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Physical Review

Correlation Function Method for Transport Phenomena

Hazime Mori

Published Jul 15, 1959• 61 citations
Publisher

Abstract

An expression for the nonequilibrium density matrix is derived in terms of dynamical fluxes, which leads to a rigorous formulation of the correlation function method for transport phenomena with nonuniform thermodynamic quantities.
DOI
10.1103/physrev.115.298

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In this paper, we formally demonstrate that the nonequilibrium density matrix developed by Hershfield for the steady state has the form of a McLennan-Zubarev nonequilibrium ensemble. The correction term in this pseudoequilibrium Gibbs-like ensemble is directly related to the entropy production in the quantum open system. The fact that both methods state that a nonequilibrium steady state can be mapped onto a pseudoequilibrium, permits us to develop nonequilibrium quantities from formal expressions equivalent to the equilibrium case. We provide an example: the derivation of a nonequilibrium distribution function for the electron population in a scattering region in the context of quantum transport.
Building upon Zubarev's nonequilibrium statistical operator formalism, we derive a relativistic canonical-like second-order spin hydrodynamics for two power-counting schemes. We obtain comprehensive second-order expressions for dissipative fluxes, including the shear stress tensor, bulk viscous pressure, charge-diffusion currents, rotational stress tensor, boost heat vector, and spin tensor-related dissipative flux. By introducing novel transport coefficients and expressing them in terms of equilibrium correlation functions, we establish new Kubo-type formulas for second-order transport. Our findings have significant implications for understanding the collective spin dynamics of strongly interacting matter and provide a robust theoretical basis for future experimental and theoretical studies.