We study the angular correlations of photons emitted spontaneously by a set of sources placed at fixed positions with the use of a model of harmonic oscillators coupled to the electromagnetic field. In our previous study of angular correlations, in which the oscillators were treated as one dimensional and their Coulomb interactions were disregarded, we found only positive angular correlations over the whole range of interatomic separations for which the model was applicable. In this paper we use the model of three-dimensional oscillators interacting with the quantized electromagnetic field and also directly among themselves via the Coulomb forces. We solve this model analytically in the dipole approximation, and we calculate the angular correlation coefficient for different separations between the emitters. For separations less than half of the wavelength, we find negative angular correlations (spatial antibunching). This is a purely quantum effect that is not present in the corresponding classical stochastic model.
We study the angular correlations of photons emitted spontaneously by a set of sources placed at fixed positions with the use of a model of harmonic oscillators coupled to the electromagnetic field. In our previous study of angular correlations, in which the oscillators were treated as one dimensional and their Coulomb interactions were disregarded, we found only positive angular correlations over the whole range of interatomic separations for which the model was applicable. In this paper we use the model of three-dimensional oscillators interacting with the quantized electromagnetic field and also directly among themselves via the Coulomb forces. We solve this model analytically in the dipole approximation, and we calculate the angular correlation coefficient for different separations between the emitters. For separations less than half of the wavelength, we find negative angular correlations (spatial antibunching). This is a purely quantum effect that is not present in the corresponding classical stochastic model.
We study angular correlations of the radiation emitted by spatially extended sets of atoms. Such correlations result from the fact that the photons are identical quantum particles. We show that the symmetry (or the antisymmetry) alone of the wave function for identical, indistinguishable particles always leads to significant angular correlations and that in full agreement with our intuition, bosons tend to travel in the same direction while fermions tend to travel in opposite directions. In order to quantify these intuitive notions, we introduce---as a measure of angular correlations---the average value of the cosine of the angle between the directions of the momenta of two particles. The angular correlation coefficient is calculated for simple, model wave functions and the results are compared with those obtained from an exactly soluble model describing radiating harmonic oscillators. We find that even though the interaction modifies the exact values of the angular correlation coefficient, the gross features can be obtained from quantum statistics, i.e., from the symmetry of the many-photon wave functions. Moreover, the angular correlations as measured by the average cosine exhibit an almost universal character, at least for a small number of emitting atoms. Finally, we compare angular correlations obtained in quantum electrodynamics with the correlations resulting from the phenomenologically introduced randomness of the phases in the classical description of the electromagnetic field.
Sub- and superradiant dynamics of spontaneously decaying atoms are manifestations of collective many-body systems. We study the internal dynamics and the radiation properties of two atoms in free space. Interesting results are obtained when the atoms are separated by less than half a wavelength of the atomic transition, where the dipole-dipole interaction gives rise to new coherent effects, such as (a) coherence between two intermediate collective states, (b) oscillations in the two-photon correlation G(2), (c) emission of two photons by one atom, and (d) the loss of directional correlation. We compare the population dynamics during the two-photon emission process with the dynamics of single-photon emission in the cases of a $\ensuremath{\Lambda}$ and a V scheme. We compute the temporal correlation and angular correlation of two successively emitted photons using the G(2) for different values of atomic separation. We find antibunching when the atomic separation is a quarter wavelength $\ensuremath{\lambda}∕4$. Oscillations in the temporal correlation provide a useful feature for measuring subwavelength atomic separation. Strong directional correlation between two emitted photons is found for atomic separation larger than a wavelength. We also compare the directionality of a photon spontaneously emitted by the two atoms prepared in phased-symmetric and phased-antisymmetric entangled states ${\ensuremath{\mid}\ifmmode\pm\else\textpm\fi{}⟩}_{{\mathbf{k}}_{0}}={e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{1}}\ensuremath{\mid}{a}_{1},{b}_{2}⟩\ifmmode\pm\else\textpm\fi{}{e}^{i{\mathbf{k}}_{0}∙{\mathbf{r}}_{2}}\ensuremath{\mid}{b}_{1},{a}_{2}⟩$ by a laser pulse with wave vector k0. Photon emission is directionally suppressed along k0 for the phased-antisymmetric state. The directionality ceases for interatomic distances less than $\ensuremath{\lambda}∕2$.
