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Optics Letters

Lock-in detection of single photons after two-step frequency conversion

Andreas Lenhard, Sebastian Zaske, Christoph Becher

Published Oct 9, 2012• 4 citations
Publisher

Abstract

We report on cascaded frequency conversion at the single-photon level, consisting of a downconversion from the red (738 nm) to a telecom band (1403 nm) and the reverse upconversion process in the same nonlinear crystal. Detecting the converted single photons suffers from a large noise floor. We were able to recover the signal by implementing a lock-in analyzer technique in the data postprocessing.

DOI
10.1364/ol.37.004254

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We report on cascaded frequency conversion at the single-photon level, consisting of a downconversion from the red (738 nm) to a telecom band (1403 nm) and the reverse upconversion process in the same nonlinear crystal. Detecting the converted single photons suffers from a large noise floor. We were able to recover the signal by implementing a lock-in analyzer technique in the data postprocessing.
We present a device for two-stage frequency upconversion of single-photon-level signals in the 1.55 μm telecom band to the green spectral region with low excess noise, suitable for detection by low-timing-jitter silicon single-photon avalanche photodiodes (APDs). We achieve a net conversion efficiency of 87% and a system timing jitter below 70 ps FWHM, dominated by the jitter of the APD. Modifications of our device are suitable for downconversion of single photons from visible-wavelength quantum emitters into the telecom band.
We propose a method of single photon detection of infrared (IR) photons at potentially higher efficiencies and lower noise than allowed by traditional IR band Avalanche Photodiodes (APD). By up-converting the photon from IR, e.g., 1550 nm, to a visible wavelength in a nonlinear crystal, we can utilize the much higher efficiency of visible wavelength APDs. We have used a nonlinear crystal -- Periodically Poled Lithium Niobate (PPLN) -- and a pulsed 1064-nm Nd:YAG laser to perform the up-conversion to a 631-nm photon. When properly quasi-phase-matched, PPLN provides a large enough second order nonlinear susceptibility that near unit conversion efficiency of the IR photon into the visible should be possible. We have been able to observe peak conversion efficiencies as high as 80%, and have demonstrated scaling down to the single photon level while maintaining a background of 3 x 10-4 dark counts/count. Since the PPLN only acts on one polarization of the single photon, we also propose a 2-crystal extension of this scheme whereby orthogonal polarizations may be up-converted coherently, thereby enabling complete quantum state transduction.
We report on an experiment demonstrating storage of single-photonlevel light pulses at telecommunication wavelength by frequency up-converting them to the visible range to be resonant with a solid-state optical memory based on a Pr:Y2SiO5 crystal. We convert the telecom photons at 1570 nm to 606 nm using a periodically-poled potassium titanyl phosphate nonlinear waveguide. The maximum device efficiency is inferred to be η dev = 22±1% with a signal to noise ratio exceeding 1 for single-photon-level pulses with durations of up to 560 ns. The converted light is then stored in the crystal using the atomic frequency comb scheme with storage and retrieval efficiencies exceeding ηAFC = 20% for predetermined storage times of up to 5μs. The retrieved light is time delayed from the noisy conversion process allowing us to measure a signal to noise ratio exceeding 100 with telecom single-photon-level inputs. These results represent the first demonstration of single-photon-level optical storage interfaced with frequency up-conversion. PACS numbers: 03.67.Hk,42.50.Gy,42.50.Md,42.65.Wi
We propose a method of single photon detection of infrared (IR) photons at potentially higher efficiencies and lower noise than allowed by traditional IR band avalanche photodiodes (APDs). By up-converting the photon from the IR, e.g. 1550 nm, to a visible wavelength in a nonlinear crystal, we can utilize the much higher efficiency of silicon APDs at these wavelengths. We have used a periodically poled lithium niobate (PPLN) crystal and a pulsed 1064 nm Nd:YAG laser to perform the up-conversion to a 631 nm photon. We observed conversion efficiencies as high as ∼ 80%, and demonstrated scaling down to the single photon level while maintaining a background of 3 ×s; 10−4 dark counts per count. We also propose a 2-crystal extension of this scheme, whereby orthogonal polarizations may be up-converted coherently, thus enabling complete quantum state transduction of arbitrary states.
A single-photon signal at 1.55 microm was converted to the visible region by sum-frequency mixing with a strong pumping beam at 1064 nm in a periodically poled lithium niobate crystal placed in a diode-pumped Nd:YVO4 laser cavity. As the intracavity pump laser could be automatically stabilized without cavity lock, robust long-term stability was demonstrated for single-photon frequency upconversion, with a conversion efficiency of 74.3%. Such a stable single-photon upconversion was demonstrated to be efficient and robust for single-photon counting at 1550 nm, and the corresponding background noise was measured at less than 420 x 10(3) s(-1).