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Chemical Physics

Partitioning of entangling interactions in terms of rotating wave approximation: An approach to the Bell state generation by laser fields

K. Mishima, Koichi Yamashita

Published Oct 2, 2007• 10 citations
Publisher
DOI
10.1016/j.chemphys.2007.09.041

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In this paper, we extend our theoretical work on the pure state entanglement of bipartite or two-mode physical and chemical systems interacting with general static entangling interactions and external electromagnetic fields to include the mixed state entanglement. It is assumed that the Markov approximation is valid in our model system. Based on the partitioning of the entangling interaction matrix, we investigate the effect of the entangling interaction matrix elements and the relaxation constants on the decoherence of the Bell states. Our calculations indicate that only a few elements of the entangling interaction matrix and relaxation constants are dominant for the decoherence dynamics of the Bell states.
It is well established that an entanglement encoded in the Bell states of a two-qubit system with correlated spins exhibits completely different evolution properties from that encoded in states with the anticorrelated spins. A complete and abrupt loss of the entanglement, called the entanglement sudden death, can be found to occur for the spin-correlated states, but the entanglement evolves without any discontinuity or decays asymptotically for the spin-anticorrelated states. We consider the evolution of an initial entanglement encoded in the spin-anticorrelated states and demonstrate that the asymptotic behavior predicted before occurs only in the weak-coupling limit or equivalently when the rotating-wave approximation (RWA) is made on the interaction Hamiltonian of the qubits with the field. If we do not restrict ourselves to the RWA, we find that the entanglement undergoes a discontinuity, the sudden-death phenomenon. We illustrate this behavior by employing an efficient scheme for entanglement evolution between two cold-trapped atoms located inside a single-mode cavity. Although only a single excitation is initially present in the system, we find that the two-photon excited state, which plays the key role for the discontinuity in the behavior of the entanglement, gains a population over a short time of the evolution. When the RWA is made on the interaction, the two-photon excited state remains unpopulated for all times and the discontinuity is absent. We attribute this phenomenon to the principle of complementarity between the evolution time and energy, and the presence of the counter-rotating terms in the interaction Hamiltonian.