Spontaneous emission is one of the most fundamental out-of-equilibrium processes in which an excited quantum emitter relaxes to the ground state due to quantum fluctuations. In this process, a photon is emitted that can interact with other nearby emitters and establish quantum correlations between them, e.g., via super and subradiance effects. One way to modify these photon-mediated interactions is to alter the dipole radiation patterns of the emitter, e.g., by placing photonic crystals near them. One recent example is the generation of strong directional emission patterns - key to enhancing super and subradiance effects - in two dimensions by employing photonic crystals with band structures characterized by linear isofrequency contours and saddle points. However, these studies have predominantly used oversimplified toy models, overlooking the electromagnetic field's intricacies in actual materials, including aspects like geometrical dependencies, emitter positions, and polarization. Our study delves into the interaction between these directional emission patterns and the variables mentioned above, revealing the untapped potential to fine-tune collective quantum optical phenomena.
Spontaneous emission is one of the most fundamental out-of-equilibrium processes in which an excited quantum emitter relaxes to the ground state due to quantum fluctuations. In this process, a photon is emitted that can interact with other nearby emitters and establish quantum correlations between them, e.g., via super and subradiance effects. One way to modify these photon-mediated interactions is to alter the dipole radiation patterns of the emitter, e.g., by placing photonic crystals near them. One recent example is the generation of strong directional emission patterns-key to enhancing super and subradiance effects-in two dimensions by employing photonic crystals with band structures characterized by linear isofrequency contours and saddle-points. However, these studies have predominantly used oversimplified toy models, overlooking the electromagnetic field's intricacies in actual materials, including aspects like geometrical dependencies, emitter positions, and polarization. Our study delves into the interaction between these directional emission patterns and the aforementioned variables, revealing the untapped potential to fine-tune collective quantum optical phenomena.
The spontaneous emission of a set of N identical two-level atoms interacting with a quantized electromagnetic field is studied. The atoms are assumed to be close together compared to the mean wavelength of the emitted radiation, and their initial state is either a Dicke state or a superposition of the ground and excited state for each atom. Approximate expressions are obtained for transition probabilities, expectation values, and correlations as functions of time. The spontaneous emission for a very large separation of the atoms is also studied. In this case the directional properties of the emitted radiation, as well as the time within which the atoms decay to their ground state, depend on the position of each atom.
Using the formalism developed earlier, we treat spontaneous emission from a pair of identical two-level atoms A1, A2, whose separation r21 can be comparable to the wavelength $\ensuremath{\lambda}$. We obtain expressions for time-dependent intensities and damping rates with the initial conditions (a) both atoms inverted, (b) prior excitation by a short $\frac{1}{2}\ensuremath{\pi}$ pulse, and (c) only A1 inverted. The results in (a) are compared with those obtained for a model consisting of two initially excited harmonic oscillators O1, O2. The atoms exhibit superradiant behavior, whereas O1, O2 tend to trap radiation. In (a), the intensity pattern $\mathcal{R}(\ensuremath{\theta},t)$ develops lobes in different directions at different times, so that the spatial distribution of photons at time $t\ensuremath{\rightarrow}\ensuremath{\infty}$ is the same as in the independent-atom case ${r}_{21}\ensuremath{\gg}\ensuremath{\lambda}$. For the oscillators, the lobes of $\mathcal{R}(\ensuremath{\theta},t)$ do not change direction, but only become more pronounced as time increases. In (b) and (c), the lobes oscillate back and forth at frequency $2{\ensuremath{\Omega}}_{12}$ corresponding to the shifts $\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$ of the triplet and singlet states due to the ${A}_{1}\ensuremath{-}{A}_{2}$ interaction. The intensity can therefore have a sinusoidal component. Field correlation functions calculated for (a) and (c) show that A2 and A2 radiate simultaneously around the frequencies $\ensuremath{\epsilon}\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$, where $\ensuremath{\epsilon}$ is the single-atom resonant frequency. The spectrum is calculated for case (c), and shows the effects of coherent linewidth enhancement in addition to the frequency shifts.