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Physical Review Letters

Energy Decay in Superconducting Josephson-Junction Qubits from Nonequilibrium Quasiparticle Excitations

John M. Martinis, M. Ansmann, José Aumentado

Published Aug 26, 2009• 246 citations
Publisher

Abstract

We calculate the energy decay rate of Josephson qubits and superconducting resonators from nonequilibrium quasiparticles. The decay rates from experiments are shown to be consistent with predictions based on a prior measurement of the quasiparticle density n(qp) = 10/microm(3), which suggests that nonequilibrium quasiparticles are an important decoherence source for Josephson qubits. Calculations of the energy-decay and diffusion of quasiparticles also indicate that prior engineered gap and trap structures, which reduce the density of quasiparticles, should be redesigned to improve their efficacy. This model also explains a striking feature in Josephson qubits and resonators-a small reduction in decay rate with increasing temperature.

DOI
10.1103/physrevlett.103.097002

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We calculate the energy decay rate of Josephson qubits and superconducting resonators from nonequilibrium quasiparticles. The decay rates from experiments are shown to be consistent with predictions based on a prior measurement of the quasiparticle density n(qp) = 10/microm(3), which suggests that nonequilibrium quasiparticles are an important decoherence source for Josephson qubits. Calculations of the energy-decay and diffusion of quasiparticles also indicate that prior engineered gap and trap structures, which reduce the density of quasiparticles, should be redesigned to improve their efficacy. This model also explains a striking feature in Josephson qubits and resonators-a small reduction in decay rate with increasing temperature.
We calculate the energy decay rate of Josephson qubits and superconducting resonators from non-equilibrium quasiparticles. The decay rates from experiments are shown to be consistent with predictions based on a prior measurement of the quasiparticle density n_qp = 10/um^3, which suggests that non-equilibrium quasiparticles are an important decoherence source for Josephson qubits. Calculations of the energy-decay and diffusion of quasiparticles also indicate that prior engineered gap and trap structures, which reduce the density of quasiparticles, should be redesigned to improve their efficacy. This model also explains a striking feature in Josephson qubits and resonators - a small reduction in decay rate with increasing temperature.
Quasiparticles are an important decoherence mechanism in superconducting qubits, and can be described with a complex admittance that is a generalization of the Mattis-Bardeen theory. By injecting nonequilibrium quasiparticles with a tunnel junction, we verify qualitatively the expected change of the decay rate and transition frequency in a phase qubit. With their relative change in agreement to within 4 % of prediction, the theory can be reliably used to infer quasiparticle density. We describe how settling of the decay rate may allow determination of whether qubit energy relaxation is limited by nonequilibrium quasiparticles.
Superconducting qubits hold promise for quantum computing, but their operation is challenged by various sources of noise, including excitations known as quasiparticles. Qubits with gap asymmetry larger than their transition energy are less susceptible to quasiparticle decoherence as the quasiparticles are mostly trapped in the low-gap side of the junction. Because of this trapping, the gap asymmetry can contribute to maintaining the quasiparticles out of equilibrium. Here we address the temperature dependence of the quasiparticle densities in the two sides of the junction. We show that four qualitatively different regimes are possible with increasing temperature: (i) nonequilibrium, (ii) local quasiequilibrium, (iii) global quasiequilibrium, and (iv) full equilibrium. We identify shortcomings in assuming global quasiequilibrium when interpreting experimental data, highlighting how measurements in the presence of magnetic field can aid the accurate determination of the junction parameters, and hence the identification of the nonequilibrium regimes. Quasiparticle poisoning challenges the operation of superconducting qubits, but errors can be suppressed by engineering gap asymmetry between the electrodes of the qubit’s Josephson junction. The authors present a model of the qubit-quasiparticle system valid beyond the low-temperature limit and identify different nonequilibrium regimes, which can affect the interpretation of experimental data.
Quasiparticles, especially the ones near the Josephson junctions in the superconducting qubits, are known as an important source of decoherence. By injecting quasiparticles into a quantum chip, we characterized the diffusion feature by measuring the energy relaxation time and the residual excited-state population of a transmon qubit. From the extracted transition rates, we phenomenologically modeled the quasiparticle diffusion in a superconducting circuit that contained “hot” nonequilibrium quasiparticles in addition to low-energy ones.
Superconducting qubits probe environmental defects such as nonequilibrium quasiparticles, an important source of decoherence. We show that "hot" nonequilibrium quasiparticles, with energies above the superconducting gap, affect qubits differently from quasiparticles at the gap, implying qubits can probe the dynamic quasiparticle energy distribution. For hot quasiparticles, we predict a non-negligible increase in the qubit excited state probability Pe. By injecting hot quasiparticles into a qubit, we experimentally measure an increase of Pe in semiquantitative agreement with the model and rule out the typically assumed thermal distribution.
The quasiparticle density observed in low-temperature superconducting circuits is several orders of magnitude larger than the value expected at thermal equilibrium. The tunneling of this excess of quasiparticles across Josephson junctions is recognized as one of the main loss and decoherence mechanisms in superconducting qubits. Here we present a unified impedance theory that accounts for quasiparticle energy loss in circuit regions both far from and near to (across) junctions. Our theory leverages the recent experimental demonstration that the excess quasiparticles are in quasiequilibrium [Connolly et al., Phys. Rev. Lett. 132, 217001 (2024)] and uses a generalized fluctuation-dissipation theorem to predict the amount of charge and flux noise generated by them. We compute the resulting energy relaxation time T1{T}_{1}T1​ in transmon qubits with and without junction asymmetric gap engineering, and show that quasiparticles residing away from junctions can play a dominant role in the former case. They also may provide an upper limit for resonator quality factors if the density of amorphous two-level systems is reduced. In addition, we show that charge noise from quasiparticles leads to flux noise that is logarithmic in frequency, giving rise to a ``nearly white'' contribution that is comparable to the flux noise observed in flux qubits. This contrasts with amorphous two-level systems, whose associated flux noise is shown to be super-Ohmic. We discuss how this quasiparticle flux noise can limit ${T}_{2}^{\ensuremath{\ast}}$ coherence times in flux-tunable qubits. The final conclusion is that asymmetric gap engineering can greatly reduce noise and increase coherence times in superconducting qubits.