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Physical Review A

Radiative cascade of highly excited hydrogen atoms in strong magnetic fields

Türker Topçu, F. Robicheaux

Published Apr 10, 2006• 31 citations
Publisher

Abstract

We have studied the radiative decay of atomic hydrogen in strong magnetic fields of up to $4\phantom{\rule{0.3em}{0ex}}\mathrm{T}$. We have followed the radiative cascade from completely $l,m$ mixed distributions of highly excited states as well as from distributions that involve highly excited states with $\ensuremath{\mid}m\ensuremath{\mid}\ensuremath{\sim}n$. We have found that the time it takes to populate the ground state is not affected by the magnetic field for the initial states with $n\ensuremath{\lesssim}20$. For higher $n$ manifolds, the electrons in the most negative $m$ states are substantially slowed down by the magnetic field resulting in a much longer lifetime. We show that less than 10% of the antihydrogen atoms with $n\ensuremath{\sim}35$ generated in antihydrogen experiments at $4\phantom{\rule{0.3em}{0ex}}\mathrm{K}$ will decay to their ground states before they hit the wall of the vacuum container unless they are trapped. We have also found that the decay time is mainly determined by the fraction of atoms that were initially in highest negative $m$ states due to the fact that only $\ensuremath{\mid}\ensuremath{\Delta}m\ensuremath{\mid}+\ensuremath{\mid}\ensuremath{\Delta}\ensuremath{\pi}\ensuremath{\mid}=1$ transitions are allowed in the magnetic field. We give a semiclassical method for calculating the decay rates for circular states and show that when the initial states have high-$\ensuremath{\mid}m\ensuremath{\mid}$, semiclassical rates agree with the full quantum mechanical rates within a couple of percent for states with effective $n\ensuremath{\gtrsim}20$.

DOI
10.1103/physreva.73.043405

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The dynamics of (de)excitation between highly excited Rydberg states (15<n<6015<n<6015<n<60 of Rb) in a magnetic field of 0.85 $\ifmmode\pm\else\textpm\fi{}0.05\phantom{\rule{0.3em}{0ex}}\mathrm{T}$ is studied with far-infrared pulses (90--110 and $50\phantom{\rule{0.3em}{0ex}}\mathrm{\ensuremath{\mu}}\mathrm{m}$) originating from a free electron laser. We measured the excitation spectrum to states around n=40n=40n=40 from a deeper bound state near n=25n=25n=25. Moreover, starting from a highly excited state (30<n<60)(30<n<60)(30<n<60) below and in the nnn-mixing regime we investigated the efficiency of the deexcitation channel vs the ionization channel. We measured deexcitation efficiencies well above 50% for some of the states. However, starting deep in the nnn-mixing regime the deexcitation efficiency is less than 10%. The measurements were in good agreement with fully quantum mechanical calculations. Calculations for deexcitation of n=35n=35n=35 states in H found the largest amount of deexcitation for m=0m=0m=0 and almost none for m=20m=20m=20. In recent experiments at CERN, antihydrogen is produced in high nnn states in a strong magnetic field with a wide distribution of mmm. Our measurements and calculations suggest that deexcitation stimulated by infrared photons is not an efficient method for accelerating cascade to the ground state.
Using a classical Monte Carlo method, we have computed the three-body recombination (two free electrons and a proton scattering into one free electron and a hydrogen atom, $e+e+p\ensuremath{\rightarrow}\mathrm{H}+e$) in strong magnetic fields. The proton is fixed in space but the electrons are allowed their full, three-dimensional motion. We investigate recombination for temperatures and fields similar to those used in recent experiments that generated antihydrogen. The present rate is compared to that when the electrons' motion is given by the guiding center approximation, validating previous results at low temperature and demonstrating the breakdown of this approximation at higher temperature. Unlike the B=0B=0B=0 case, strong BBB gives preferential recombination to atoms with positive magnetic moment. Also, the canonical angular momentum in the field direction is often negative even when the magnetic moment is negative. Both results affect the trapping of antihydrogen using spatially dependent magnetic fields.
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We have simulated the centre-of-mass motion of Rydberg anti-hydrogen atoms in spatially varying magnetic fields. We find that a population of anti-hydrogen can lose substantial centre-of-mass kinetic energy during the radiative cascade to the ground state. The loss of energy is due to the change in magnetic moment when photons are emitted and is akin to adiabatic cooling. We also simulate the pattern of anti-hydrogen hits on the walls of the trap and find that the existence of trapped Rydberg atoms leads to a distinctive distribution along the trap axis.
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We have simulated the motion of a Rydberg hydrogen atom in electric and magnetic fields that have a strong position dependence. The orientation and strengths of the fields depend strongly on the spatial position of the atom. The angle between the fields could take on any value. We use the quantum energy levels for a Rydberg state in electric and magnetic fields to derive a spatially dependent potential energy for the centre-of-mass motion of the atom. We compute the radiative decay rate into states with low principal quantum numbers. After the decay, the atom could be trapped using the magnetic moment of the electron. We present results for a specific trap geometry which could be experimentally realized.