Allegations that our theoretical description of neutron scattering by entangled spin and spatial degrees of freedom is incorrect are shown to be misplaced for the allegations are derived from a naively incomplete, quantum mechanical calculation of neutron scattering by identical nuclei.
It is shown that quantum entanglement in condensed matter can be observed with scattering experiments if the energy resolution of the experiments enables a clear separation between the elastic scattering and the scattering from the excitations in the system. These conditions are not satisfied in recent deep inelastic neutron scattering experiments from hydrogen-containing systems that have been interpreted as showing the existence of quantum entanglement for short times in, for example, water at room temperature. It is shown that the theory put forward to explain these experiments is inconsistent with the first-moment sum rule for the Van Hove scattering function and we suggest that the theory is incorrect. The experiments were performed using the unique EVS spectrometer at ISIS and suggestions are made about how the data and their interpretation should be re-examined.
Several recent experiments on liquid and solid samples containing protons or deuterons show an interesting anomaly, which is a shortfall in the intensity of energetic neutrons scattered by the samples. Previously we demonstrated that quantum correlations in the spatial and spin degrees of freedom of the hydrogen isotopes lead to entanglement in scattering and a reduction in the scattered intensity. The viability of short-lived quantum correlations as the cause of the observed anomalies is further explored and found to be entirely feasible. General features of the basic premiss, that quantum entanglement reduces the scattered signal, are discussed and the interpretation of the neutron scattering experiments is set in context to related work on other systems. For the experiments in question, the duration of a scattering event, τ s , is a fraction of a femtosecond which is extremely short compared to solid-state relaxation times. Increasing τ s , by suitably changing experimental conditions, restores the intensity to the standard value calculated from the single atom cross-section and concentration of particles. Our physical picture of the restoration is evolution with increasing τ s from a pure state of the particles (described by a wavefunction) to a mixed state (described by a density matrix) that is created, through decoherence, by steadily engaging the solid-state environment of the particles.
Several recent experiments on liquid and solid samples containing protons or deuterons have shown an interesting anomaly, which is apparently absent when the hydrogen isotopes are replaced by heavier particles. The anomaly is a shortfall in the intensity of energetic neutrons scattered by the samples; specifically, the intensity per hydrogen isotope in bulk samples is smaller than the intensity for total scattering by an isolated hydrogen isotope. Short-lived correlations in the spatial and spin degrees of freedom of the hydrogen isotopes have been proposed as an explanation of the anomaly. The correlations involve entanglements of the degrees of freedom created by the requirements of quantum mechanics applied to identical particles. By using energetic neutrons to perform Compton scattering experiments on the hydrogen isotopes, the time scale of the experimental probe covers the region of ${10}^{\ensuremath{-}16}--{10}^{\ensuremath{-}15}\mathrm{s}$ where entangled states might still be expected to survive. The proposed explanation is pursued here by reporting the cross section for Compton scattering, also known as deep inelastic scattering, by two identical nuclei occupying nonequivalent states. The model reproduces the observed dependence of the cross section on energy transfer, in which intensity accumulates at the recoil energy of a single nucleus. Several features of the model demand that the intensity at the recoil energy is indeed less than the intensity for total scattering by an isolated nucleus. Although the pair approximation used here is unquestionably a first approximation to real many-body entanglements, it is a compelling explanation of all the observations, including the restoration of the normal cross section at longer observation times achieved by moving to longer scattering times.