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Physical Review A

Control of interferences in an Autler-Townes doublet: Symmetry of control parameters

M. Wollenhaupt, Andreas Assion, O. Bazhan, C. Horn, D. Liese, Cristian Sarpe, Martin Winter, Thomas Baumert

Published Jul 18, 2003• 96 citations
Publisher

Abstract

Coherent control beyond population control and spectral interferences is demonstrated on the interferences and intensity of the two Autler-Townes (AT) components in the photoelectron spectrum of K atoms, using a sequence of two intense time-delayed femtosecond laser pulses. Photoelectron spectra were taken at various delay times between the two laser pulses and at different laser intensities at a fixed delay time. With respect to the interferences in the AT doublet the role of time delay and laser intensity is interchangeable for $(n+0.5)\ensuremath{\pi}$ excitation. Strong laser fields or the optical phase of the delayed laser pulse allow the quantum mechanical phase of an atomic state to be manipulated in a symmetrical fashion. The observations are discussed in terms of a two-level model coupled to the continuum. For suitable combinations of the laser intensity of the first pulse and the time delay, the second laser pulse leaves the excited state population unchanged.

DOI
10.1103/physreva.68.015401

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Physical Review A•Feb 10, 2025•3 citations
Coherent control beyond population control and spectral interferences is demonstrated on the interferences and intensity of the two Autler-Townes (AT) components in the photoelectron spectrum of K atoms, using a sequence of two intense time-delayed femtosecond laser pulses. Photoelectron spectra were taken at various delay times between the two laser pulses and at different laser intensities at a fixed delay time. With respect to the interferences in the AT doublet the role of time delay and laser intensity is interchangeable for (n+0.5)\ensuremathπ(n+0.5)\ensuremath{\pi}(n+0.5)\ensuremathπ excitation. Strong laser fields or the optical phase of the delayed laser pulse allow the quantum mechanical phase of an atomic state to be manipulated in a symmetrical fashion. The observations are discussed in terms of a two-level model coupled to the continuum. For suitable combinations of the laser intensity of the first pulse and the time delay, the second laser pulse leaves the excited state population unchanged.
We propose a scheme to control the shape of the Autler-Townes (AT) doublet in the photoelectron spectrum from atomic resonance-enhanced multiphoton ionization (REMPI). The scheme is based on the interference of two AT doublets created by ionization of the strongly driven atom from the ground and the resonantly excited state using tailored bichromatic femtosecond laser pulses. In this scheme, the quantum phase of the photoelectrons is crucial for the manipulation of the AT doublet. The laser polarization state and the relative optical phase between the two colors are used to manipulate the interference pattern. We develop an analytical model to describe the bichromatic REMPI process and provide a physical picture of the control mechanism. To validate the model, the results are compared to an ab initio calculation based on the solution of the two-dimensional time-dependent Schr\"odinger equation for the nonperturbative interaction of an atom with intense polarization-shaped bichromatic femtosecond-laser pulses. Our results indicate that the control mechanism is robust with respect to the laser intensity, facilitating its experimental observation.
Population of the 4p state of K atom was studied theoretically by means of dressed states theory when a sequence of two laser pulses is used to excite K atom from the 4s to the 4p state.Relationships of the population of the dressed states and area of the first pulse and delay time between two pulses were obtained.Then the relationship between Autler-Townes doublet and the delay time was investigated by using the formula attained.It is shown that Autler-Townes doublet of the 4p state can be controlled by the delay time between the two pulses selecting the population of the dressed state,because of the delay time and the area of the first pulse which has a fixed value equal to 0.5π.
Abstract We investigated the Autler–Townes splitting in photoelectron spectra of molecules steered by ultrashort laser pulses using the time-dependent wave-packet method. Structure of the Autler–Townes splitting was presented to analyze the information of a selective population of the dressed states. It was found that population transfer process, structure of photoelectron spectrum and pattern of Autler–Townes splitting can be controlled by adjusting the intensity, wavelength and delay time of laser pulses.
We study the photoelectron spectra of hydrogen and helium ionized by intense ultrafast two-color XUV laser pulses by numerically solving the time-dependent Schrödinger equation.The photon energy of the pump pulse is tuned to the 1s-2p excitation energy, inducing Rabi oscillations between these bound states and forming an Autler-Townes (AT) doublet of dressed states.When ionized by a time-delayed ultrafast XUV pulse with duration shorter than the Rabi oscillation period, we find novel and drastically enhanced AT splittings in the photoionization spectrum.We identify their origin in terms of the temporal interference of two attosecond wave packets whose spectral distribution is controlled by the interplay between Rabi frequency and bandwidth of the probe pulse.These time-dependent features in the spectra can be much larger than the standard AT spacing induced by the pump pulse alone and can be controlled by the time delay and the duration of the probe pulse.
The existence of subpeak structures between the Autler-Townes (AT) doublet of the photoelectron spectrum during resonant ionization of an atom has been predicted in a large number of theoretical calculations, but a convincing physical explanation is still lacking. In this study we establish a temporal interference picture to elucidate the physical origin of these subpeaks. We derive an analytical estimation for the photoelectron spectra based on a three-level model, which agrees well with the numerical solution of the time-dependent Schr\"odinger equation at moderately strong pulse intensities. Our interpretation suggests that the interference of the photoelectron wave packet emitted during each Rabi cycle results in the subpeak structure between the AT doublet. By analyzing the phase difference between two temporally adjacent photoelectron wave packets, we successfully predict the interference minima in the photoelectron energy spectra.
We theoretically investigate the resonant two-photon ionization of a hydrogen atom in the counter-rotating circularly polarized double-pulse sequences, by solving the time-dependent Schr\"odinger equation. Due to the induced Rabi oscillations between the ground and excited states, the well-known Autler-Townes doublet is observed in the photoelectron spectra. More interestingly, our numerical results reveal an additional peak located between the Autler-Townes doublets, which originates from single-photon ionization from the excited state by the second pulse. By adjusting the laser intensity of the two pulses, the photoelectron yields of the three peaks can be sensitively modulated, under the control of completed Rabi cycles within the first pulse. In addition, our results show a potential of manipulating the photoemission anisotropy by both the laser intensity and the two-pulse time delay, through adjusting the competition of different partial waves generated by the two pulses.