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Soviet Journal of Quantum Electronics

Resonant four-wave interaction in the field of pump waves of arbitrary intensity

Anatolii A Afanas'ev, С. П. Жвавый

Published Jun 30, 1985• 0 citations
Publisher

Abstract

A theoretical investigation is made of the influence of the asymmetry of the intensities of pump waves on the spectrum of weak radiation participating in a nondegenerate four-wave interaction in a resonant medium with a homogeneously broadened absorption line. It is shown that a difference between the intensities of pump waves results in additional modulation of the spectrum of reflected and transmitted waves. In particular, an increase in the asymmetry of the pump wave intensities increases the phase mismatch between the waves and reduces the central maximum in the weak radiation spectrum. When the difference between the intensities of the pump waves becomes sufficiently large, this central maximum of the reflected radiation disappears completely and the side maxima acquire a doublet structure. It is shown that the position of the maxima in the reflected radiation spectrum corresponds exactly to the minima of the phase matching between the waves. An analysis is made of the characteristics of a reflecting narrow-band optical filter based on a nondegenerate four-wave interaction in a resonant medium.

DOI
10.1070/qe1985v015n06abeh007159

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A theoretical investigation is made of the influence of the asymmetry of the intensities of pump waves on the spectrum of weak radiation participating in a nondegenerate four-wave interaction in a resonant medium with a homogeneously broadened absorption line. It is shown that a difference between the intensities of pump waves results in additional modulation of the spectrum of reflected and transmitted waves. In particular, an increase in the asymmetry of the pump wave intensities increases the phase mismatch between the waves and reduces the central maximum in the weak radiation spectrum. When the difference between the intensities of the pump waves becomes sufficiently large, this central maximum of the reflected radiation disappears completely and the side maxima acquire a doublet structure. It is shown that the position of the maxima in the reflected radiation spectrum corresponds exactly to the minima of the phase matching between the waves. An analysis is made of the characteristics of a reflecting narrow-band optical filter based on a nondegenerate four-wave interaction in a resonant medium.
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An analysis is made of nondegenerate four-wave interaction (FWI) in a resonant medium (two-level model) with Doppler line broadening allowing for nonlinear absorption of the weak radiation. The cubic approximation with respect to the field is used to derive expressions for the coefficients of parametric coupling and absorption of the mixed waves. The angular dependences of the reflection coefficient are studied for quasicollinear and orthogonal FWI geometries. It is shown that, as a result of the thermal motion of the particles, the dependence of the reflection coefficient on the angle θ between the interacting waves results in considerable limitation of the angular width of the reversed beams. This limitation is greater for degenerate FWI. In the case of nondegenerate FWI, as a result of the selective action of waves on groups of atoms having a specific velocity projection, the reversal efficiency may increase on increase in θ.
A theoretical analysis is made of the efficiency of wavefront reversal under conditions of a degenerate form of the four-wave interaction in a resonantly absorbing (amplifying) medium allowing for changes in the pump waves as a result of their natural resonant absorption (amplification). The coefficient of reflection into a reversed wave is obtained as a function of the optical thickness of a layer of the medium, the boundary values of the pump wave intensity, and the shift of the field frequency from the line center. The optimal values of these parameters and the corresponding maximum reflection coefficient are determined.
A theoretical analysis is made of a four-wave parametric interaction accompanied by reversal of the signal wavefront in a thin layer of a two-level medium as a result of a two-photon resonance of opposite waves of randomly modulated pumping. An allowance is made for the inertia of the interaction, saturation of the transition involved in the interaction, Stark shift of the levels, and width of the pump spectrum. A study is made of the influence of random modulation of the pump waves on the average value and relative variance of the intensity of the reversed wave. It is shown that the relative amplitude of the intensity fluctuations of the reversed wave is minimal when the maximum average intensity is reached.
The formulation of phase conjugation via nondegenerate four-wave mixing in a homogeneously broadened resonant medium is generalized to include saturating pump waves. An ultrahigh-Qoptical filter is predicted, showing both gain and a bandwidth less than the homogeneous linewidth of the atom. The dependence of the filter function on the ac Stark effect and on the use of asymmetric pump wave intensities is discussed. In addition, several new phenomena are shown which manifest themselves as a dip in the degenerate reflectivity at line center.
An investigation is reported of the characteristic features of four-wave interaction of a chirped signal with bandwidth-limited pump waves in a resonant medium modelled by a two-level scheme. Analytic estimates are obtained and a numerical analysis is made of the combined influence of various mechanisms (spatial phase matching, a finite nonlinear response time, and phase cross-modulation) on the spectral composition and on the temporal behaviour of the fourth pulse. Conditions are found for achieving, with practically undetectable distortions, phase conjugation of a chirped signal accompanied by shortening of the pulse envelope and narrowing of the spectrum of the phase-conjugate wave.