Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physica Scripta

Optical pumping effects in high resolution laser spectroscopy

Shigeru Nakayama

Published Jan 1, 1997• 29 citations
Publisher

Abstract

A theoretical analysis of the relative intensities of the Doppler-free signals in saturation spectroscopy, velocity selective optical pumping (VSOP) spectroscopy, polarization spectroscopy and a mixing of saturation and polarization spectroscopies is presented using the approximation of a single cycle of optical pumping in a four-level system. An optical pumping process in the Zeeman sublevels is taken into account owing to the important role of spontaneous emission even if the sublevels are degenerate. Arbitrary polarization combinations are considered for pump and probe beams. The similarities and differences between three kinds of spectroscopy are made clear. Both circular and linear optical anisotropies induced by the pump beam are considered in this theoretical calculation. The magnitude and sign of Doppler-free resonances in each spectroscopy are quite different owing to the polarizations of the pump and probe beams. The four-level system is important as a three-level approximation. The results obtained from the four-level optical pumping theory are in good agreement with experimental reports.

DOI
10.1088/0031-8949/1997/t70/010

Related papers

Doppler-free laser spectroscopic techniques with optical pumping in D_1 lines of alkali atoms

Shigeru Nakayama

A theoretical analysis of the D1 lines of alklai atoms in Doppler-free polarization spectroscopy, velocity-selective optical-pumping (VSOP) spectroscopy, and saturation spectroscopy is presented that uses the approximation of a single cycle of optical pumping in a four-level system. The similarities and differences among these three kinds of spectroscopy are made clear, and the magnitude and the sign of the resonances in each spectroscopic technique are calculated. The four-level system is as important as a three-level approximation, which has already been described in many papers. We deal with linear and circular optical anisotropies induced in polarization, VSOP, and saturation spectroscopy.

Journal of the Optical Society of America B•Sep 1, 1985•26 citations

Theoretical Analysis of Rb and Cs D2 Lines in Doppler-Free Spectroscopic Techniques with Optical Pumping

Shigeru Nakayama

The relative intensities of the Doppler-free signals of the 85Rb and Cs D2 lines in saturation spectroscopy, velocity-selective optical pumping (VSOP) spectroscopy, and polarization spectroscopy were calculated theoretically, taking into accont the optical pumping process in the Zeeman sublevels and arbitrary polarization combinations for pump and probe beams. Both circular and linear optical anisotropy induced by the pump beam were considered in the theoretical calculation. The magnitude and sign of the Doppler-free resonances in each spectroscopic method were quite different owing to the polarizations of the pump and probe beams. The theoretical results obtained from a single-cycle optical pumping in a four-level approximation were in good agreement with recent experimental reports.

Japanese Journal of Applied Physics•Jan 1, 1985•57 citations

Saturation Effects in Polarization Spectroscopy and Polarization effects in Saturation Spectroscopy

Shigeru NAKAYAMA

The relative intensities of the Doppler-free signals in the transition from polarized and dispersive signals to absorptive signals of the Na D1 line are calculated theoretically from the approximation of a single cycle of opticalpumping in a four-level system. The transition from polarized signals to saturated signals is made by varying the angle of an analyzer. Since the signal in polarization spectroscopy is mixed with the signal in saturation spectroscopy during the transition, spurious signals due to saturation and polarization effects should be taken into account in the signal analysis of polarization and saturation spectroscopies, respectively. Both theories, of polarization spectroscopy and saturation spectroscopy are unified and applied to the Doppler-free signals of the Na D1 line. The results obtained from the four-level optical pumping theory which mixes polarization spectroscopy with saturation spectroscopy are in good agreement with experimental reports.

The Review of Laser Engineering•Jan 1, 1986•3 citations

Velocity Selective Optical Pumping Spectroscopy of D1 Lines in Alkali Atoms

Shigeru Nakayama

Theoretical analysis of D 1 lines of most stable alkali atoms in velocity selective optical pumping (VSOP) spectroscopy is presented by using the approximation of a single cycle of optical pumping in a four-level system. VSOP spectroscopy is clearly compared with polarization spectroscopy and then it is shown that the results obtained for polarization spectroscopy can be applied to the theory in VSOP spectroscopy. The relative signal intensities of Na D 1 line in polarization spectroscopy have been theoretically calculated and experimentally confirmed to be in good agreement with those in VSOP spectroscopy. The first-order theory in VSOP spectroscopy can be applied to the cases of the D 1 lines of the other alkali atoms. It is expected that the theoretical analysis can be useful for future experiments of the Doppler-free D lines in the alkali atoms.

Journal of the Physical Society of Japan•Oct 1, 1984•7 citations

Doppler-Free Laser Spectroscopy Using Polarization Modulation in Na D1 and D2 Lines

김점술, 김중복, 공홍진 +1 more

Doppler-free laser spectroscopy using polarization modulation has been carried out in Na D₁ and D₂ lines. The polarization of the pump beam is modulated between identically and orthogonally to a linear or circular polarization of the probe beam. The recorded signals of the hyperfine and crossover resonances are in agreement with a recent theoretical analysis of Nakayama which is based on velocity-selective optical pumping in a four-level system. Some exceptional discrepancy occuring in the D₂ is considered to be due to several relatively close lying resonances.

