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Physical Review Letters

Trapping Excitons in a Two-Dimensional In-Plane Harmonic Potential: Experimental Evidence for Equilibration of Indirect Excitons

Z. Vörös, David W. Snoke, Loren N. Pfeiffer, K. W. West

Published Jul 7, 2006• 79 citations
Publisher

Abstract

We have trapped a gas of long-lifetime, high-mobility excitons in an in-plane harmonic potential. Trapping is an important step toward the goal of a controlled Bose-Einstein condensate of excitons. We show that the repulsive interaction between the excitons plays a dominant role in the behavior of the excitons, in contrast with the weak interactions in atomic gases. We show that under proper conditions the excitons thermalize in the trap to a well-defined equilibrium spatial distribution.

DOI
10.1103/physrevlett.97.016803

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We study the condensation of a two-dimensional exciton gas in a harmonic trap using a quantum Boltzmann equation. The excitons interact with a lattice that is kept at a constant temperature and we also include exciton–photon coupling (dissipation) and exciton–exciton interactions. We compare the condensation time for both an interacting and a non-interacting exciton gas. For a non-interacting gas anti-Stokes type processes dominate the relaxation rate of low-energy states. The condensation time-scale is determined by the (phonon) scattering rate into the ground state. The presence of dissipation results in a heating effect which increases the mean number of Bose particles required for the onset of condensation. For a dissipative gas the steady state is a nonequilibrium condensate (exciton matter laser), where the exciton temperature remains above the lattice temperature. We also discuss the effects of dimensionality and trapping on the relaxation process, which has a fundamental role in establishing the condensation time-scale.

