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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Rydberg excitation of ultracold atoms in optical lattices

Matthieu Viteau, J. Radogostowicz, Alessandro Zenesini, D. Ciampini, O. Morsch, E. Arimondo

Published Jun 1, 2009• 0 citations
Publisher

Abstract

Summary form only given. Interactions between neutral atoms are generally weak, but exciting these atoms in a Rydberg state considerably enhances their interaction through a long-range dipole-dipole potential. An interesting application of this dipole-dipole interaction is the dipole blockade in Rydberg excitation. This effect offers exciting possibilities for manipulating quantum bits stored in a single collective excitations in mesoscopic ensembles, or for realizing scalable quantum logic gate. The dipole blockade effect has been demonstrated in atomic ensembles by different groups, and recently also with two independently trapped atoms, which shows the possibility of creating entangle states and quantum logic gates. To extend and continue these results with more atoms, a promising method is to use atoms trapped in an optical lattice in the Mott insulator phase. To excite atoms into a Rydberg state, and to control the interactions and the dipole blockade, a high resolution laser scheme is needed. We use a two-photon excitation scheme 5s1/2rarr 6p3/2rarr ns or nd. The first step, at 420 nm, is realized by doubling a MOPA laser, with the second step at ~ 1000 nm. Both lasers are locked to a Fabry-Perot cavity, and the total excitation bandwidth is less than 3 MHz. After the excitation into the Rydberg state, we apply a pulsed electric field to ionize and detect the Rydberg atoms with an ion detector. To characterize and improve the efficiency of our ion detection, we have explored the direct ionization of ultracold atoms in a magneto-optical trap, or in a Bose-Einstein condensate. This calibration will allows us to characterize precisely the Rydberg excitation and to monitor its time evolution. First results on the Rydberg excitation of ultracold atoms in dipole traps and optical lattices will be presented. The prospect for creating Rydberg excitations inside a Mott insulator will also be discussed.

