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High-Precision Calculations for Four-Body Atomic Systems

Zong-Chao Yan

Published Aug 1, 2002• 0 citations
Publisher
DOI
10.1142/9789812776785_0076

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Quantum sensing using Rydberg atoms is an emerging technology for precise measurement of electric fields. However, most existing computational methods are all based on a single-particle model and neglect Rydberg-Rydberg interaction between atoms. In this study, we introduce the interaction term into the conventional four-level optical Bloch equations. By incorporating fast iterations and solving for the steady-state solution efficiently, we avoid the computation of a massive 4 N × 4 N dimensional matrix. Additionally, we apply the Doppler frequency shift to each atom used in the calculation, eliminating the requirement for an additional Doppler iteration. These schemes allow for the calculation of the interaction between 7000 atoms around one minute. Based on the many-body model, we investigate the Rydberg-Rydberg interaction of Rydberg atoms under different atomic densities. Furthermore, we compare our results with the literature data of a three-level system and the experimental results of our own four-level system. The results demonstrate the validity of our model, with an effective error of 4.59% compared to the experimental data. Finally, we discover that the many-body model better predicts the linear range for measuring electric fields than the single-particle model, making it highly applicable in precise electric field measurements.
We calculated, using seven realistic $^{4}\mathrm{He}\text{\ensuremath{-}}^{4}\mathrm{He}$ potentials in the literature, the Efimov spectra of the 4He^{4}\mathrm{He}4He trimer and tetramer and analyzed the universality of the systems. The three-(four-)body Schr\"odinger equations were solved fully nonadiabatically with the high-precision calculation method employed in our previous work on the 4He^{4}\mathrm{He}4He trimer and tetramer [Phys. Rev. A 85, 022502 (2012); Phys. Rev. A 85, 062505 (2012)]. We found the following universality in the four-boson system: (i) The critical scattering lengths at which the tetramer ground and excited states couple to the four-body threshold are independent of the choice of the two-body realistic potentials in spite of the difference in the short-range details and do not contradict the corresponding values observed in the experiments in ultracold alkali-metal atoms when scaled with the van der Waals length rvdW{r}_{\mathrm{vdW}}rvdW​, and (ii) the four-body hyperradial potential has a repulsive barrier at the four-body hyperradius ${R}_{4}\ensuremath{\approx}3\phantom{\rule{0.16em}{0ex}}{r}_{\mathrm{vdW}}$, which prevents the four particles from getting close together to explore nonuniversal features of the interactions at short distances. This result is an extension of the universality in Efimov trimers that the appearance of the repulsive barrier at the three-body hyperradius ${R}_{3}\ensuremath{\approx}2\phantom{\rule{0.16em}{0ex}}{r}_{\mathrm{vdW}}$ makes the critical scattering lengths independent of the short-range details of the interactions as reported in the literature and also in the present work for the 4He^{4}\mathrm{He}4He trimer with the realistic potentials.
The spectral features of the velocity of light-induced drift (LID) of lithium atoms in a neon buffer gas have been theoretically studied using four known ab initio calculated interatomic interaction potentials for the Li–Ne system of colliding particles. The calculations with each of these four potentials predict a strong temperature dependence of the spectral shape of the LID signal of Li atoms in the Ne atmosphere in various temperature intervals. The results allow the high-precision test of the interatomic interaction potentials in experiments on anomalous LID.