciprocal bandwidth of the accepted photons. As a result two photons cannot be detected at two points separated by a distance corresponding to an odd number of half-interference fringes. This is an interference effect that violates the laws of classical probability.
In the process of spontaneous parametric down-conversion, photons from a pump field are converted to signal and idler photon pairs in a nonlinear crystal. The reversed process, or up-conversion of these pairs back to single photons in a second crystal, is also possible. Here, we present experimental measurements of the up-conversion rate with a controlled time delay introduced between the signal and idler photons. As a function of delay, this rate presents a full width at half maximum of 27.9 fs under our experimental conditions, and we further demonstrate that group delay dispersion of the photon pairs broadens this width. These observations are in close agreement with our calculations, thus demonstrating an ultrafast, nonclassical correlation between the signal and idler waves.
By resonating both fields of the spontaneous parametric down-conversion with an optical cavity, the bandwidth of the fields is reduced to a level that can be resolved by photodetectors. This enables us to directly measure the distribution of the time intervals between the two down-converted photons. The correlation time is found inversely proportional to the down-conversion bandwidth. In the meantime, the signal levels of the fields are greatly enhanced by the resonance. Such a two-photon source will find wide application in quantum information processing.
Taking advantage of our previous experimental results and calculations that establish a new approach to the calibration of photo detectors using correlated photon pairs, we developed an experimental setup with a fast electronic control unit for the direct measurement of photon statistics. The most convenient source for generating such correlated photon pairs is a nonlinear optical process of spontaneous parametric down conversion (SPDC). When a photon of the pump beam is incident to a nonlinear crystal with phase matching condition, a pair of photons (signal and idler) is created at the same time. The photons are detected in the signal beam, and a controllable shutter is placed in the idler beam. When a detection event is made in the signal beam the fast optical shutter opens for a certain (pre-programmed) time. While the opening time of the shutter is adjustable with good time resolution, the time interval between the photons in the idler beam can be scanned, so the photon statistics can be determined.