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Physical review. B, Condensed matter

Marginal-Fermi-liquid behavior of charge carriers scattered by two-dimensional quantum antiferromagnetic spin fluctuations

Y. R. Wang, M. J. Rice, Han-Yong Choi

Published Oct 1, 1992• 7 citations
Publisher

Abstract

In the Wigner-Jordan (WJ) fermion representation of quantum spins with antiferromagnetic interaction, the WJ fermions always fill half of the total available states, and their energy spectrum possesses a particle-hole symmetry. These two intrinsic properties of the WJ representation, together with a finite density of states at small WJ-fermion excitation energy, give rise to the marginal-Fermi-liquid behavior of the charge carriers when they are scattered by the WJ fermions. The finite density of states of the WJ fermions at zero excitation energy is demonstrated for the defected quantum antiferromagnetic Heisenberg model in a square lattice.

DOI
10.1103/physrevb.46.8624

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In the Wigner-Jordan (WJ) fermion representation of quantum spins with antiferromagnetic interaction, the WJ fermions always fill half of the total available states, and their energy spectrum possesses a particle-hole symmetry. These two intrinsic properties of the WJ representation, together with a finite density of states at small WJ-fermion excitation energy, give rise to the marginal-Fermi-liquid behavior of the charge carriers when they are scattered by the WJ fermions. The finite density of states of the WJ fermions at zero excitation energy is demonstrated for the defected quantum antiferromagnetic Heisenberg model in a square lattice.
The excitation spectrum of the quantum antiferromagnetic Heisenberg model for a square lattice, as predicted from the in-phase flux state of Wigner-Jordan fermions, is calculated and compared with that calculated from conventional spin-wave theory. While the two spectra are overall similar, there are significant differences for short-wavelength excitations. The ratio of the excitation energy at wave vector (\ensuremath{\pi}/2,\ensuremath{\pi}/2) to that at (\ensuremath{\pi}/2,0) is predicted to be \ensuremath{\surd}2 for the Wigner-Jordan fermion excitations, and 2/ \ensuremath{\surd}3 for the spin-wave excitations. At long wavelengths, in contrast to the gapped spin-wave spectrum of Auerbach and Arovas, the excitation spectrum of Wigner-Jordan fermions is gapless at any finite temperature. Possible experimental examination of the excitation spectrum is discussed.
A disordered spin state, the nearest-neighbor virtual bonding state of Wigner-Jordan fermions, of the quantum antiferromagnetic Heisenberg model on a triangular lattice is found to have a zero-temperature energy -1.106J per spin, lower than that calculated from spin-wave theories, and in excellent agreement with that from numerical calculations, (-1.094\ifmmode\pm\else\textpm\fi{}0.018)J per spin. The excitations of the state are Wigner-Jordan fermions with a gapless spectrum. The low-temperature specific heat is predicted to be proportional to ${\mathit{T}}^{\ensuremath{\nu}}$, with \ensuremath{\nu} between 2/3 and 1, significantly deviating from the spin-wave prediction, T2{\mathit{T}}^{2}T2. At higher temperature, a broad peak in the specific heat near T/2J\ensuremath{\approxeq}0.75 is also predicted.
A Wigner-Jordan (WJ) transformation is used to study the one-dimensional (1D) and two-dimensional (2D) quantum antiferromagnetic Heisenberg model. The advantage of using the Wigner-Jordan transformation is that it preserves all spin-commutation relations as well as the spin on-site exclusion principle. In the 1D case a nearest-neighbor covalent-bonding state of the WJ fermions is found to have a ground-state energy (-0.4351J per site) comparable with that from the Bethe-ansatz solution (-0.4431J per site), and a linear energy spectrum at low energies with velocity 1.6366J, in close agreement with the velocity obtained by Haldane for the quantum antiferromagnetic Heisenberg model with 1/d2{\mathit{d}}^{2}d2 interaction (1.5708J). The method used for studying the 1D model is then applied to the 2D Heisenberg model in a square lattice. The resulting state at finite temperature is the in-phase flux state, i.e., a flux state of the Wigner-Jordan spinless fermions with an in-phase fermion orbital current circulating around each elementary plaquette.The single-particle excitation spectrum, i.e., the energy dispersion of reversing orientation of a spin in the system, of the in-phase flux state is overall similar to that of spin waves, with significant difference near the edge point k=(\ensuremath{\pi},0), at which the excitation energy of the WJ fermion is zero, whereas that of the spin-wave excitation is 2J. The specific heat of the in-phase flux state predicts a correct temperature dependence over the entire temperature range, namely a T2{\mathit{T}}^{2}T2 dependence at low temperature, a peak near T/J=0.6, and a 1/T2{\mathit{T}}^{2}T2 decreasing at high temperature. It also gives excellent agreement with the specific heat calculated from numerical methods. In contrast, the spin-wave theory only correctly predicts a T2{\mathit{T}}^{2}T2 dependence at low temperature. The Raman spectrum of the in-phase flux state is calculated and shows significant improvement over that from spin-wave theories compared with the experimental spectrum of La2{\mathrm{La}}_{2}La2​CuO4{\mathrm{CuO}}_{4}CuO4​. The exchange parameter, J, obtained from the comparison is 1060 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}1}$, in agreement with that obtained from analyzing the neutron-scattering data.
Spin and hole excitations are investigated in the doped two-dimensional (2D) antiferromagnets described by the t-J model based on the spin-wave approximation. The polarizability of spin excitations is found to be consistent with the marginal-Fermi-liquid hypothesis. As a consequence, the imaginary part of the self-energy for holes scattered by the spin excitations is demonstrated to give a linear dependence in temperature T (for \ensuremath{\omega}T) and in frequency \ensuremath{\omega} (for \ensuremath{\omega}>T).
The ground-state properties and spin excitation spectrum of the Heisenberg model are studied within the framework of the two-dimensional Jordan-Wigner theory. The mean-field state with the lowest energy is the magnetized \ensuremath{\pi}-flux state with a gap in the spin excitation spectrum. It is shown that this mean-field gap is decreased significantly by considering amplitude fluctuations in the random-phase approximation (RPA). The RPA ground-state energy and staggered magnetization are E0{\mathit{E}}_{0}E0​=-0.332J per bond and M=0.327, respectively, which are very close to the best numerical estimates. \textcopyright{} 1996 The American Physical Society.
The Jordan–Wigner transformation is applied to the spatially anisotropic spin-1/2 Heisenberg model on a square lattice with the nearest-neighbor and next-nearest-neighbor antiferromagnetic interactions. The transformed Hamiltonian describes the interacting spinless fermions that hop between neighbor sites in a gauge field. Using the mean-field-type approximation to both the direct interaction between fermions and the phase factors, which represent the gauge field, the problem is reduced to that concerning a free Fermi gas. Two types of antiferromagnetic ordering (the N´eel and collinear ones) are considered. By calculating the ground-state energies, the phase transitions induced by the interaction frustration were analyzed.