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Frontiers in Optics

Atomic self-organization around tappered nanofibers

J. I. Cirac

Published Jan 1, 2012• 2 citations
Publisher

Abstract

Atoms can be trapped and laser cooled by a two-color evanescent field surrounding an optical nanofiber [1]. They can simultaneously be interrogated with light sent through the nanofiber [1,2]. This situation can be described in terms of a 1-dimensional electrodynamic theory, where dissipation may occur via the fiber itself, or in the rest of the modes of the electromagnetic field [3]. In such a theory, the light emitted by one atom may be absorbed by any other atom, thus giving rise to a long-range dipole-dipole interaction and the corresponding inter-atomic force. Thus, atoms may move in the self-created field. Additionally, light emitted by the atoms may dissipate energy, and thus drive the atoms into an equilibrium situation. This phenomenon is similar to the crystallization occurring in ion-trap experiments, or neutral atoms in optical lattices or cavities. The main difference, however, is that here there is no external structure which determines the equilibrium position, and that the forces between the atoms are dynamical in nature. In this contribution we will explain this phenomenon theoretically, and analyze the possibility of observing it with current experiments.

DOI
10.1364/ls.2012.lw1j.6

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Atoms can be trapped and laser cooled by a two-color evanescent field surrounding an optical nanofiber [1]. They can simultaneously be interrogated with light sent through the nanofiber [1,2]. This situation can be described in terms of a 1-dimensional electrodynamic theory, where dissipation may occur via the fiber itself, or in the rest of the modes of the electromagnetic field [3]. In such a theory, the light emitted by one atom may be absorbed by any other atom, thus giving rise to a long-range dipole-dipole interaction and the corresponding inter-atomic force. Thus, atoms may move in the self-created field. Additionally, light emitted by the atoms may dissipate energy, and thus drive the atoms into an equilibrium situation. This phenomenon is similar to the crystallization occurring in ion-trap experiments, or neutral atoms in optical lattices or cavities. The main difference, however, is that here there is no external structure which determines the equilibrium position, and that the forces between the atoms are dynamical in nature. In this contribution we will explain this phenomenon theoretically, and analyze the possibility of observing it with current experiments.
We present experimental techniques and recently demonstrated results related to the optimization and characterization of our recently demonstrated nanofiber-based atom trap. The atoms are confined in an optical lattice that is created using a two-color evanescent field surrounding the optical nanofiber. For this purpose, the polarization state of the trapping light fields has to be properly adjusted. We demonstrate that this can be accomplished by analyzing the light scattered by the nanofiber. Furthermore, we show that loading the nanofiber trap from a magneto-optical trap leads to sub-Doppler temperatures of the trapped atomic ensemble and yields a sub-Poissonian distribution of the number of trapped atoms per trapping site.
In this thesis I present a developing project to elaborate a scientific platform towards the realization of light-matter interaction based on tapered optical nanofiber (TNF) that enables optical fields to interface with trapped neutral atoms in their vicinity. In such a configuration, the guided light exhibits a large portion of evanescent field into the vacuum thus laser cooled atoms can couple to the fiber mode. By trapping and cooling atoms around the nanofiber I investigated the interaction of the atoms with the field. My work presented in this thesis includes: Calculating the evanescent modes propagating through our fiber; Implementing fiber pulling setup using oxyhydrogen flame and analyzing nanofiber’s thermal dynamics and degradation; Constructing a Rubidium 87 MOT and characterizing its critical parameters; Realizing some atom-light interface through an experiment on coupling spontaneously emitted photons from MOT into TNF; Calculating two-color dipole trap parameters for our nanofiber.
