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Physical Review A

Generation of squeezed light by intracavity frequency doubling

Silvania F. Pereira, Min Xiao, Harry J. Kimble, J. L. Hall

Published Nov 1, 1988• 179 citations
Publisher

Abstract

Squeezed states of light are generated by the process of second-harmonic conversion within an optical cavity resonant at both fundamental and harmonic frequencies. Observations of squeezing are made by analyzing the spectral density of photocurrent fluctuations produced by the total field reflected from the nonlinear cavity. Reductions in photocurrent noise of 13% relative to the coherent-state or shot-noise level are achieved for frequency offsets near 4 MHz.

DOI
10.1103/physreva.38.4931

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Squeezed states of light are generated by the process of second-harmonic conversion within an optical cavity resonant at both fundamental and harmonic frequencies. Observations of squeezing are made by analyzing the spectral density of photocurrent fluctuations produced by the total field reflected from the nonlinear cavity. Reductions in photocurrent noise of 13% relative to the coherent-state or shot-noise level are achieved for frequency offsets near 4 MHz.
We have generated squeezed states of light by the process of second harmonic conversion within an optical cavity resonant at both fundamental and harmonic frequencies. The experiment consists of a standing-wave cavity containing a crystal of lithium niobate doped with magnesium oxide and driven by the field from a frequency-stabilized Nd:YAG laser (incident power, ~10 mW). The total field reflected from the cavity illuminates a pair of high quantum efficiency photodiodes, whose individual photocurrents are summed. Observations of squeezing are made by analyzing the spectral density of fluctuations for this sum photo-current while the cavity detuning is scanned through resonance. An intensity regulator holds the reflected light intensity constant during the scan by control of the incident light level. Reductions in photocurrent fluctuations of 12% relative to the vacuum-state or shot-noise level are achieved for frequency offsets near 4 MHz. Since significantly higher degrees of squeezing are predicted by our theoretical analysis, we discuss those processes that currently limit the observed noise reduction, including phase noise produced by the intracavity crystal in the absence of nonlinear conversion.
We present the analysis of a laser in which an intractivity χ (2) -nonlinear element couples the lasing mode to its second harmonic. The cavity is resonant for both modes. We investigate the potential for squeezing in this system by linearizing the quantum fluctuations around the steady states of the problem. In principle, more than 50% noise reduction below the vacuum level is possible in the second-harmonic field outside the cavity. The maximum squeezing, which is neither pure amplitude nor pure phase squeezing, occurs at a finite frequency-offset from the cavity resonance.
The input-output theory, originally developed for a linear coupling between cavity mode a and a bath, is extended to a coupling that is quadratic in the cavity mode operator a. We then apply this to second-harmonic generation, in a cavity that is resonant at the fundamental frequency and has an active laser medium working at the fundamental frequency. We find intensity squeezing of 50% below the shot-noise level in the output light at the second-harmonic frequency, whether or not the cavity is resonant at the second-harmonic frequency. To compare the singly resonant cavity to the doubly resonant cavity, we develop in an appendix a general technique for extracting a single mode from a continuum.
Experiments to generate squeezed states of light are described for a collection of two-level atoms within a high-finesse cavity. The investigation is conducted in a regime for which the weak-field coupling of atoms to the cavity mode produces a splitting in the normal mode structure of the atom–field system that is large compared with the atomic linewidth. Reductions in photocurrent noise of 30% (−1.55 dB) below the noise level set by the vacuum state of the field are observed in a balanced homodyne detector. A degree of squeezing of approximately 50% is inferred for the field state in the absence of propagation and detection losses. The observed spectrum of squeezing extends over a very broad range of frequencies (~±75 MHz), with the frequency of best squeezing corresponding to an offset from the optical carrier given by the normal mode splitting.
We analyze the quantum-fluctuation properties of second-harmonic radiation generated in the high-efficiency conversion process used in a recent experiment by Hakuta, Marmet, and Stoicheff [Phys. Rev. Lett. 66, 596 (1991)]. We extend their work by studying the second-harmonic generation inside an optical cavity. The active medium inside the cavity is modeled by three-level atoms with degenerated upper levels (1s, 2p, and 2s states of atomic hydrogen) interacting with a strong constant electric field. An enhancement of the conversion efficiency and a reduction of the added noise are found as a result of an electromagnetically induced transparency. We show that the scheme is capable of producing light in a squeezed or coherent state close to a minimum-uncertainty state with a large mean amplitude.