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Soviet Physics Uspekhi

Interference of Atomic States

Evgenii B. Aleksandrov, O. V. Konstantinov, V. I. Perel

Published Jan 1, 1970• 132 citations
Publisher

Abstract

This monograph is devoted to the description and interpretation of interference between quantum states of an atom, as manifested in the angular distribution and polarization of spontaneous emission and absorption. The basic phenomena are first introduced and explained in terms of the simple classical dipole model. A more quantitative description follows, making use of the density matrix formalism and the statistical tensor. The theoretical sections are complemented by detailed accounts of experimental methods and results, such that the monograph as a whole gives a comprehensive picture of this field.

DOI
10.1070/pu1970v013n02abeh004212

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This monograph is devoted to the description and interpretation of interference between quantum states of an atom, as manifested in the angular distribution and polarization of spontaneous emission and absorption. The basic phenomena are first introduced and explained in terms of the simple classical dipole model. A more quantitative description follows, making use of the density matrix formalism and the statistical tensor. The theoretical sections are complemented by detailed accounts of experimental methods and results, such that the monograph as a whole gives a comprehensive picture of this field.
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A density-matrix approach is developed to provide a theoretical description of the intensity, angular distribution, and polarization of superradiative emission from an ensemble of many-electron atomic systems. The many-electron atomic systems are described as cooperatively interacting by means of forces that can be long range. Particular emphasis is given to the coherent excitation of the collective atomic-ensemble states, which may be produced by incident laser radiation. The initial excitation and spontaneous emission processes may be described as independent. Both frequency-domain and time-domain formulations of the density-matrix approach are developed. The collective atomic-ensemble states are specified in a detailed hyperfine representation, corresponding to successively coupling the individual hyperfine angular momenta F pertaining to the many-electron atoms. A less detailed fine-structure angular-momentum representation may also be used. In the density-operator approach, account can be taken of the coherent excitation of a particular subspace of the initial atomic-ensemble states. For a comprehensive and unified development of time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations, a reduced-density-matrix (quantum-open-systems) approach is introduced. The non-equilibrium atomic-ensemble-state kinetics and the homogeneous spectral-line shapes can thereby be systematically and self-consistently determined. The collective atomic-ensemble states may be obtained using a variety of different methods. These states can be determined using a dressed-state approach, in which the required states are calculated in the presence of an electromagnetic field.
The field of quantum optics has witnessed significant theoretical and experimental developments in recent years. This book provides an in-depth and wide-ranging introduction to the subject, emphasising throughout the basic principles and their applications. The book begins by developing the basic tools of quantum optics, and goes on to show the application of these tools in a variety of quantum optical systems, including lasing without inversion, squeezed states and atom optics. The final four chapters are devoted to a discussion of quantum optical tests of the foundations of quantum mechanics, and to particular aspects of measurement theory. Assuming only a background of standard quantum mechanics and electromagnetic theory, and containing many problems and references, this book will be invaluable to graduate students of quantum optics, as well as to researchers in this field.
This chapter begins with a brief outline of some of the key motivations for considering a quantum theory: the early attempts to determine the spectral distribution of energy density of black bodies; stability of atoms and molecules; specific heats of solids; interference and diffraction of light beams; polarization of photons. The experimental foundations of wave mechanics are then presented in detail, but in a logical order quite different from its historical development: photo-emission of electrons by metallic surfaces, X- and γ-ray scattering from gases, liquids and solids, interference experiments, atomic spectra and the Bohr hypotheses, the experiment of Franck and Hertz, the Bragg experiment, diffraction of electrons by a crystal of nickel (Davisson and Germer), and measurements of position and velocity of an electron. The need for a quantum theory In the second half of the nineteenth century it seemed that the laws of classical mechanics, developed by the genius of Newton, Lagrange, Hamilton, Jacobi and Poincaré, the Maxwell theory of electromagnetic phenomena and the laws of classical statistical mechanics could account for all known physical phenomena. Still, it became gradually clear, after several decades of experimental and theoretical work, that one has to formulate a new kind of mechanics, which reduces to classical mechanics in a suitable limit, and makes it possible to obtain a consistent description of phenomena that cannot be understood within the classical framework. It is now appropriate to present a brief outline of this new class of phenomena, the systematic investigation of which is the object of the following sections and of chapters 4 and 14.