Precision Measurements with Ion Traps

A. Walther, U. Poschinger, K. Singer +1 more

Pradip Kumar Ghosh

Abstract In this chapter we present applications of ion traps to: (i) determination of the g-value of an electron from electron spin resonance experiments on a single electron, (ii) observation of quantum jumps in a single trapped ion, (iii) an experimental test of the quantum Zeno effect, (iv) a precision test of the linearity of quantum mechanics, (v) a range of studies on one-component microplasmas, (vi) optical spectroscopy of molecular ions, (vii) precision mass measurement of stable isotopes, (viii) precision mass measurement of radioactive isotopes, (ix) trapping and precision mass measurement of antimatter, specifically of antiprotons, (x) lifetime measurement of neutron undergoing beta decay, and (xi) atomic physics of highly charged ions.

Kevin Sheridan

A range of experimental techniques for application in reaction studies between ionic and neutral atoms/molecules and high resolution spectroscopy experiments with sympathetically cooled molecular ions are presented. A novel ion trap loading scheme using the photo-ionisation of atoms generated by the pulsed laser ablation of a solid calcium target has been characterised. We have identified the range of ablation laser fluences that must be used in order to produce a flux of neutral calcium atoms, which is a prerequisite for isotope selective ion trap loading. Calcium ions are trapped and laser cooled in a linear radio-frequency ion trap. We have developed a spectroscopy scheme that allows the entire fluorescence spectrum of trapped ions to be rapidly collected with high precision while maintaining a low ion temperature and good ion localisation throughout interrogation. The scheme has been demonstrated by measuring the saturation intensity of the calcium ion 4S1/2?4P1/2 transition. We have developed a novel scheme to measure the secular motion of trapped ions and demonstrated the application of the technique to ion-neutral collision reaction experiments. Employing pulsed excitation and Doppler velocimetry, we have measured the centre-of-mass mode frequency of single ions as well as large ion crystals with a frequency precision better than 2x10-3 within an interrogation time on the order of seconds. This method has been used to measure the mass of ions and observe charge exchange collisions between trapped calcium isotopes. In particular, we have measured the 44Ca++40Ca!40Ca++44Ca reaction cross section and demonstrated the single-event resolution of the technique. Finally, we have developed a novel all-optical broadband scheme for exciting, amplifying and measuring the secular motion of ions in the trap. Oscillation induced by optical excitation has been coherently amplified to control and measure the ion's secular motion. Requiring only a single interrogation laser, the ion's oscillation amplitude can be precisely controlled. The application of this technique to non-destructive spectroscopy of trapped molecular ions is discussed.

Günther Werth

Martina Knoop

Fabian Wolf

Optical atomic clocks based on trapped ions suffer from systematic frequency shifts of the clock transition due to interaction with blackbody radiation from the environment. These shifts can be compensated if the blackbody radiation spectrum and the differential dynamic polarizability is known to a sufficient precision. Here, we present a new measurement scheme, based on quantum logic that allows a direct transfer of precision for polarizability measurements from one species to the other. This measurement circumvents the necessity of calibrating laser power below the percent level, which is the limitation for state-of-the-art polarizability measurements in trapped ions. Furthermore, the presented technique allows one to reference the polarizability transfer to hydrogenlike ions for which the polarizability can be calculated with high precision.