We have developed a novel source for the generation of powerful phase-coherent light pulses. Our setup uses an acousto-optic modulator (AOM) inside an external high-finesse resonator. By applying a short rf pulse to the AOM, we dump the cavity and extract a large part of the stored and enhanced power within a short optical pulse and with a controllable optical phase. In preliminary experiments we reached 100 W of peak power in a 15-ns optical pulse. The mutual phase coherence of successive light pulses is demonstrated with a molecular iodine interferometer experiment in a cell.
We have developed a novel source for the generation of powerful phase-coherent light pulses. Our setup uses an acousto-optic modulator (AOM) inside an external high-finesse resonator. By applying a short rf pulse to the AOM, we dump the cavity and extract a large part of the stored and enhanced power within a short optical pulse and with a controllable optical phase. In preliminary experiments we reached 100 W of peak power in a 15-ns optical pulse. The mutual phase coherence of successive light pulses is demonstrated with a molecular iodine interferometer experiment in a cell.
We demonstrate a system for fast and agile digital control of laser phase, amplitude and frequency for applications in coherent atomic systems. The full versatility of a direct digital synthesis radiofrequency source is faithfully transferred to laser radiation via acousto-optic modulation. Optical beatnotes are used to measure phase steps up to 2π, which are accurately implemented with a resolution of ≤ 10 mrad. By linearizing the optical modulation process, amplitude-shaped pulses of durations ranging from 500 ns to 500 ms, in excellent agreement with the programmed functional form, are demonstrated. Pulse durations are limited only by the 30 ns rise time of the modulation process, and a measured extinction ratio of > 5 × 10(11) is achieved. The system presented here was developed specifically for controlling the quantum state of trapped ions with sequences of multiple laser pulses, including composite and bichromatic pulses. The demonstrated techniques are widely applicable to other atomic systems ranging across quantum information processing, frequency metrology, atom interferometry, and single-photon generation.
Bragg diffraction for atom interferometry conventionally requires two laser frequencies whose difference makes the two-photon transition resonant. We show that this frequency difference can instead be generated by serrodyne modulation, allowing Bragg pulses to be driven with a single-frequency laser. The serrodyne modulation is performed using an acousto-optic modulator driven with a phase-modulated RF drive, and generated kilohertz-scale frequency shifts on top of the AOM carrier frequency. While in general serrodyne modulation generates strong unwanted frequency components, we find conditions so that the Bragg diffraction pulses, and atom interferometers constructed from them, are robust to these imperfections, opening the door to the development of ultra compact, single frequency Bragg diffraction based atom interferometers with serrodyne modulation implemented by a position modulated retroreflection mirror.
A new robust laser system for mobile atom interferometers is reported. Phase modulation of a single diode laser provide two phase-coherent frequencies necessary for the Raman transition in light-pulse atom interferometers. Additional laser frequencies generated by the phase modulation, which would disturb the phase of atom interferometers, is filtered by a Fabry-Perot cavity. The two sidebands of the phase-modulated light is tuned to the adjacent resonances of the cavity and the carrier mode and even-order higher sidebands are filtered. The laser beam is then fed to a single tapered amplifier, and the two sidebands are both amplified without mode competition. The phase noise is lower than that of a state-of-the-art optically phase-locked external-cavity diode laser (-135 dBrad2/Hz at 10 kHz). This technique can be used in all-fiber-based laser systems for future mobile atom interferometers. The laser system has advantage of low phase noise, high mechanical stability, low power consumption and compactness.
