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Journal of Quantitative Spectroscopy and Radiative Transfer

Laser absorption under saturation conditions with allowance for spectral hole burning

R. M. Measures, Harald Herchen

Published Jan 1, 1983• 7 citations
Publisher
DOI
10.1016/0022-4073(83)90140-1

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Spectral hole burning and pulse filtering in optically dense samples

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\n\nSpectral hole-burning in an erbium-doped silica fibre at room temperature has been experimentally demonstrated. This demonstration can be considered as a clear experimental evidence of the relationship between slow light and coherent population oscillations in erbium-doped fibres. In a 3.5 m erbium-doped silica fibre, spectral holes with a depth up to 1.5textm−11.5\\ \\text{m}^{-1}1.5textm−1 were obtained by coupling a strong and narrow saturating power and measuring changes in the spectral absorption coefficient for a weak and wide probe power. A tuneable ring-cavity erbium-doped fibre laser was employed as saturating source. To obtain a higher saturating power, laser emission was amplified by means of a second fibre amplifier.\n
Abstract In limit of saturation spectroscopy, we theoretically study the spectral hole burning (SHB) in the absorption spectrum of a probe field through a tripod atomic system. The response function for the probe field is calculated in a Doppler-broadened medium. Burning of spectral holes is observed only for the counter propagation of either one or both the coupling fields in the medium. The SHB is not observed below some critical temperature which is a condition for the electromagnetically induced transparency (EIT) in the medium. The most interesting and significant feature is that the Doppler broadening acts as a decoherence effect in case of EIT, however, the Doppler broadening acts inversely in case of SHB and consequently the burning effect enhances. The SHB is further enhanced and controlled by classes of the average velocity of atoms. The classes of high average atomic velocity in the medium increase the number of spectral hole burns (HBs). The widths of HBs can be controlled by the intensity of the driving fields. A single HB can be switched to multiple HBs in a well-controlled manner using different classes of high average atomic velocity. The various switchable holes can be burned in a desired position of the absorption spectrum which in turn simultaneously slow down multiple probe fields. The phenomenon of SHB may be useful in the construction of multichannel optical switching and storage devices.
We study CuBr nanocrystals embedded in a borosilicate matrix. The excitonic absorption line is strongly inhomogeneously broadened by the size dispersion of the quantum dots. We explore two ways in order to study the dephasing processes of the transition. The homogeneous absorption linewidth is first determined by spectral hole-burning (SHB) measurements, using a nanosecond dye laser excitation. We then perform degenerate four-wave-mixing experiments (FWM), using 100 fs pulses from a frequency-doubled Ti:sapphire laser. Due to the inhomogeneous broadening, we observe a so-called photon-echo signal and we measure its dynamics. From SHB experiments, we obtain homogeneous linewidths larger than 0.3 meV. From the FWM experiment, we obtain values smaller than 0.2 meV. These discrepancies between SHB and FWM measurements can be explained if we take into account the high excitation intensity necessary to induce absorption saturation in SHB experiments. Moreover, during the 20 ns pulses used, spectral diffusion may occur due to interactions between the nanocrystals and their matrix. Spectrally resolved four-wave-mixing experiments (SR-FWM) are also performed. The oscillations with a 250 fs period we observe at short time delays could be interpreted in terms of quantum beats between two-exciton and one-exciton states.