한국광학회 학술대회논문집•Jan 1, 1988•0 citations

Theoretical Analysis of Rb and Cs D2 Lines in Saturation Spectroscopy with Optical Pumping

Shigeru Nakayama

The relative intensities of the Doppler-free signals of 85Rb and Cs D2 lines in saturation spectroscopy were calculated theoretically, taking into account the optical pumping process in a four-level system. The optical pumping effect in saturation spectroscopy is important when atoms with long-lived lower states are pumped by a weak beam. The theoretical results calculated from a simple analysis without any knowledge of the saturation parameters were found to be in good agreement with the experimental results on Rb and Cs D2 lines previously obtained using semiconductor laser.

Japanese Journal of Applied Physics•Jul 1, 1984•27 citations
A theoretical analysis of the relative intensities of the Doppler-free signals in saturation spectroscopy, velocity selective optical pumping (VSOP) spectroscopy, polarization spectroscopy and a mixing of saturation and polarization spectroscopies is presented using the approximation of a single cycle of optical pumping in a four-level system. An optical pumping process in the Zeeman sublevels is taken into account owing to the important role of spontaneous emission even if the sublevels are degenerate. Arbitrary polarization combinations are considered for pump and probe beams. The similarities and differences between three kinds of spectroscopy are made clear. Both circular and linear optical anisotropies induced by the pump beam are considered in this theoretical calculation. The magnitude and sign of Doppler-free resonances in each spectroscopy are quite different owing to the polarizations of the pump and probe beams. The four-level system is important as a three-level approximation. The results obtained from the four-level optical pumping theory are in good agreement with experimental reports.
A theoretical analysis of the D1 lines of alklai atoms in Doppler-free polarization spectroscopy, velocity-selective optical-pumping (VSOP) spectroscopy, and saturation spectroscopy is presented that uses the approximation of a single cycle of optical pumping in a four-level system. The similarities and differences among these three kinds of spectroscopy are made clear, and the magnitude and the sign of the resonances in each spectroscopic technique are calculated. The four-level system is as important as a three-level approximation, which has already been described in many papers. We deal with linear and circular optical anisotropies induced in polarization, VSOP, and saturation spectroscopy.
The relative intensities of the Doppler-free signals of the 85Rb and Cs D2 lines in saturation spectroscopy, velocity-selective optical pumping (VSOP) spectroscopy, and polarization spectroscopy were calculated theoretically, taking into accont the optical pumping process in the Zeeman sublevels and arbitrary polarization combinations for pump and probe beams. Both circular and linear optical anisotropy induced by the pump beam were considered in the theoretical calculation. The magnitude and sign of the Doppler-free resonances in each spectroscopic method were quite different owing to the polarizations of the pump and probe beams. The theoretical results obtained from a single-cycle optical pumping in a four-level approximation were in good agreement with recent experimental reports.
The relative intensities of the Doppler-free signals in the transition from polarized and dispersive signals to absorptive signals of the Na D1 line are calculated theoretically from the approximation of a single cycle of opticalpumping in a four-level system. The transition from polarized signals to saturated signals is made by varying the angle of an analyzer. Since the signal in polarization spectroscopy is mixed with the signal in saturation spectroscopy during the transition, spurious signals due to saturation and polarization effects should be taken into account in the signal analysis of polarization and saturation spectroscopies, respectively. Both theories, of polarization spectroscopy and saturation spectroscopy are unified and applied to the Doppler-free signals of the Na D1 line. The results obtained from the four-level optical pumping theory which mixes polarization spectroscopy with saturation spectroscopy are in good agreement with experimental reports.
Theoretical analysis of D 1 lines of most stable alkali atoms in velocity selective optical pumping (VSOP) spectroscopy is presented by using the approximation of a single cycle of optical pumping in a four-level system. VSOP spectroscopy is clearly compared with polarization spectroscopy and then it is shown that the results obtained for polarization spectroscopy can be applied to the theory in VSOP spectroscopy. The relative signal intensities of Na D 1 line in polarization spectroscopy have been theoretically calculated and experimentally confirmed to be in good agreement with those in VSOP spectroscopy. The first-order theory in VSOP spectroscopy can be applied to the cases of the D 1 lines of the other alkali atoms. It is expected that the theoretical analysis can be useful for future experiments of the Doppler-free D lines in the alkali atoms.
Doppler-free laser spectroscopy using polarization modulation has been carried out in Na D₁ and D₂ lines. The polarization of the pump beam is modulated between identically and orthogonally to a linear or circular polarization of the probe beam. The recorded signals of the hyperfine and crossover resonances are in agreement with a recent theoretical analysis of Nakayama which is based on velocity-selective optical pumping in a four-level system. Some exceptional discrepancy occuring in the D₂ is considered to be due to several relatively close lying resonances.
The relative intensities of the Doppler-free signals of 85Rb and Cs D2 lines in saturation spectroscopy were calculated theoretically, taking into account the optical pumping process in a four-level system. The optical pumping effect in saturation spectroscopy is important when atoms with long-lived lower states are pumped by a weak beam. The theoretical results calculated from a simple analysis without any knowledge of the saturation parameters were found to be in good agreement with the experimental results on Rb and Cs D2 lines previously obtained using semiconductor laser.