In this paper we undertake a theoretical study of the quantum properties of a dipole nanolaser proposed by Protsenko et al. [Phys. Rev. A 71, 063812 (2005)]. The dynamics of the system is studied in both density-matrix and quantum Langevin formulations, with attention directed to noise sources. The result of the analysis indicates that in the most directly accessible parameter regime, photons will be emitted in a broad spectral distribution and the time delay between consecutive emissions of single photons exceeds the coherence time. Another parameter regime exists within which the emitted light more closely resembles conventional laser light.
In this paper we undertake a theoretical study of the quantum properties of a dipole nanolaser proposed by Protsenko et al. [Phys. Rev. A 71, 063812 (2005)]. The dynamics of the system is studied in both density-matrix and quantum Langevin formulations, with attention directed to noise sources. The result of the analysis indicates that in the most directly accessible parameter regime, photons will be emitted in a broad spectral distribution and the time delay between consecutive emissions of single photons exceeds the coherence time. Another parameter regime exists within which the emitted light more closely resembles conventional laser light.
Recent technological advances allow entire optical systems to be lithographically implanted on small silicon chips. These systems include tiny semiconductor lasers that function as light sources for digital optical signals. Future advances will rely on even smaller components. At the theoretical limit of this process, the smallest lasers will have an active medium consisting of a single atom (natural or artificial). Several suggestions for how this can be accomplished have already been published, such as nano-lasers based on photonic crystals and nano wires. In particular, the "dipole nanolaser" consists of a single quantum dot functioning as the active medium. It is optically coupled to a metal nanoparticles that form a resonant cavity. Laser light is generated from the near-field optical signal. The proposed work is a theoretical exploration of the nature of the resulting laser light.\nThe dynamics of the system will be studied and relevant time scales described. These will form the basis for a set of operator equations describing the quantum properties of the emitted light. The dynamics will be studied in both density matrix and quantum Langevin formulations, with attention directed to noise sources. The equations will be linearized and solved using standard techniques. The result of the study will be a set of predicted noise spectra describing the statistics of the emitted light. The goal will be to identify the major noise contributions and suggest methods for suppressing them. This will be done by studying the probability of getting squeezed light from the nanoparticle for the certain scheme of parameters.
The random nature of spontaneous emission leads to unavoidable fluctuations in a laser's output. This is often included through random Langevin forces in laser rate equations, but this approach falls short for nanolasers. In this paper, we show that the laser quantum noise can be quantitatively computed for a very broad class of lasers by starting from simple and intuitive rate equations and merely assuming that the number of photons and excited electrons only takes discrete values. While the approach has seen previous success, we here derive it rigorously from an open quantum system master equation, whereas it was previously introduced only on phenomenological grounds. We further show that in the many-photon limit, the model simplifies to Langevin equations. We perform an extensive comparison of different approaches for computing quantum noise in lasers, identifying the best approach for different system sizes, ranging from nanolasers to macroscopic lasers, and different levels of excitation, i.e., cavity photon number. In particular, we show that below the laser threshold, stochastic fluctuations in the numerical solution to the Langevin equations can drive populations to unphysical negative values, requiring the introduction of population bounds, which in turn skew the noise statistics, leading to inaccuracies. The Laser Markov Chain model, on the other hand, is accurate for all pump values and laser sizes when collective emitter effects are excluded.
Using two equivalent methods, the Heisenberg-Langevin and the master equation, we investigate the properties of a single-emitter nanolaser: an incoherently pumped single two-level system interacting with a single cavity mode of finite finesse. We are interested in a stationary generation regime when the mean number of photons inside the laser cavity is much larger than unity. In this case we linearize the Heisenberg-Langevin equations around the stationary classical solution and obtain analytical results for the linewidth, the quadrature fluctuation spectra, and the intracavity Mandel Q parameter. As the second method we use the master equation for the density operator of the laser field. Using the coherent-state representation of the density matrix we obtain the stationary solution for the Glauber P function of the laser mode and investigate the quantum statistics of the laser field and its threshold behavior. We compare the results of both methods with numerical simulations and find very good agreement. In the end we use our theoretical results for analyzing experiment with single-ion nanolasers.
Laser amplification kicks off with just a few photons in the cavity, a regime where standard additive Langevin noise cannot capture the real fluctuations. To understand how this amplification begins, we map out a single-mode photon-carrier model that links macroscopic lasers directly into nanolasers. Stationary rate equations reveal that stimulated emission takes over across a tight pump window. In nanolasers, however, spontaneous processes coexist across a much broader range. Because steady-state averages miss the individual events that lead to the macroscopic photon number, we frame the stochastic dynamics around the actual discrete transitions, deriving a state-dependent diffusion approximation. The destruction of an excited carrier concurrent with the generation of a photon creates a negative photon-carrier cross-correlation. This unavoidably leads to a correlated, multiplicative Gaussian-noise framework. We track the resulting discrete dynamics with an established, event-based Laser Markov Chain (LMC) which stochastically samples pump, relaxation, emission, and cavity-loss events keeping all physical quantities as non-negative integers. Comparing its predictions to those of our multiplicative model proves that the latter reproduces excellently well the statistical behavior of photons and carrier, as long as a continuous diffusion description holds. Once the emission drops into the few-photon regime, however, the discrete model becomes indispensable. On the other hand, at large photon counts relative fluctuations shrink to a level where the state-dependence of the diffusion matrix can be ignored, to leading order, thus returning to the classic Langevin description of the system's stochastic dynamics.
The laser has evolved from table size apparatuses to truly nano sized devices, in much the same way that computer chips have been continuously minimized. The few-emitter nanolaser represents an extreme in terms of size. The emitters can be either atoms or quantum dots, and they are coupled to a high-Q optical cavity. This system has previously been studied for the one and two emitters case, see e.g. [1, 2]. The emitters and cavity are modelled as two-level systems and a harmonic oscillator, respectively. The coupled system is modelled using the Jaynes-Cummings Hamiltonian and the two-level systems are pumped incoherently by a rate P. Solutions are found using the corresponding master equation. However, with cavity populations exceeding 100 and several emitters, the dimension of the Hilbert space of the system becomes too large to handle efficiently on a conventional computer. E.g. for four emitters and 100 photon states the density matrix has more than 2.5 × 106 elements. We have been able to simplify the problem significantly by adiabatically eliminating the photon-assisted polarizations and the correlations between emitters and cavity [3]. This results in a set of rate equations for the population of the cavity, na, and the occupation of the emitters. Fig. 1a) shows na for up to 4 emitters coupled to a cavity, as a function of the pumping rate P. The figure also shows results from a full master equation solution, and the correspondence is very good for large values of P. In Fig. 1b) the second order correlation functions g(2)(0) are shown, as obtained using the full model. The second order correlation functions become 1 for sufficiently large values of P signifying the onset of lasing. However, for larger values of P the laser quenches and the emission becomes chaotic (g(2)(0) = 2). This quenching effect is well-known in two-level models [3], but might not be realistic for semiconductor quantum dots. A proposed application for these nanolasers is in on-chip optical interconnects. In this application the modulation bandwidth is important. We have calculated the modulation bandwidth using a small-signal analysis of the rate equations, which has the advantage compared the full model of yielding a semianalytical result. The results are shown in Fig. 1c). The nanolaser has a high bandwidth, which is mostly limited by the cavity lifetime (/ 1/), but shows a prominent drop during the lasing regime. The modulation bandwidth again becomes limited by as the output becomes chaotic.