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Physical Review Letters

Phase-Coupling-Induced Ultraslow Light Propagation in Solids at Room Temperature

Guoquan Zhang, Bo Fang, Rong Dong, Jingjun Xu

Published Sep 23, 2004• 69 citations
Publisher

Abstract

We show that the group velocities of light pulses can be decelerated dramatically by the use of a dispersive phase-coupling effect through a wave mixing process. We have observed experimentally such a phase-coupling-induced ultraslow light propagation with a group velocity as low as $0.05\text{ }\text{ }\mathrm{m}/\mathrm{s}$ in a photorefractive ${\mathrm{B}\mathrm{i}}_{12}{\mathrm{S}\mathrm{i}\mathrm{O}}_{20}$ crystal at room temperature. Moreover, the ultraslow light is amplified in the ${\mathrm{B}\mathrm{i}}_{12}{\mathrm{S}\mathrm{i}\mathrm{O}}_{20}$ crystal because of the unidirectional energy transfer from a coupling beam to the ultraslow light. This technique to produce ultraslow light propagation is valid for all nonlinear wave mixing processes with a dispersive phase-coupling effect.

DOI
10.1103/physrevlett.93.133903

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We show that the group velocities of light pulses can be decelerated dramatically by the use of a dispersive phase-coupling effect through a wave mixing process. We have observed experimentally such a phase-coupling-induced ultraslow light propagation with a group velocity as low as 0.05  m/s0.05\text{ }\text{ }\mathrm{m}/\mathrm{s}0.05  m/s in a photorefractive Bi12SiO20{\mathrm{B}\mathrm{i}}_{12}{\mathrm{S}\mathrm{i}\mathrm{O}}_{20}Bi12​SiO20​ crystal at room temperature. Moreover, the ultraslow light is amplified in the Bi12SiO20{\mathrm{B}\mathrm{i}}_{12}{\mathrm{S}\mathrm{i}\mathrm{O}}_{20}Bi12​SiO20​ crystal because of the unidirectional energy transfer from a coupling beam to the ultraslow light. This technique to produce ultraslow light propagation is valid for all nonlinear wave mixing processes with a dispersive phase-coupling effect.
We demonstrated superluminal light propagation with a negative group velocity of -5.7 m/s in a photorefractive Bi 12SiO20 crystal by using the dispersive phase coupling effect in a nondegenerate two-wave mixing process. To the best of our knowledge, this is the first experimental demonstration of superluminal light propagation at room temperature in solids by using a classical wave mixing technique. In addition, we showed the tunability of the group velocity of light between the negative (superluminal light) and the positive (subluminal light) by simply tuning the experimental conditions such as the frequency of the coupling beam, the incident intensity, and the externally applied electric fields.
We show theoretically that the group velocity of light pulses can be reduced significantly by use of the steep dispersion properties of the phase coupling effect in the photorefractive two-wave mixing process. The group velocity of light pulses of the order of 0.1 m/s can be achieved in typical photorefractive BSO crystals with an appropriate externally applied electric field and moving gratings of appropriate speeds. It is also shown that the slowly propagating light pulses can be set to be amplified after passing through the photorefractive material.
We demonstrate slow and fast light at room temperature by dispersive phase-coupling in a photorefractive SBN:60 crystal. Non-degenerated wave-mixing is used to obtain delayed and amplified pulses with reduced or increased group velocity of vg = 0. 2c m s −1 and vg =− 1. 3c m s −1 , respectively. The gain spectrum is modulated by using multiple frequency shifted pumps simultaneously. The complete dispersion of the spectrum is determined via the phase modulation technique. We compare the experimental results to numerical simulations based on coupled-wave equations.
Summary form only given. Electromagnetically induced transparency (EIT) has been the subject of many experimental and theoretical studies over recent years. Most recently, substantial experimental and theoretical work in this area has been focused on the use of EIT to give ultraslow group velocities for light in both ultracold atomic gas and hot atomic vapors. Much of this interest is based on the fact that slowing the group velocity of a laser pulse down to the speed of sound in the same material can produce strong coupling between acoustic waves and the electromagnetic field. It has been suggested that a giant nonlinearity obtained by this method might be utilized for efficient multi-wave mixing and quantum nondemolition measurements. Slow light might also allow a very efficient nonlinear interaction between laser pulses of extremely low (down to a single photon) energies. Here, we report the first direct observation of an ultraslow group velocity of light down to 45 m/s in a solid, well below the speed of sound in the medium. This group velocity is fundamentally limited only by the inhomogeneous broadening of the ground state transition. At low coupling beam intensities, the fraction of centers that are pumped into the "dark state" increases with coupling laser power, so that the observed group delay is increasing with coupling beam intensity. At higher intensities, power broadening reduces the sharpness of the dispersive feature and the observed group delay decreases.
Slow and fast light are achieved in two experiments using SPS photorefractive crystal at room temperature. We report that the photorefractive gain achieved by the two wave mixing (TWM) method can control the group velocity of the transmitted light pulses at visible wavelength. It is shown theoretically and experimentally that the time delay and the shape of the output pulse change as a function of the photorefractive gain. The beam fanning has also been used to control the velocity propagation of a single light pulse in the same crystal at λ = 1064 nm. Depending on the orientation of the polar axis, it is possible to accelerate or decelerate a short pulse with duration of order of μs in the crystal.