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Journal of Physics Conference Series

Boltzmann Description of Non-Interacting Electrons in Weakly Localized Regime

Yoko Yamane, Masaki Itoh

Published Dec 17, 2012• 0 citations
Publisher

Abstract

Transport process of non-interacting electrons is reformulated, in view of the exact treatment of interacting fermions reported by the present authors in this conference. It makes correspondence to the Boltzmann theory, covering the weakly localized regime, and also eliminates the hidden ultraviolet divergence by incorporating the particle-particle and hole-hole pairs. A mass renormalization of purely two-particle nature appears in the transport equation, giving rise to the conductivity of the Drude form. Taking the maximally crossed diagrams, the 2D conductivity is shown to vanish in the elastic scattering limit, while the distribition function preserves its sharp peak and the transport mass reduces to the free-electron value. The description differs from the self-consistent theory by Vollhardt and Wölfle, in which the Bethe-Salpeter structure of the scattering vertex is abandoned in favour of the time-reversal symmetry so the correspondence to the Boltzmann theory is lost.

DOI
10.1088/1742-6596/400/4/042073

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Transport process of non-interacting electrons is reformulated, in view of the exact treatment of interacting fermions reported by the present authors in this conference. It makes correspondence to the Boltzmann theory, covering the weakly localized regime, and also eliminates the hidden ultraviolet divergence by incorporating the particle-particle and hole-hole pairs. A mass renormalization of purely two-particle nature appears in the transport equation, giving rise to the conductivity of the Drude form. Taking the maximally crossed diagrams, the 2D conductivity is shown to vanish in the elastic scattering limit, while the distribition function preserves its sharp peak and the transport mass reduces to the free-electron value. The description differs from the self-consistent theory by Vollhardt and Wölfle, in which the Bethe-Salpeter structure of the scattering vertex is abandoned in favour of the time-reversal symmetry so the correspondence to the Boltzmann theory is lost.
We investigate a many-body localization transition based on Boltzmann transport theory. Introducing weak-localization corrections into a Boltzmann equation, Hershfield and Ambegaokar rederived the Wolfle-Vollhardt self-consistent equation for the diffusion coefficient [Phys. Rev. B 34, 2147 (1986)]. We generalize this Boltzmann equation framework, introducing electron-electron interactions into the Hershfield-Ambegaokar Boltzmann transport theory based on the study of Zala-Narozhny-Aleiner [Phys. Rev. B 64, 214204 (2001)]. Here, not only Altshuler-Aronov corrections but also dephasing effects are taken into account. As a result, we obtain a self-consistent equation for the diffusion coefficient in terms of the disorder strength and temperature, which extends the Wolfle-Vollhardt self-consistent equation in the presence of electron correlations. Solving our self-consistent equation numerically, we find a many-body localization insulator-metal transition, where a metallic phase appears from dephasing effects dominantly instead of renormalization effects at high temperatures. Although this mechanism is consistent with that of recent seminal papers [Ann. Phys. (NY) 321, 1126 (2006); Phys. Rev. Lett. 95, 206603 (2005)], we find that our three-dimensional metal-insulator transition belongs to the first-order transition, which differs from the Anderson metal-insulator transition described by the Wolfle-Vollhardt self-consistent theory. We speculate that a bimodal distribution function for the diffusion coefficient is responsible for this first-order phase transition.
Spinless fermions with repulsion are treated non-perturbatively by classifying the diagrams of the generating functional Φ in powers of the inverse lattice dimension 1/d. The equations derived from the first two orders are evaluated on the one- and on the two-particle level. The order parameter of the AB-charge density wave (AB-CDW) occurring at larger interaction is calculated in d = 3. The Bethe-Salpeter equation is evaluated for the conductivity σ(ω) which is found to have two peaks within the energy gap 2∆ in the AB-CDW: a remnant of the Drude peak and an excitonic resonance. Unexpectedly, σ DC does not vanish for T → 0 1 The limit of infinite dimensions d → ∞ for itinerant fermion systems [1, 2] has proven very useful for the understanding of strongly interacting electron systems [3]. The research focusses on one-particle properties in the strict limit d = ∞. There exist also some results on transport properties [4, 5]. The present contribution extends the knowledge on the AC- and DC-conductivity including 1/d-corrections in the model of spinless fermions with repulsive interaction. The results cover and the non-symmetry broken (homogeneous) phase and the AB-CDW occurring on bipartite lattices. The techniques used in the description of the latter are certainly transferable to other symmetry broken phases in related models. The Hamiltonian of the spinless fermion model at half-filling (n = 0.5) is given in second quantisation
