We present a general method for calculating the fraction of energy stored in a medium that is transferable to an optical pulse. We also calculate the minimum energy required to create a pulse/medium excitation.
We discuss the inevitable dissipation of energy that must accompany the creation of a pulse-medium excitation state in a passive dielectric. We show that there is a minimum amount of energy that an optical pulse must deposit in the medium to create a given pulse-medium state and that energy deposited beyond this minimum value must be dissipated in the medium. We compare this notion of dissipation to a related concept found by determining the fraction of energy stored in a medium that is irrecoverable by future fields. These two notions of dissipation are model-independent and form upper and lower bounds for real-time loss. Any model-dependent notion of loss that falls outside these bounds has serious conceptual difficulties. We show that a traditional notion of real-time loss based on a multiple-Lorentz oscillator model fails to give reasonable results in classes of passive linear media near EIT, while the notions of loss we introduce give sensible results for all passive media.
Pulse reshaping effects that give rise to fast and slow light phenomena are inextricably linked to the dynamics of energy exchange between the pulse and the propagation medium. Energy that is dissipated from the pulse can no longer participate in this exchange process, but previous methods of calculating real-time dissipation are not valid for extended propagation media. We present a method for calculating real-time dissipation that is valid for electromagnetic pulse propagation in extended media. This method allows one to divide the energy stored in an extended medium into the portion that can be later transmitted out of the medium, and that portion which must be lost to either dissipation or reflection.
We investigate ultrashort pulse propagation in a dense medium of two-level atoms. We numerically solve the coupled nonlinear Maxwell-Bloch equations by assuming that the fields are slowly varying in time only. We find that while intrinsic optical switching of the atomic inversion persists in extended media, self-phase-modulation effects, coherent energy transfer, and reflections can be large even for films that are only a small fraction of a wavelength thick. If the propagation distance is sufficiently large, a physical boundary that separates fully excited atoms from atoms in the ground state can be created within the medium. In turn, this leads to a rapid spatial modulation of the nonlinear polarization, and a deterioration of the intrinsic optical switching mechanism. We then show that, although the slowly varying envelope approximation in space may be preempted by the fast longitudinal variation of the field and atomic variables, the mean-field approximation remains valid in the regime of ultrafast optical switching, provided the film thickness is sufficiently small such that the medium is nearly uniformly excited. These results are generated by utilization of our calculational method that fully accounts for the longitudinal dynamics of the fields, including reflections.