DOI
10.1109/cleoe-eqec.2009.5194834

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Summary form only given. Interactions between neutral atoms are generally weak, but exciting these atoms in a Rydberg state considerably enhances their interaction through a long-range dipole-dipole potential. An interesting application of this dipole-dipole interaction is the dipole blockade in Rydberg excitation. This effect offers exciting possibilities for manipulating quantum bits stored in a single collective excitations in mesoscopic ensembles, or for realizing scalable quantum logic gate. The dipole blockade effect has been demonstrated in atomic ensembles by different groups, and recently also with two independently trapped atoms, which shows the possibility of creating entangle states and quantum logic gates. To extend and continue these results with more atoms, a promising method is to use atoms trapped in an optical lattice in the Mott insulator phase. To excite atoms into a Rydberg state, and to control the interactions and the dipole blockade, a high resolution laser scheme is needed. We use a two-photon excitation scheme 5s1/2rarr 6p3/2rarr ns or nd. The first step, at 420 nm, is realized by doubling a MOPA laser, with the second step at ~ 1000 nm. Both lasers are locked to a Fabry-Perot cavity, and the total excitation bandwidth is less than 3 MHz. After the excitation into the Rydberg state, we apply a pulsed electric field to ionize and detect the Rydberg atoms with an ion detector. To characterize and improve the efficiency of our ion detection, we have explored the direct ionization of ultracold atoms in a magneto-optical trap, or in a Bose-Einstein condensate. This calibration will allows us to characterize precisely the Rydberg excitation and to monitor its time evolution. First results on the Rydberg excitation of ultracold atoms in dipole traps and optical lattices will be presented. The prospect for creating Rydberg excitations inside a Mott insulator will also be discussed.
We review here the studies performed about interactions in an assembly of cold Rydberg atoms. We focus especially on the review of the dipole–dipole interactions and on the effect of the dipole blockade in the laser Rydberg excitation, which offers attractive possibilities for quantum engineering. We present first the various interactions between Rydberg atoms. The laser Rydberg excitation of such an assembly is then described with the introduction of the dipole blockade phenomenon. We report recent experiments performed in this subject by starting with the case of a pair of atoms allowing the entanglement of the wave-functions of the atoms and opening a fascinating way for the realization of quantum bits and quantum gates. We consider then several works on the blockade effect in a large assembly of atoms for three different configurations: blockade through electric-field induced dipole, through Förster resonance, and in van der Waals interaction. The properties of coherence and cooperativity are analyzed. Finally, we treat the role of dipole–dipole interactions between Rydberg atoms responsible for Penning ionization. The perturbation of the dipole blockade by ions and the evolution of the Rydberg towards an ultracold plasma are discussed.
Abstract The dipole blockade effect at laser excitation of mesoscopic ensembles of Rydberg atoms lies in the fact that the excitation of one atom to a Rydberg state blocks the excitation of other atoms due to the shift in the collective energy levels of interacting Rydberg atoms. It is used to obtain the entangled qubit states based on single neutral atoms in optical traps. In this paper, we present our experimental results on the observation of the dipole blockade for mesoscopic ensembles of 1–5 atoms when they are detected by the selective field ionization method. We have investigated the spectra of the three-photon laser excitation 5S1/2 → 5P3/2 → 6S1/2 → nP3/2 of cold Rydberg Rb atoms in a magneto-optical trap. We have found that for mesoscopic ensembles this method allows only a partial dipole blockage to be observed. This is most likely related to the presence of parasitic electric fields reducing the interaction energy of Rydberg atoms, the decrease in the probability of detecting high states, and the strong angular dependence of the interaction energy of Rydberg atoms in a single interaction volume.
Ultracold cesium n S ( n =60–70) Rydberg atoms are prepared using the two-photon scheme in a magneto-optical trap (MOT). The number of resonant Rydberg atoms is measured by the pulsed field ionization technique, and the dependences of the Rydberg signal on excitation duration and external DC electric field are investigated. The excitation dynamics and blockade effects due to long-range interactions are obtained. The effect of external electric field on Rydberg excitation is also investigated, and the experimental result shows an enhanced blockade with a weak external electric field.
We have performed two-photon excitation via the 6 2 P 3/2 state to the n = 50–80 S or D Rydberg state in Bose–Einstein condensates of rubidium atoms. The Rydberg excitation was performed in a quartz cell, where electric fields generated by plates external to the cell created electric charges on the cell walls. Avoiding accumulation of the charges and realizing good control over the applied electric field was achieved when the fields were applied for only a short time, typically a few microseconds. Rydberg excitations of the Bose–Einstein condensates loaded into quasi-one-dimensional traps and in optical lattices have been investigated. The results for condensates expanded to different sizes in the one-dimensional trap agree well with the intuitive picture of a chain of Rydberg excitations controlled by the dipole–dipole interaction. The optical lattice applied along the one-dimensional geometry produces localized, collective Rydberg excitations controlled by the nearest-neighbour blockade.
Creating ultracold Rydberg atoms in lattices imprinted with a spatial light modulator offers the possibility to simulate quantum processes. Strong dipole forces between Rydberg atoms provide the required correlations between lattice sites. With a high ground-state atomic density per lattice site, blockade phenomenon may induce single Rydberg atom occupancy per lattice site. Readout of resulting patterns requires single-atom detection with spatial resolution. The grand challenge is to create systems of interacting Rydberg atoms with scalability. So far, we have achieved spatial imaging of Rydberg atoms using ion optics and incorporated in-vacuo aberration correction for imprinted light patterns. Presently, we are studying the effect of dipole blockade on Rydberg excitation statistics. For this we have set up a tuneable Rydberg excitation laser system using an ultra stable reference. Measurements of spatial correlation functions show that achieving a blockade radius of 10 μm is possible. Combined with a dark-spot MOT, this is sufficient to achieve precisely one Rydberg atom per lattice site.
High resolution laser Stark excitation of np (60<n<85) Rydberg states of ultracold cesium atoms shows an efficient blockade of the excitation attributed to long-range dipole-dipole interaction. The dipole blockade effect is observed as a quenching of the Rydberg excitation depending on the value of the dipole moment induced by the external electric field. Effects of ions which could match the dipole blockade effect are discussed in detail but are ruled out for our experimental conditions. Analytic and Monte Carlo simulations of the excitation of an ensemble of interacting Rydberg atoms agree with the experiments and indicate a major role of the nearest neighboring Rydberg atom.