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Physical Review A

Interaction of Rydberg atoms with two contrapropagating ultrashort laser pulses

Andrey V. Lugovskoy, Igor Bray

Published Jun 2, 2006• 3 citations
Publisher

Abstract

In this paper we investigate how Rydberg atoms respond to perturbation by two contrapropagating ultrashort laser pulses. We consider the case where the durations of both pulses ${\ensuremath{\tau}}_{1}$ and ${\ensuremath{\tau}}_{2}$ are shorter than the inverse of the initial-state energy ${\ensuremath{\epsilon}}_{i}^{\ensuremath{-}1}$. When acting alone such a pulse passes through the atom without noticeable alteration in the atomic state. The situation is different if two such pulses interfere in the region of atom localization. In this case the atomic response is significantly enhanced. This is due to the nonzero momentum transferred to the electron by the interplay of the electric field of one pulse and the magnetic field of the other. The sudden perturbation approximation is used to evaluate the transition probabilities. They are shown to depend on the atom position with respect to the pulse interference region. This dependence is determined by the relationship between the atomic diameter ${d}_{i}$ and the interference-region size $l=c({\ensuremath{\tau}}_{1}+{\ensuremath{\tau}}_{2})$ ($c$ is the speed of light). If ${d}_{i}\ensuremath{\ll}l$ this dependence is sensitive to the function form of the pulses. For sufficiently strong fields the atoms can be ionized completely. In the opposite case of ${d}_{i}\ensuremath{\gg}l$ the transition probabilities are sensitive to the electron density distribution along the propagation direction. The probabilities of the initial-state destruction and atom ionization drop as $l∕{d}_{i}$ irrespective of the characteristics of the pulses.

DOI
10.1103/physreva.73.063401

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In this paper we investigate how Rydberg atoms respond to perturbation by two contrapropagating ultrashort laser pulses. We consider the case where the durations of both pulses \ensuremathτ1{\ensuremath{\tau}}_{1}\ensuremathτ1​ and \ensuremathτ2{\ensuremath{\tau}}_{2}\ensuremathτ2​ are shorter than the inverse of the initial-state energy \ensuremathϵi\ensuremath−1{\ensuremath{\epsilon}}_{i}^{\ensuremath{-}1}\ensuremathϵi\ensuremath−1​. When acting alone such a pulse passes through the atom without noticeable alteration in the atomic state. The situation is different if two such pulses interfere in the region of atom localization. In this case the atomic response is significantly enhanced. This is due to the nonzero momentum transferred to the electron by the interplay of the electric field of one pulse and the magnetic field of the other. The sudden perturbation approximation is used to evaluate the transition probabilities. They are shown to depend on the atom position with respect to the pulse interference region. This dependence is determined by the relationship between the atomic diameter di{d}_{i}di​ and the interference-region size l=c(\ensuremathτ1+\ensuremathτ2)l=c({\ensuremath{\tau}}_{1}+{\ensuremath{\tau}}_{2})l=c(\ensuremathτ1​+\ensuremathτ2​) (ccc is the speed of light). If di\ensuremath≪l{d}_{i}\ensuremath{\ll}ldi​\ensuremath≪l this dependence is sensitive to the function form of the pulses. For sufficiently strong fields the atoms can be ionized completely. In the opposite case of di\ensuremath≫l{d}_{i}\ensuremath{\gg}ldi​\ensuremath≫l the transition probabilities are sensitive to the electron density distribution along the propagation direction. The probabilities of the initial-state destruction and atom ionization drop as l∕dil∕{d}_{i}l∕di​ irrespective of the characteristics of the pulses.
Strong-field ionization of Rydberg atoms is investigated in its dependence on phase features of the initial coherent population of Rydberg levels. In the case of a resonance between Rydberg levels and some lower-energy atomic level (V-type transitions), this dependence is shown to be very strong: by a proper choice of the initial population an atom can be made either completely or very little ionized by a strong laser pulse. It is shown that phase features of the initial coherent population of Rydberg levels and the ionization yield can be efficiently controlled in a scheme of ionization by two strong laser pulses with a varying delay time between them.
Currently, the Magnus expansion method is widely used in studying Rydberg atoms in intense laser fields. In these studies, pulse lengths are usually set as an integer multiple of wavelength, at the same time, the initial phase of the laser pulse are usually set as zero, i.e. , without considering the effect of the initial phase in the calculation. However, this will result in some items multiplied by zero. Then, contributions from these items will be lost. Herein, we investigated the effects of the non-integer-cycle pulse and laser initial phase in the calculation of the transition probability of Rydberg atoms in intense laser fields. Our calculation result shows that these effects are trivial when the nondipole approximation is adopted. In dipole approximation i.e. , when the wavelength of the laser field exceeds the characteristic size of atomic or molecular orbitals, these effects are trivial only in the case of a long pulse duration and a large principal quantum number, however in the case of ultrashort laser pulses, these effects are obvious.
It is shown that the rate and degree of ionization of an atom can be controlled by preparing a specific superposition of Rydberg states. This effect is due to the Raman interaction of Rydberg levels via resonant lower-lying levels of the atom. Depending on the initial population of an atom interacting with a strong laser field, the atom either ionizes completely or exhibits an extremely high degree of stability (in this case the probability of the atom remaining in a bound state when the laser pulse is switched off is close to 1). It is shown that states which are stable against ionization decay or, conversely, decay rapidly into the continuum can be prepared using double laser pulses with a controllable time delay.
Interference stabilization of atoms is discussed. Raman-type transitions to Rydberg states with higher values of the electron orbital momentum l are taken into account in numerical calculations. These transitions are shown to change qualitatively theoretical predictions concerning the dependence of the time of ionization ti on the light field-strength amplitude (epsilon) 0: the time of ionization is shown to be a falling function of (epsilon) 0 in the weak-field region and, then, in a rather large interval of (epsilon) 0, to be approximately constant. The results derived are shown to be in a rather good agreement with the existing experiments.© (1996) COPYRIGHT SPIE--The International Society for Optical Engineering. Downloading of the abstract is permitted for personal use only.
We study the ionization of Rydberg atoms in a single-cycle-pulse electric field based on both classical and quantum calculations. The ionization-probability curve exhibits a ``ripple'' structure as a function of the pulse duration and the field amplitude. These ripple structures are found to be dependent on the angular distribution of the initial state. A large electron-emission asymmetry is observed, and the ionized electron is almost completely emitted to one side of the atom except when the pulse length is roughly one Rydberg period. In both the long-pulse and the short-pulse regimes, larger electron energy can be expected from the ionization of lower-lying Rydberg states, matching the observation in a recent experiment [S. Li and R. R. Jones, Phys. Rev. Lett. 112, 143006 (2014)]. This trend is closely related to the electron-emission asymmetry associated with the field-direction change in a single-cycle pulse. The possible implications of the different energy transfer in a single-cycle pulse from that in a multicycle pulse are also discussed briefly for the strong-field ionization of the ground atomic state.