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Annalen der Physik

Cooperative Spontaneous Emission from an Initially Fully Excited System of Three Identical Two‐level Atoms

Th. Richter

Published Jan 1, 1983• 21 citations
Publisher

Abstract

Abstract Using Lehmberg's master equation and taking into account dipole‐dipole near‐field interaction the time‐dependent intensity pattern, intensity – and angular correlations of the cooperative spontaneous radiation from an initially fully excited system of three identical two‐level atoms are calculated. The intensity pattern developes lobes in different directions at different times in such a way that contrary to the two‐atom system the spatial distribution of the total number of the emitted photons differs from that of the single‐atom radiation pattern. In particular three atoms placed in proper distances on a straight line emit preferentially their energy along this line. At the beginning of the emission process the probability to find two photons simultaneously in the same (or geometrical equivalent) direction is always highest but in the course of time, contrary to the two‐atom case, it may well happen that the probability of finding two photons in quite different directions becomes more favoured.

DOI
10.1002/andp.19834950409

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Physical Review A•Sep 1, 1970•42 citations
Abstract Using Lehmberg's master equation and taking into account dipole‐dipole near‐field interaction the time‐dependent intensity pattern, intensity – and angular correlations of the cooperative spontaneous radiation from an initially fully excited system of three identical two‐level atoms are calculated. The intensity pattern developes lobes in different directions at different times in such a way that contrary to the two‐atom system the spatial distribution of the total number of the emitted photons differs from that of the single‐atom radiation pattern. In particular three atoms placed in proper distances on a straight line emit preferentially their energy along this line. At the beginning of the emission process the probability to find two photons simultaneously in the same (or geometrical equivalent) direction is always highest but in the course of time, contrary to the two‐atom case, it may well happen that the probability of finding two photons in quite different directions becomes more favoured.
Abstract The total radiation rate of the cooperative spontaneous emission from an initially single‐quantum excited three‐atom system is calculated using Lehmberg's master equation and taking into account dipole‐dipole near field interaction. We find a strong influence of the precise configuration of the atomic dipoles and of the position of the initially excited atom on the temporal behaviour of the total radiation rate, especially if the atoms are separated by distances much smaller than the resonance wavelength.
The cooperative spontaneous emission from three identical, initially excited two-level atoms separated by distances much smaller than the resonance wavelength is studied taking into account the dipole-dipole near-field interaction. Approximate expressions are obtained for the time evolution of the atomic system, the radiated intensity and the one-time intensity correlation function. As a new result the authors find that the near-field interaction may lead to the occurrence of beats in the intensity. Moreover, the destructive effect of the near-field interaction on the coherence properties of the emitted radiation is discussed.
Using the formalism developed earlier, we treat spontaneous emission from a pair of identical two-level atoms A1{A}_{1}A1​, A2{A}_{2}A2​, whose separation r21{r}_{21}r21​ can be comparable to the wavelength $\ensuremath{\lambda}$. We obtain expressions for time-dependent intensities and damping rates with the initial conditions (a) both atoms inverted, (b) prior excitation by a short $\frac{1}{2}\ensuremath{\pi}$ pulse, and (c) only A1{A}_{1}A1​ inverted. The results in (a) are compared with those obtained for a model consisting of two initially excited harmonic oscillators O1{O}_{1}O1​, O2{O}_{2}O2​. The atoms exhibit superradiant behavior, whereas O1{O}_{1}O1​, O2{O}_{2}O2​ tend to trap radiation. In (a), the intensity pattern $\mathcal{R}(\ensuremath{\theta},t)$ develops lobes in different directions at different times, so that the spatial distribution of photons at time $t\ensuremath{\rightarrow}\ensuremath{\infty}$ is the same as in the independent-atom case ${r}_{21}\ensuremath{\gg}\ensuremath{\lambda}$. For the oscillators, the lobes of $\mathcal{R}(\ensuremath{\theta},t)$ do not change direction, but only become more pronounced as time increases. In (b) and (c), the lobes oscillate back and forth at frequency $2{\ensuremath{\Omega}}_{12}$ corresponding to the shifts $\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$ of the triplet and singlet states due to the ${A}_{1}\ensuremath{-}{A}_{2}$ interaction. The intensity can therefore have a sinusoidal component. Field correlation functions calculated for (a) and (c) show that A2{A}_{2}A2​ and A2{A}_{2}A2​ radiate simultaneously around the frequencies $\ensuremath{\epsilon}\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$, where $\ensuremath{\epsilon}$ is the single-atom resonant frequency. The spectrum is calculated for case (c), and shows the effects of coherent linewidth enhancement in addition to the frequency shifts.
The intensity correlation function of the cooperative radiation from a continuously pumped three-atom system is calculated using Lehmberg's master equation supplemented by an incoherent-pumping term. Cooperative effects are found to change drastically the intensity fluctuations of the emitted radiation. Particularly, if the pumping rate is adjusted to three times the single-atom spontaneous decay rate, increased radiation, compared with that from three independently emitting atoms, should be observed, exhibiting a reduced intensity fluctuation.
The spontaneous emission of a set of NNN identical two-level atoms interacting with a quantized electromagnetic field is studied. The atoms are assumed to be close together compared to the mean wavelength of the emitted radiation, and their initial state is either a Dicke state or a superposition of the ground and excited state for each atom. Approximate expressions are obtained for transition probabilities, expectation values, and correlations as functions of time. The spontaneous emission for a very large separation of the atoms is also studied. In this case the directional properties of the emitted radiation, as well as the time within which the atoms decay to their ground state, depend on the position of each atom.