In this thesis, I present the realization of a fiber-optical interface using optically trapped cesium atoms, which is an efficient tool for coupling light and atoms. The basic principle of the presented scheme relies on the trapping of neutral cesium atoms in a two-color evanescent field surrounding a nanofiber. The strong confinement of the fiber guided light, which also protrudes outside the nanofiber, provides strong confinement of the atoms as well as efficient coupling to near-resonant light propagating through the fiber. In chapter 1, the necessary physical and mathematical background describing the propagation of light in an optical fiber is presented. The exact solution of Maxwell’s equations allows us to model fiber-guided light fields which give rise to the trapping potentials and the atom-light coupling in the close vicinity of a nanofiber. Chapter 2 gives the theoretical background of light-atom interaction. A quantum mechanical model of the light-induced shifts of the relevant atomic levels is reviewed, which allows us to quantify the perturbation of the atomic states due to the presence of the trapping light-fields. The experimental realization of the fiber-based atom trap is the focus of chapter 3. Here, I analyze the properties of the fiber-based trap in terms of the confinement of the atoms and the impact of several heating mechanisms. Furthermore, I demonstrate the transportation of the trapped atoms, as a first step towards a deterministic delivery of individual atoms. In chapter 4, I present the successful interfacing of the trapped atomic ensemble and fiber-guided light. Three different approaches are discussed, i.e., those involving the measurement of either near-resonant scattering in absorption or the emission into the guided mode of the nanofiber. In the analysis of the spectroscopic properties of the trapped ensemble we find good agreement with the prediction of theoretical model discussed in chapter 2. In addition, I introduce a non-destructive scheme for the interrogation of the atoms states, which is sensitive to phase shifts of far-detuned fiber-guided light interacting with the trapped atoms. The inherent birefringence in our system, induced by the atoms, changes the state of polarization of the probe light and can be thus detected via a Stokes vector measurement.
We have recently demonstrated a new experimental platform for trapping and optically interfacing laser-cooled cesium atoms. The scheme uses a two-color evanescent field surrounding an optical nanofiber to localize the atoms in a one-dimensional optical lattice 200 nm above the nanofiber surface [1]. In order to use this fiber-coupled ensemble of trapped atoms for applications in the context of quantum communication and quantum information processing, non-classical states of the atomic spins have to be prepared and should live long enough to allow one to apply successive quantum gates. The close proximity of the trapped atoms to the nanofiber surface and the strong polarization gradients of nanofiber-guided light fields are potentially important sources of decoherence. Here, we present our latest experimental results on the coherence properties of atomic spins in our nanofiber-based trap. Using a microwave field to drive the clock transition, we determine inhomogeneous and homogeneous dephasing times by Ramsey and spin echo techniques, respectively. Our results constitute the first measurement of the coherence properties of atoms trapped in the vicinity of a nanofiber and represent a fundamental step towards establishing nanofiber-based traps for cold atoms as a building block in a quantum network.
Trapping and optically interfacing laser-cooled neutral atoms are essential requirements for their use in advanced quantum technologies. Here we simultaneously realize both of these tasks with cesium atoms interacting with a multicolor evanescent field surrounding an optical nanofiber. The atoms are localized in a one-dimensional optical lattice about 200 nm above the nanofiber surface and can be efficiently interrogated with a resonant light field sent through the nanofiber. Our technique opens the route towards the direct integration of laser-cooled atomic ensembles within fiber networks, an important prerequisite for large scale quantum communication schemes. Moreover, it is ideally suited to the realization of hybrid quantum systems that combine atoms with, e.g., solid state quantum devices.
Tapered optical fibers with a nanofiber waist are versatile tools for interfacing light and matter. In this context, laser-cooled atoms trapped in the evanescent field surrounding the optical nanofiber are of particular interest: They exhibit both long ground-state coherence times and efficient coupling to fiber-guided fields. Here, we demonstrate electromagnetically induced transparency, slow light, and the storage of fiber-guided optical pulses in an ensemble of cold atoms trapped in a nanofiber-based optical lattice. We measure a slow-down of light pulses to group velocities of 50 m/s. Moreover, we store optical pulses at the single photon level and retrieve them on demand in the fiber after 2 microseconds with an overall efficiency of (3.0 +/- 0.4) %. Our results show that nanofiber-based interfaces for cold atoms have great potential for the realization of building blocks for future optical quantum information networks.