The many-body linear response expressions obtained in previous papers [J. Math. Phys. 19, 1345 (1978); 20, 2573 (1979)] are applied to systems of weakly interacting particles. General expressions for the susceptibility and conductivity in such systems are obtained. The diagonal parts depend on the scattering processes, for which we consider interactions with bosons with mass and electron-phonon interaction. For elastic collisions simple closed forms result. For general two-body collisions, the closed expressions are cumbersome, except when the current is due to collisional current through localized states, such as Landau orbits; in that event a generalized Adams-Holstein result is obtained. The nondiagonal electrical conductivity is shown to be of paramount importance for the quantum mechanical Hall effect. We also derive quantum mechanical Boltzmann equations, both for the diagonal occupancy operator 〈nζ〉t and for the nondiagonal operator 〈c+ζ′ cζ\〉t. The total Boltzmann equation is shown to be fully equivalent with the linear response results. Finally, in the last part we derive the Boltzmann equation for the Wigner function of inhomogeneous systems. In the classical limit this yields the usual Boltzmann transport equation. This equation has therefore been obtained by first principles from the von Neumann equation.
We generalize the fermionic renormalization group method to describe analytically transport through a double barrier structure in a one-dimensional system. Focusing on the case of weakly interacting electrons, we investigate thoroughly the dependence of the conductance on the strength and the shape of the double barrier for arbitrary temperature T. Our approach allows us to systematically analyze the contributions to renormalized scattering amplitudes from different characteristic scales absent in the case of a single impurity, without restricting the consideration to the model of a single resonant level. Both a sequential resonant tunneling for high T and a resonant transmission for T smaller than the resonance width are studied within the unified treatment of transport through strong barriers. For weak barriers, we show that two different regimes are possible. Moderately weak impurities may get strong due to a renormalization by interacting electrons, so that transport is described in terms of theory for initially strong barriers. The renormalization of very weak impurities does not yield any peak in the transmission probability; however, remarkably, the interaction gives rise to a sharp peak in the conductance, provided asymmetry is not too high.
The ways of introducing and handling renormalizations in the many-body perturbation theory are reviewed. We stress the indispensable role the technique of Green functions plays in extrapolating the weak-coupling perturbative approaches to intermediate and strong couplings. We separately discuss mass and charge renor- malizations. The former is incorporated in a self-consistent equation for the self-energy derived explicitly from generating Feynman diagrams within the Baym and Kadanoff approach. The latter amounts to self-consistent equations for two-particle irreducible vertices. We analyze the charge renormalization initiated by De Domi- nicis and Martin and demonstrate that its realization via the parquet approach may become a powerful and viable way of using the many-body diagrammatic approach reliably in non-perturbative regimes with coopera- tive phenomena induced by either strong interaction or strong static randomness. Electric and magnetic properties of solids are determined by the behavior of valence electrons weakly bound to the atoms forming the crystalline lattice. The behavior of the gas of valence electrons in solids is most profound in metals with an open Fermi surface. Conduction electrons in metals can be described in a number of situations and for various purposes quite accurately by Bloch waves, eigenstates of the Fermi-gas Hamiltonian. We know, however, that electrons even in metals are not a noninteracting gas. They are generally exposed to forces driving them out of the equilibrium state of the Fermi gas. Firstly, no metal is a pure crystal and hence the electrons do not move freely in space. They are scattered on randomly distributed impurities and lattice defects. Secondly, the electrons are neither free and their mutual repulsion cannot be neglected particularly for transition and heavy metals. It is the most important and long standing task of condensed-matter theorists to comprehend and qualitatively capture the deviations in the behavior of electrons in real metals from their idealized representation via Bloch waves. The problem with quantification of the behavior of electrons beyond the almost free-electron picture is in paucity of available tools for accomplishing this task. Even if we can reduce the description of the electron gas in metals to rather simple and generic models, we are unable to solve them exactly, except for a few limiting cases that mostly do not correspond to situations of physical interest. With the increasing power of modern computers the role of numerical solutions and numerical brute force approaches has increased. Numerical solutions are usually unbiased and can reach a rather high level of quantitative precision. In some aspects they substitute the missing exact analytic solutions. Numerical solutions are suitable and even indispensable in showing and displaying the trends and some global features of the models studied. They, however, fail in critical regions of phase transitions in the vicinity of singularities in correlation functions. In these