physica status solidi (a)•Nov 1, 1997•5 citations
We have trapped a gas of long-lifetime, high-mobility excitons in an in-plane harmonic potential. Trapping is an important step toward the goal of a controlled Bose-Einstein condensate of excitons. We show that the repulsive interaction between the excitons plays a dominant role in the behavior of the excitons, in contrast with the weak interactions in atomic gases. We show that under proper conditions the excitons thermalize in the trap to a well-defined equilibrium spatial distribution.
Recent experiments have shown that it is possible to create an in-plane harmonic potential trap for a two-dimensional (2D) gas of exciton polaritons in a microcavity structure, and evidence has been reported of Bose-Einstein condensation of polaritons accumulated in this type of trap. We present here the theory of Bose-Einstein condensation (BEC) and superfluidity of the exciton polaritons in a harmonic potential trap. Along the way, we determine a general method for defining the superfluid fraction in a 2D trap, in terms of angular momentum representation. We show that in the continuum limit, as the trap becomes shallower, the superfluid fraction approaches the 2D Kosterlitz--Thouless limit, while the condensate fraction approaches zero, as expected.
Summary form only given. In the dilute limit excitons behave as weakly interacting Bose particles and are expected to undergo the Bose-Einstein condensation (BEC). Because the exciton mass is very small at experimentally accessible exciton densities the critical temperature for exciton BEC should reach several Kelvins, i.e., about six orders of magnitude higher than the T/sub c/ for atom BEC. To create degenerate Bose-gas of excitons we propose quasi-2D gas of indirect excitons in coupled quantum wells (CQWs) which have two primary advantages for realizing a quantum degenerate exciton gas and, ultimately, the BEC-like phase transition: (i) the long lifetime of indirect excitons and (ii) the short exciton cooling time.
This thesis includes theoretical studies regarding stability and manipulation of Bose-Einstein condensates (BECs) of ultra-cold atoms in 2D trapping geometry, as well as formation of steady states of exciton-polariton Bose-Einstein condensates created in solid states. We analyze and numerically model the dynamics and localization of the condensates using mean-field model. Chapter 1 contains an introduction to the physics of ultra-cold atom BEC and excitonpolariton BEC which provides a framework for the work presented in later chapters. In Chapter 2, we consider a method for achieving dynamically controllable transport of highly mobile matter-wave solitons in an ultra-cold atom BEC with attractive interparticle interaction loaded into a driven two-dimensional optical lattice. Our numerical analysis based on the mean-field model and the theory based on the effective particle approach demonstrate that fast, time-periodic rocking of the two-dimensional optical lattice enables efficient stabilization and manipulation of spatially localized matter wave packets via induced reconfigurable mobility channels. Chapter 3 consists of an investigation of the instability - collapse of a BEC with attractive interactions. In this chapter we explore the influence of an orbital angular momentum on the collapse of vortex-free elliptic clouds of Bose-Einstein condensates trapped in a radially symmetric harmonic potential or a rotating elliptic potential. The results of our analysis show that the number of trapped ultracold atoms corresponding to the collapse threshold can be radically increased for such rotating nonlinear matter waves in a radially harmonic trap. The results corresponding to a BEC cloud confined in a rotating elliptic trap show that the elongated stationary states can be parallel or perpendicular to the long axis of the trap and display bistable nature. In Chapter 4, we examine spatial localization and dynamical stability of Bose-Einstein condensates of exciton-polaritons in microcavities under the condition of off-resonant spatially inhomogeneous optical pumping both with and without a harmonic trapping potential. We employ the open-dissipative Gross-Pitaevskii model for describing an incoherently pumped polariton condensate coupled to an exciton reservoir. We reveal that spatial localization of the steady-state condensate occurs due to effective self-trapping created by the polariton flows, regardless of the presence of the external potential. A ground state of the polariton condensate with repulsive interactions between the quasiparticles represents a dynamically stable bright dissipative soliton. We also investigate the conditions for sustaining spatially localized structures, with nonzero angular momentum, in the form of single-charge vortices. Chapter 5 consider the existence of novel spatially localized states of exciton-polariton Bose-Einstein condensates in semiconductor microcavities with fabricated periodic inplane potentials. Our theory shows that, under the conditions of continuous nonresonant pumping, localization is observed for a wide range of optical pump parameters due to effective potentials self-induced by the polariton flows in the spatially periodic system. We show that the self-localization of exciton-polaritons in the lattice may occur both in the gaps and bands of the single-particle linear spectrum, and is dominated by the effects of gain and dissipation rather than the structured potential, in sharp contrast to the conservative condensates of ultra-cold alkali atoms.
In recent years, experiments by several groups have demonstrated spontaneous coherence in polariton systems, which can be viewed as a type of nonequilibrium Bose-Einstein condensation. In these systems, the polariton lifetime is longer than, but not much longer than, the polariton-polariton scattering time which leads to the thermalization. By contrast, over the past twenty years several groups have pursued experiments in a different system, which has very long exciton lifetime, up to 30 microseconds or more, essentially infinite compared to the thermalization time of the excitons. Thermal equilibrium of this type of exciton in a trap has been demonstrated experimentally. In this system, the interactions between the excitons are not short-range contact interactions, but instead are dipole-dipole interactions, with the force at long range going as 1/r31/r^{3}1/r3. Up to now there has not been a universally accepted demonstration of BEC in this type of system, and the way forward will require better understanding of the many-body effects of the excitons. I review what has been learned and accomplished in the past two decades in the search for an equilibrium BEC in this promising system.
We study the condensation of a two-dimensional exciton gas in a harmonic trap using a quantum Boltzmann equation. The excitons interact with a lattice that is kept at a constant temperature and we also include exciton–photon coupling (dissipation) and exciton–exciton interactions. We compare the condensation time for both an interacting and a non-interacting exciton gas. For a non-interacting gas anti-Stokes type processes dominate the relaxation rate of low-energy states. The condensation time-scale is determined by the (phonon) scattering rate into the ground state. The presence of dissipation results in a heating effect which increases the mean number of Bose particles required for the onset of condensation. For a dissipative gas the steady state is a nonequilibrium condensate (exciton matter laser), where the exciton temperature remains above the lattice temperature. We also discuss the effects of dimensionality and trapping on the relaxation process, which has a fundamental role in establishing the condensation time-scale.