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Quantum Electronics

Use of the ac Stark effect to alter the mechanism of formation of doubly charged ions in the ionisation of barium atoms by visible light

І. І. Бондар, В. В. Суран

Published Aug 31, 1999• 0 citations
Publisher

Abstract

The influence of an additional perturbation (the ac Stark effect) of neutral barium atoms on the formation of doubly charged ions in the course of ionisation of these atoms by visible light (by the second harmonic radiation of an yttrium-aluminium garnet laser) was investigated experimentally. The frequency-tunable radiation of a colour-centre laser (ω = 8500 — 8950 cm -1 ) was used in these investigations to effect the additional perturbation of barium atoms. It was found that this perturbation changed the mechanism of formation of the doubly charged Ba 2+ ions from a stepwise to a two-electron mechanism. The yield of the Ba 2+ ions increased sharply under these conditions.

DOI
10.1070/qe1999v029n08abeh001559

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Summary form only given. Beginning with first experiments, where the effect of doubly-charged ions formation was discovered, intensive investigations to determine the mechanism leading to the production of doubly-charged ions in different spectral ranges are carried out. The main goal of our work is the creation of conditions for realization of direct two-electron mechanism of Ba/sup 2+/ ions formation in the visible spectral range. The experimental setup consists in following: during ionization of Ba atoms by visible laser radiation we realized strong additional perturbation of atoms by laser radiation of another frequency range.