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Journal of Modern Optics

Level Crossing in a Frequency-dependent Photon Reservoir

Jakub Zakrzewski, T. Dohnalik

Published Jul 1, 1991• 0 citations
Publisher

Abstract

The level-crossing effect for a three-level atom placed into the resonant cavity (waveguide) and illuminated by a strong monochromatic laser light is discussed. The cavity plays the role of a frequency-dependent photon reservoir that modifies the spontaneous decay of the atom. The effect is studied by considering the modifications of the level-crossing (Hanle effect) signals. The non-Markovian character of spontaneous emission in frequency-dependent reservoirs is taken into account. Calculated signals are interpreted in terms of a dressed atom picture.

DOI
10.1080/09500349114551481

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The level-crossing effect for a three-level atom placed into the resonant cavity (waveguide) and illuminated by a strong monochromatic laser light is discussed. The cavity plays the role of a frequency-dependent photon reservoir that modifies the spontaneous decay of the atom. The effect is studied by considering the modifications of the level-crossing (Hanle effect) signals. The non-Markovian character of spontaneous emission in frequency-dependent reservoirs is taken into account. Calculated signals are interpreted in terms of a dressed atom picture.
A two-level atom coupled to a reservoir with Lorentzian spectral response function is considered. It is shown that if the free oscillations of the atomic dipole are suitably modulated by an external field, then the dynamics of the spontaneous decay can be strongly modified. As a result, the probability of finding the atom in an excited state can be large even for very long times. This is because the frequency modulation may lead to both effective detuning of the atom from the resonance with reservoir modes and to effective cancellation of the coupling between the atom and the reservoir. Non-Markovian features of the reservoir are found to be essential for this effect to be observable. Conditions of experimental verifications are provided.
Interesting new aspects of atomic behavior in the presence of strong driving fields appear when the driven atom resides not in free space, but in a region (such as an optical cavity) that displays a frequency-dependent photon-mode density. Under such conditions, it is found that a strong driving field can modify the spontaneous decay properties of an atom, and thereby give rise to interesting new features in the spectrum of strong-field resonance fluorescence. It is also found that a high level of dressed-state polarization can be maintained in a sample of resonantly or nonresonantly driven atoms by appropriate tuning of an enclosing cavity. Furthermore, for appropriate laser and cavity tunings, it is found that the atomic states become highly squeezed. In the course of analyzing these effects, a set of modified Bloch equations is derived that explicitly accounts for the finite response time associated with a frequency-dependent photon-mode density.
We study the spontaneous emission of atoms coupled to frequency-dependent photon-mode reservoirs, and find atomic emission spectra qualitatively different from those of free space. Frequency-dependent photon-mode reservoirs are found in a variety of physical situations (e.g., in waveguides, microcavities, dielectrics, systems with photonic spectral gaps, etc.), and are shown to lead to nonexponential decay and concomitant complicated non-Lorentzian emission line shapes. By studying Autler-Townes spectra in the presence of a frequency-dependent photon-mode density, we present simple examples of dynamical modifications of spontaneous decay properties.
Complete density-matrix equations and a one-photon counting probability are used to examine the photon statistics of fluorescence light of a single three-level atom, weakly coupled to an external cavity of low QQQ value. The internal structure of the atom is supposed to be characterized by a weak and a strong transition. The strong transition is coherently driven by an external laser field, whereas no external field is acting on the weak transition. In free space the system exhibits quantum jumps. By placing the atom within the mirrors of an external cavity, tuned close to the transition frequency of the two upper levels, modifications in the quantum jump behavior of the atom are shown due to a modified spontaneous decay rate between the two states. In particular, it is demonstrated that the effect of the cavity is to modify the repetition rate of quantum jumps into the metastable dark state and the average duration of bright periods of fluorescence, whereas the average duration of dark periods is not changed in first order of the spontaneous decay rates involved. In view of current experiments in our laboratory a quantitative analysis is presented for the special case of a single indium ion located between the mirrors of a high-order symmetric confocal cavity.
The spontaneous emission spectrum for a three-level cascade configuration atom in a single mode high-Q cavity coupled to a zero temperature reservoir of continuum external modes is determined from the atom–cavity mode master equation using the quantum regression theorem. Initially the atom is in its upper state and the cavity mode empty of photons. Following Glauber, the spectrum is defined via the response of a detector atom. Spectra are calculated for the detector located inside the cavity (case A), outside the cavity end mirror (case B—end emission), or placed for emission out the side of the cavity (case C). The spectra for case A and case B are found to be essentially the same. In all the cases the predicted lineshapes are free of instrumental effects and only due to cavity decay. Spectra are presented for intermediate and strong coupling regime situations (where both atomic transitions are resonant with the cavity frequency), for cases of non-zero cavity detuning, and for cases where the two atomic transition frequencies differ. The spectral features for cases B(A) and C are qualitatively similar, with six spectral peaks for resonance cases and eight for detuned cases. These general features of the spectra can be understood via the dressed atom model. However, case B and C spectra differ in detail, with the latter exhibiting a deep spectral hole at the cavity frequency due to quantum interference effects.
We investigate a cavity mode that interacts with a three-level atom in an open cavity that is coupled to a vacuum reservoir and is driven by coherent light. In our analysis, the interaction of the three-level atom with the external vacuum reservoir is taken into account and the noise operators of the vacuum reservoir are placed in normal order. While the spontaneous emission rate fluctuates as [Formula: see text], [Formula: see text], [Formula: see text], and [Formula: see text], the cavity damping constant and stimulated emission decay constant, both set to 0.8, govern the system dynamics. Both the plus and negative components of the cavity light display quadrature squeezing. For coherent driving strengths [Formula: see text] and [Formula: see text] at [Formula: see text], and [Formula: see text] at [Formula: see text], the plus quadrature exhibits [Formula: see text] squeezing below the vacuum level, indicating that increasing the coherent drive can compensate for the decoherence introduced by spontaneous emission. Moreover, for [Formula: see text], the minus quadrature achieves [Formula: see text] squeezing. At high driving strengths, the squeezing in both quadratures becomes independent of spontaneous emission. In the absence of spontaneous emission, the mean photon number increases, and the photon number distribution shows a higher probability for even photon numbers than for odd ones, with the overall distribution decreasing as the photon number increases.