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Physical Review Letters

Ultrafast Fourier Transform with a Femtosecond-Laser-Driven Molecule

Kouichi Hosaka, Hiroyuki Shimada, H. Chiba, Hiroyuki Katsuki, Yoshiaki Teranishi, Yukiyoshi Ohtsuki, Kenji Ohmori

Published May 3, 2010• 46 citations
Publisher

Abstract

Wave functions of electrically neutral systems can be used as information carriers to replace real charges in the present Si-based circuit, whose further integration will result in a possible disaster where current leakage is unavoidable with insulators thinned to atomic levels. We have experimentally demonstrated a new logic gate based on the temporal evolution of a wave function. An optically tailored vibrational wave packet in the iodine molecule implements four- and eight-element discrete Fourier transform with arbitrary real and imaginary inputs. The evolution time is 145 fs, which is shorter than the typical clock period of the current fastest Si-based computers by 3 orders of magnitudes.

DOI
10.1103/physrevlett.104.180501

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Wave functions of electrically neutral systems can be used as information carriers to replace real charges in the present Si-based circuit, whose further integration will result in a possible disaster where current leakage is unavoidable with insulators thinned to atomic levels. We have experimentally demonstrated a new logic gate based on the temporal evolution of a wave function. An optically tailored vibrational wave packet in the iodine molecule implements four- and eight-element discrete Fourier transform with arbitrary real and imaginary inputs. The evolution time is 145 fs, which is shorter than the typical clock period of the current fastest Si-based computers by 3 orders of magnitudes.
We numerically propose a way to perform quantum computations by combining an ensemble of molecular states and weak laser pulses. A logical input state is expressed as a superposition state (a wave packet) of molecular states, which is initially prepared by a designed femtosecond laser pulse. The free propagation of the wave packet for a specified time interval leads to the specified change in the relative phases among the molecular basis states, which corresponds to a computational result. The computational results are retrieved by means of quantum interferometry. Numerical tests are implemented in the vibrational states of the B state of I2 employing controlled-NOT gate, and 2 and 3 qubits Fourier transforms. All the steps involved in the computational scheme, i.e., the initial preparation, gate operation, and detection steps, are achieved with extremely high precision.
The quantum interference of two molecular wave packets has been precisely controlled in the B electronic state of the I2 molecule by using a pair of fs laser pulses whose relative phase is locked within the attosecond time scale and its real-time evolution has been observed by another fs laser pulse. It is clearly observed that the temporal evolution changes drastically as a function of the relative phase between the locked pulses, allowing us to read both amplitude and phase information stored in the wave functions of the molecular ensemble.
We propose an implementation of the quantum fast Fourier transform algorithm in an entangled system of multilevel atoms. The Fourier transform occurs naturally in the unitary time evolution of energy eigenstates and is used to define an alternative wave-packet basis for quantum information in the atom. A change of basis from energy levels to wave packets amounts to a discrete quantum Fourier transform within each atom. The algorithm then reduces to a series of conditional phase transforms between two entangled atoms in mixed energy and wave-packet bases. We show how to implement such transforms using wave-packet control of the internal states of the ions in the linear ion-trap scheme for quantum computing.
Unlike classical digital computers in which a bit can represent either 1 or 0 at any time, quantum computers use a two-level system, i.e., a qubit, to implement logical operations based on quantum mechanical laws, which can represent both values at once. Owing to the superposition property of qubits, quantum computers have natural parallel processing advantages and thus have potential to exceed the computational efficiency of classical computers for particular tasks. Quantum logic gates are the generalization of classical logic gates in computational networks. It has been proved that two-qubit quantum gates together with one-qubit quantum gates are adequate for constructing networks with any possible quantum computational property. Directional couplers are the most critical elementsfor constructing the quantum gates. In recent years, photonic quantum technologies have emerged as a promising experimental platform for quantum computing. Single photons have robust noise resistance, long coherence time, high transmission speed and great compatibility with other systems. They can be easily manipulated and encoded in any of several degrees of freedom, for example, polarization, path, spatial mode or time bin. Optical waveguide technology enables the realizing of complex optical schemes comprised of many elements with desired scalability, stability and miniaturization. Femtosecond laser direct writing of waveguide has been adopted as a powerful tool for integrated quantum photonics with characteristics of rapidness, cost-effectiveness, mask-less and single-step process. In particular, it has the ability to build arbitrary three-dimensional circuits directly inside bulk materials, which is impossible to achieve with conventional lithography. In this article we review the femtosecond laser writing and quantum characterization of directional coupler and important one-qubit and two-qubit optical quantum logic gates, such as Hadamard gate, Pauli-X gate, controlled-NOT gate, and controlled-Phase gate. The qubits in these gates are usually encoded through optical paths or polarizations of photons. The key to the realization of polarization-encoded one-qubit gates is to achieve flexible wave-plate operations, which is described in detail. Controlled-NOT gate and controlled-phase gate are the most crucial two-qubit gates in the linear optics computation and sometimes they can be converted into each other by adding some one-qubit gates or special superposition states. Many different kinds of waveguide circuits have been used to implement these two-qubit gates. The outlook and challenges for the femtosecond laser writing of three-qubit gates, such as Toffoli gate and Fredkin gate, are briefly introduced.
We demonstrate an experimental approach to read and write populations and relative phases of vibrational eigenstates within a wave packet created in the BBB state of the iodine molecule by using a pair of phase-locked femtosecond laser pulses. Our highly stabilized optical interferometer provides attosecond stability and resolution in the interpulse delay. The stability and resolution have realized an exquisite tuning of the interference of two vibrational wave packets to manipulate the relative populations and the relative quantum phases among the vibrational eigenstates within the wave packets. These populations and phases have been retrieved by measuring fluorescence from the upper EEE state induced by another nanosecond (ns) or femtosecond (fs) probe laser pulse. The bandwidth of the ns probe pulse is narrow enough to select only a small portion of the rotational progression of a particular vibrational band of the $E\ensuremath{-}B$ transition. By scanning the probe wavelength, we measure the population distribution of the vibrational eigenstates within the wave packet. The fs probe pulse is used to measure quantum beats arising from the temporal evolution of the wave packet. Combining these two complementary measurements, we can read both population and phase information written and stored in the wave packet.