Whenever scientific tools are significantly advanced; new discoveries soon follow. My thesis work relies on advances in ultrafast laser technology that allow precise control over the shape of sub 20-fs laser pulses. This laser system enabled many new experiments that yielded significant advances in attosecond science, atomic physics; extreme nonlinear optics, quantum chemistry, coherent control, molecular physics, ultrafast optical phase modulation, EUV coherent imagines, and EUV radiation sources. By using an automated learning control algorithm coupled to our deformable mirror pulse shaper; we have demonstrated the control of a process on an attosecond time-scale for the first time. We demonstrate the manipulation of the phase of an electron wave packet, allowing us to tailor the EUV spectrum generated by high-order harmonic generation. These optimal fields were discovered by a learning algorithm that both found an unknown optimal solution; but also discovered an unknown phase-matching mechanism that occurs in the interaction of a single atom and light pulse. We control molecular vibrational and rotational coherences with the same learning algorithm; demonstrating selective control in room temperature molecules at atmospheric pressures. Moreover, we demonstrate that modifications to the algorithm can help automatically uncover the physics of the control mechanism found by the learning algorithm. We also demonstrate a new pulse-compression technique using rotational phase modulation, where optical pulses were compressed by an order of magnitude after phase modulation by a molecular rotational coherence and subsequent propagation through a transparent window. This technique will enable efficient pulse compression in the deep-UV. Finally, we measure the coherence of EUV light generated by high-harmonic upconversion of a femtosecond laser. In phase-matched hollow-fiber geometry, the EUV light exhibits the highest inherent spatial coherence of any source in this region of the spectrum. We use this source to demonstrate the coherent image with first table-top EUV radiation. Since this source exhibits full spatial coherence at very short wavelength, this light source represents has smallest inherent effective source-size of any light source yet created. We also demonstrate that the spectrum of an optical field can be determined by measuring the interference of a double-slit pattern.
We will describe a next-generation active atomic frequency reference based on super-radiant pulses of laser light from the ultra-narrow, 1 mHz linewidth, optical clock transition in an ensemble of cold 87Sr atoms. Light is stimulated from the millihertz linewidth transition by confining an ensemble of laser cooled atoms inside of a high finesse optical cavity. Such a light source has been proposed as a next-generation active atomic frequency reference, with the potential to enable high-precision optical frequency references to be used outside laboratory environments. We achieve a remarkable short term fractional frequency stability, 6.7 × 1016 at 1 s of averaging, absolute accuracy, 2 Hz (4 × 1015 fractional frequency), and high insensitivity to changes in the cavity length that limits the performance of todays more stable lasers. We will also discuss current work on cavity-enhanced dispersive measurements to perform high resolution spectroscopy and atom counting.
Abstract Ultrashort, coherent light pulses in the extreme ultraviolet (XUV) wavelength region are excellent tools for a wide range of experiments. These XUV pulses are in particular used to characterize electron dynamics. Additionally, the high photon energy enables quantum control of short-lived transitions in atoms. These transitions are of interest for ultrafast quantum control as the bandwidth of the control pulses needs to be less than the transition frequency. Coherent XUV pulses would be even more useful if the tools to control and manipulate them existed. Presently, however, no modulators exist for these frequencies, which significantly reduces the number of possible ultrafast optics experiments and applications in the XUV regime. This Ph.D. tutorial addresses this problem and focuses on the control of XUV light in time and space. To enable control of XUV light we have developed a method for opto-optical modulation (OOM), which modulates the phase of XUV light emitted from a gas of atoms. The atoms are resonantly excited with a coherent XUV pulse generated through high order harmonic generation and emit light after the excitation pulse passed. By shifting the resonance frequencies through the AC Stark shift with a non-resonant infrared control pulse, the phase of the emitted light, and therefore its wavefront, is controlled. With OOM the direction of XUV light emitted from noble gases has been controlled, and the temporal dynamics of the emission studied. By varying the delay between the excitation and the control pulse, the time of redirection was controlled, which enabled high signal to noise study of the temporal dynamics of the emission. Furthermore, a proof-of-principle experiment with two control pulses was performed, resulting in a shaped XUV pulse with controlled duration. The technique of OOM presented in this article is still at a very early stage and in order to obtain complete control of the amplitude and phase of the XUV pulses further development is necessary. Such development would present new opportunities for ultrafast XUV quantum control.