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Quantum Electronics

Polarisation and dispersion properties of light shifts in ultrastable optical frequency standards

V. D. Ovsyannikov, Vitalii G Pal'chikov, Hidetoshi Katori, Masao Takamoto

Published Jan 31, 2006• 38 citations
Publisher

Abstract

The theoretical aspects of the Stark spectroscopy of cold alkaline-earth atoms in a three-dimensional optical lattice related to the development of ultrastable optical frequency standards of a new generation are considered. The main attention is devoted to the dispersion and polarisation properties of the light frequency shift in these atoms, which depend on the power, frequency, and polarisation of lasers forming the optical lattice. The 'light-shift-cancellation' regime is considered in detail, in which the second-order dynamic Stark shifts at the forbidden clock 3 P 0 — 1 S 0 and 3 P 1 — 1 S 0 transitions are mutually compensated. The wavelengths at which this regime takes place ('magic' wavelengths) are calculated for the He, Be, Mg, Ca, Sr, Yb, and Hg atoms. The fourth-order dynamic susceptibilities (hyperpolarisabilities) are calculated for Sr atoms and the contribution of higher-order multipole corrections to the dynamic polarisability of the 3 P 0 and 1 S 0 levels is estimated.

DOI
10.1070/qe2006v036n01abeh013098

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The theoretical aspects of the Stark spectroscopy of cold alkaline-earth atoms in a three-dimensional optical lattice related to the development of ultrastable optical frequency standards of a new generation are considered. The main attention is devoted to the dispersion and polarisation properties of the light frequency shift in these atoms, which depend on the power, frequency, and polarisation of lasers forming the optical lattice. The 'light-shift-cancellation' regime is considered in detail, in which the second-order dynamic Stark shifts at the forbidden clock 3 P 0 — 1 S 0 and 3 P 1 — 1 S 0 transitions are mutually compensated. The wavelengths at which this regime takes place ('magic' wavelengths) are calculated for the He, Be, Mg, Ca, Sr, Yb, and Hg atoms. The fourth-order dynamic susceptibilities (hyperpolarisabilities) are calculated for Sr atoms and the contribution of higher-order multipole corrections to the dynamic polarisability of the 3 P 0 and 1 S 0 levels is estimated.
The light frequency shifts induced by an external laser field are calculated for the spin-forbidden 3 P J — 1 S 0 transitions in Mg, Sr, and Yb atoms. The calculations are performed within the framework of the perturbation theory using experimentally measured transition energies. The calculations of the higher-order dynamic Stark effect were initiated by precision measurements of trapped and cooled atoms as well as by the development of a highly stable optical atomic clock. The dispersion properties of the polarisability and hyperpolarisability components are analysed in the vicinity of resonances and so-called cross points for the ground and excited atomic levels. The radial matrix elements were calculated by the Green function method for the model potential.
Higher-order perturbation theory is used to study frequency shifts of the spin-forbidden 3 P J - 1 S 0 transitions for Mg, Sr and Yb atoms in an external laser field. Calculations of the higher-order dynamic Stark effect have been performed in connection with precise measurements on cooled and trapped atoms and the design of ultra stable optical clock in an engineered light shift trap. The form of the model potential of the valence electrons suggested by Simons is used for the calculation of atomic dynamic characteristics given by second- and fourth-order perturbation theory for the interaction of the atoms with the electromagnetic field. Dispersion properties of the polarizability and hyperpolarizability components and their behavior in the vicinity of both resonances and so-called magic wavelengths for the upper and lower atomic states, are analyzed. Calculations of ac multipole polarizabilities and dipole hyperpolarizabilities for the 3 P 0 - 1 S 0 clock transition in 87 Sr indicate that the contribution of the higher- order light shifts can be reduced to less than 1 mHz, allowing for a projected accuracy of better than 10 -17 .
The circular polarized laser beam of the “magic” wavelength used to produce an optical lattice for the time-frequency standard on neutral atoms may mix the 3P 1 state to the long-living metastable state 3P 0 thus providing significant enhancement of the strongly forbidden 1S 0 -3P 0 clock transition in even isotopes of alkaline-earth-like atoms. We present a detailed analysis of various factors influencing resolution and uncertainty for this kind of optical standard, including precise estimations of the “magic” wavelengths, transition matrix elements and field induced second- and fourth-order ac Stark shifts for the ground and metastable alkaline-earth-like atoms.
The progress in optical clock with uncertainty at a level of 10−1810^{-18}10−18 requires unprecedented precision in estimating the contribution of multipolar and higher-order effects of atom-field interactions. Previous theoretical and experimental results of dynamic multipolar polarizabilities and hyperpolarizabilities at the 813 nm magic wavelength of the Sr clock differ substantially. We employ the sum-over-states method to calculate dynamic multipolar polarizabilities and hyperpolarizabilities for the Sr and Mg clocks. Our differential dynamic hyperpolarizability at the magic wavelength of 813.4280(5) nm for the Sr clock is −2.09(43)×107-2.09(43)\times10^{7}−2.09(43)×107 a.u., which agrees well with the recent theoretical and measurement results. Our differential multipolar polarizability of the Sr clock is 2.68(94)×10−52.68(94)\times 10^{-5}2.68(94)×10−5 a.u., which is consistent with the theoretical work of Porsev {\em et al.} [Phys. Rev. Lett. 120, 063204 (2018)], but different from recent measurement of Ushijima {\em et al.} [Phys. Rev. Lett. 121, 263202 (2018)]. In addition, the lattice light shifts as the detuning and trap depth changed are studied in detail by using present multipolar polarizability and hyperpolarizability. It illustrates that for the Mg clock, there exists a distinctive operational lattice depth of 5.3(1)ER5.3(1)E_R5.3(1)ER​ that allows the total light shift reduced to less than 1×10−181\times 10^{-18}1×10−18 over the trap depth variation of 4.1ER<U<6.4ER4.1E_R<U<6.4E_R4.1ER​<U<6.4ER​.
Magic-wave-induced 1S0−3P0^1S_0-^3P_01S0​−3P0​ transition in even isotopes of alkaline-earth-like atoms
The circular polarized laser beam of the ``magic'' wavelength may be used for mixing the 3P1^3P_13P1​ state into the long-living metastable state 3P0^3P_03P0​, thus enabling the strictly forbidden 1S0^1S_01S0​−-−3P0^3P_03P0​ ''clock'' transition in even isotopes of alkaline-earth-like atoms, without change of the transition frequency. In odd isotopes the laser beam may adjust to an optimum value the line width of the "clock" transition, originally enabled by the hyperfine mixing. We present a detailed analysis of various factors influencing resolution and uncertainty for an optical frequency standard based on atoms exposed simultaneously to the lattice standing wave and an additional "state-mixing" wave, including estimations of the "magic" wavelengths, Rabi frequencies for the ''clock'' and state-mixing transitions, ac Stark shifts for the ground and metastable states of divalent atoms.
The development of optical frequency standards with a relative uncertainty of reproducing the time and frequency units at a level as low as 10 −17 –10 −18 calls for an unprecedented accuracy in estimating the role of higher orders of optical nonlinearity, caused by the influence of the optical lattice on the frequency shift of the 'clock transition'. This paper presents a systematic calculation of the contributions of multipole nonlinear anharmonic effects to the error of clocks based on optical lattices for alkaline-earth-like Sr, Yb, and Hg atoms.