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Physical Review B

Entanglement of static and flying qubits in degenerate mesoscopic systems

Matthew Habgood, J. H. Jefferson, A. Ramšak, David Godfrey Pettifor, G. A. D. Briggs

Published Feb 28, 2008• 11 citations

Abstract

The entanglement of flying qubits with static qubits in the solid state is important in the development of quantum computing. It has recently been shown theoretically that the spin-dependent scattering of a propagating electron from a bound electron is sufficient to give full entanglement between the qubits embodied in their respective spins [J. H. Jefferson et al., Europhys. Lett. 74, 764 (2006); D. Gunlycke et al., J. Phys.: Condens. Matter 18, S851 (2006)]. In this paper a generalized, real-space Anderson model is introduced for a quasi-one-dimensional structure consisting of a binding site coupled to ideal leads. Degeneracy of both the binding site and the leads is incorporated to represent, for example, conduction band degeneracy in carbon nanotubes. The model is used to calculate the spin-dependent scattering behavior and resultant static-flying qubit entanglement created by the scattering process. Degeneracy (and more generally, multiplicity) in the binding site gives rise to inelastic scattering processes. In the elastic scattering regime, a degenerate binding site gives rise to antiresonant structures in the transmission spectrum. Additional degeneracy in the leads restricts this effect to the second set of leads, raising the possibility of spin filtration, though this is eliminated in the inelastic scattering regime. Degeneracy in the binding site also gives rise to multiple resonances in transmission that will improve the probability of obtaining entangled pairs relative to the nondegenerate case. This effect is maximized when the components of the degenerate binding site are symmetrically coupled to the leads.

DOI: 10.1103/physrevb.77.075337

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The entanglement of flying qubits with static qubits in the solid state is important in the development of quantum computing. It has recently been shown theoretically that the spin-dependent scattering of a propagating electron from a bound electron is sufficient to give full entanglement between the qubits embodied in their respective spins [J. H. Jefferson et al., Europhys. Lett. 74, 764 (2006); D. Gunlycke et al., J. Phys.: Condens. Matter 18, S851 (2006)]. In this paper a generalized, real-space Anderson model is introduced for a quasi-one-dimensional structure consisting of a binding site coupled to ideal leads. Degeneracy of both the binding site and the leads is incorporated to represent, for example, conduction band degeneracy in carbon nanotubes. The model is used to calculate the spin-dependent scattering behavior and resultant static-flying qubit entanglement created by the scattering process. Degeneracy (and more generally, multiplicity) in the binding site gives rise to inelastic scattering processes. In the elastic scattering regime, a degenerate binding site gives rise to antiresonant structures in the transmission spectrum. Additional degeneracy in the leads restricts this effect to the second set of leads, raising the possibility of spin filtration, though this is eliminated in the inelastic scattering regime. Degeneracy in the binding site also gives rise to multiple resonances in transmission that will improve the probability of obtaining entangled pairs relative to the nondegenerate case. This effect is maximized when the components of the degenerate binding site are symmetrically coupled to the leads.

The possibility of generating entanglement between two solid-state electron spin-qubits by spin-dependent scattering of a third, propagating electron is attractive. A process of this kind could work well beyond the range of the direct interaction between the two spins. In this study, the binding of electrons in one-dimensional structures is theoretically modeled using a real-space analog of the Anderson model. The respective binding sites are arranged in two different geometries. The first is a straightforward series arrangement, and the second a parallel arrangement in which the binding sites are embedded in either arm of an Aharonov-Bohm style ring. For the series arrangement, the entanglement between the bound electrons is calculated and is shown to be low (concurrence

<0.2

) in all regions of significant transmission. In contrast, the parallel arrangement allows full entanglement to be generated from a ${S}_{z}=1(\ensuremath{\mid}\ensuremath{\uparrow}\ensuremath{\uparrow}⟩)$ or ${S}_{z}=0(\ensuremath{\mid}\ensuremath{\uparrow}\ensuremath{\downarrow}⟩)$ starting configuration with an overall probability of success up to 0.5.

A theoretical scheme is presented for the entanglement of two-electron spin qubits bound in series within a quasi-one-dimensional mesoscopic structure at a distance beyond their normal range of interaction. A third electron is scattered from them, and full entanglement is achieved upon measurement of a transmitted electron in the correct spin state. Critically, each bound electron is trapped within an individual structure that has at least two spatial states. Two simple examples of such structures are discussed here. One is a 'stub', in which a quantum dot (for example) is coupled to one side of the quasi-one-dimensional structure. The other is a pair of degenerate, coupled quantum dots, with strong interdot Coulomb repulsion, placed within the one-dimensional superstructure. Both of these are shown to allow generation of entanglement with a significant probability of success. In contrast to the results of the authors' previous works, this allows for the generation of entanglement in a series, rather than in a parallel, configuration of the bound electrons with respect to the propagating electron.

A shallow potential well in a near-perfect quantum wire will bind a single-electron and behave like a quantum dot, giving rise to spin-dependent resonances of propagating electrons due to Coulomb repulsion and Pauli blocking. It is shown how this may be used to generate full entanglement between static and flying spin-qubits near resonance in a two-electron system via singlet or triplet spin-filtering. In a quantum wire with many electrons, the same pairwise scattering may be used to explain conductance, thermopower and shot-noise anomalies, provided the temperature/energy scale is sufficiently high for Kondo-like many-body effects to be negligible.

We investigate whether a two-qubit quantum gate can be implemented in a scattering process involving a flying and a static qubit. To this end, we focus on a paradigmatic setup made out of a mobile particle and a quantum impurity, whose respective spin degrees of freedom couple to each other during a one-dimensional scattering process. Once a condition for the occurrence of quantum gates is derived in terms of spin-dependent transmission coefficients, we show that this can be actually fulfilled through the insertion of an additional narrow potential barrier. An interesting observation is that under resonance conditions this procedure enables a gate only for isotropic Heisenberg (exchange) interactions and fails for an

\mathit{XY}

interaction. We show the existence of parameter regimes for which gates able to establish a maximum amount of entanglement can be implemented. The gates are found to be robust to variations of the optimal parameters.

While molecular spin qubits (MSQs) are a promising platform for quantum computing, read-out has been largely limited to electron paramagnetic resonance which is often slow and requires a global system drive. Moreover, because one prerequisite for the Elzerman and Pauli spin blockade readout mechanisms typical of semiconductor spin qubits is tunneling of electrons between sites, these read-out modalities are unavailable in MSQs. Here, we theoretically demonstrate electrical read-out of entangled MSQs via driven many-electron spin unpolarized currents. In particular, using a time-dependent density matrix renormalization group approach we simulate a maximally entangled MSQ pair between two electronic leads. Driving itinerant electrons between the two leads, we find that the conductance is greater when the MSQs are in the entangled singlet state as compared to the entangled triplet state. This contrast in conductance is enhanced when the electronic density of states at the Fermi energy is large and for narrow bandwidth. Our results are readily applicable to molecules supramolecularly functionalizing semiconductors with relatively flat bands such as single-wall carbon nanotubes under a magnetic field.