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Journal of Magnetism and Magnetic Materials

Spin dynamics of spin-Peierls transition in quantum Heisenberg antiferromagnetic chain

Atsuko Kouzuki, Natsuko Maya, 和子 川崎, Katsuhiro Nakamura

Published Jan 1, 1998• 0 citations
Publisher
DOI
10.1016/s0304-8853(97)00976-1

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Spin dynamics of the spin-Peierls transition in a quantum Heisenberg antiferromagnetic chain

Atsuko Kouzuki, 和子 川崎, Katsuhiro Nakamura

We investigate full dynamical behaviors of the spin-Peierls transition in $S=1/2$ Heisenberg antiferromagnetic chains by means of two-time Green's functions. The effect of temperature-dependent lattice displacements is incorporated self-consistently. Depending on temperature T and transfer wave number k, the imaginary part of the dynamical susceptibility ${\ensuremath{\chi}}_{\mathrm{zz}}^{\ensuremath{''}}(k,\ensuremath{\omega})$ shows rich structures: At $T=0,$ it is nonvanishing in the frequency region ${\ensuremath{\Omega}}_{M}(k)<\ensuremath{\Omega} (\ensuremath{\equiv}\ensuremath{\Elzxh}\ensuremath{\omega}/J)<{\ensuremath{\Omega}}_{H}(k).$ ${\ensuremath{\Omega}}_{M}(k)$ denotes a lower edge of a triplet magnetic excitation continuum, and is finite at $k=0$ due to lattice distortion. The upper edge ${\ensuremath{\Omega}}_{H}(k)$ increases as $k=0$ is approached, which is completely different from the feature without lattice distortion. An asymmetric line shape of ${\ensuremath{\chi}}_{\mathrm{zz}}^{\ensuremath{''}}(k,\ensuremath{\omega})$ is found with a peak at the frequency slightly higher than ${\ensuremath{\Omega}}_{M}(k).$ At $0<T<{T}_{\mathrm{SP}}$ (spin-Peierls transition point) there appears another structure due to thermal fluctuations in the lower-frequency region, $0<\ensuremath{\Omega}<{\ensuremath{\Omega}}_{L}(k).$ Since ${\ensuremath{\Omega}}_{L}(k)<{\ensuremath{\Omega}}_{M}(k),$ the forbidden band always exists at $T<{T}_{\mathrm{SP}}.$ Above ${T}_{\mathrm{SP}},$ ${\ensuremath{\chi}}_{\mathrm{zz}}^{\ensuremath{''}}(k,\ensuremath{\omega})$ reduces to a smooth curve characterized by a single broad maximum. These features in dynamics are systematically explained in terms of different quasiparticle scattering processes proper to the spin-Peierls phase. The results are compared with recent experimental data of neutron scattering for the inorganic compound ${\mathrm{CuGeO}}_{3}.$

Physical review. B, Condensed matter•Nov 1, 1999•10 citations

Spin-Peierls Instabilities vs Antiferromagnetic Transition and Phonon Dynamics

Yasunari Kurihara

We discuss a competition between a spin-Peterls state and the antiferromagnetic state for a Heisenberg antiferromagnetic linear chain system including a phonon Hamiltonian. A Hartree-Fock approximation is applied to a Hamiltonian redescribed in terms of spin-less fermions. We get Dyson's equation of phonons which is consistent with this Hartree-Fock approximation. We point out that Pytte's work is not still complete even in the framework of the Hartree-Fock theory since a term was left out there which gave a quantitative difference between the Heisenberg model and the X Y model. We find the softening of phonons in the antiferromagnetic state which has overcome the spin-Peierls state.

Journal of the Physical Society of Japan•Mar 1, 1984•2 citations
We investigate full dynamical behaviors of the spin-Peierls transition in S=1/2S=1/2S=1/2 Heisenberg antiferromagnetic chains by means of two-time Green's functions. The effect of temperature-dependent lattice displacements is incorporated self-consistently. Depending on temperature T and transfer wave number k, the imaginary part of the dynamical susceptibility ${\ensuremath{\chi}}_{\mathrm{zz}}^{\ensuremath{''}}(k,\ensuremath{\omega})$ shows rich structures: At T=0,T=0,T=0, it is nonvanishing in the frequency region ${\ensuremath{\Omega}}_{M}(k)<\ensuremath{\Omega} (\ensuremath{\equiv}\ensuremath{\Elzxh}\ensuremath{\omega}/J)<{\ensuremath{\Omega}}_{H}(k).$ ${\ensuremath{\Omega}}_{M}(k)$ denotes a lower edge of a triplet magnetic excitation continuum, and is finite at k=0k=0k=0 due to lattice distortion. The upper edge ${\ensuremath{\Omega}}_{H}(k)$ increases as k=0k=0k=0 is approached, which is completely different from the feature without lattice distortion. An asymmetric line shape of ${\ensuremath{\chi}}_{\mathrm{zz}}^{\ensuremath{''}}(k,\ensuremath{\omega})$ is found with a peak at the frequency slightly higher than ${\ensuremath{\Omega}}_{M}(k).$ At 0<T<TSP0<T<{T}_{\mathrm{SP}}0<T<TSP​ (spin-Peierls transition point) there appears another structure due to thermal fluctuations in the lower-frequency region, $0<\ensuremath{\Omega}<{\ensuremath{\Omega}}_{L}(k).$ Since ${\ensuremath{\Omega}}_{L}(k)<{\ensuremath{\Omega}}_{M}(k),$ the forbidden band always exists at T<TSP.T<{T}_{\mathrm{SP}}.T<TSP​. Above TSP,{T}_{\mathrm{SP}},TSP​, ${\ensuremath{\chi}}_{\mathrm{zz}}^{\ensuremath{''}}(k,\ensuremath{\omega})$ reduces to a smooth curve characterized by a single broad maximum. These features in dynamics are systematically explained in terms of different quasiparticle scattering processes proper to the spin-Peierls phase. The results are compared with recent experimental data of neutron scattering for the inorganic compound CuGeO3.{\mathrm{CuGeO}}_{3}.CuGeO3​.
We discuss a competition between a spin-Peterls state and the antiferromagnetic state for a Heisenberg antiferromagnetic linear chain system including a phonon Hamiltonian. A Hartree-Fock approximation is applied to a Hamiltonian redescribed in terms of spin-less fermions. We get Dyson's equation of phonons which is consistent with this Hartree-Fock approximation. We point out that Pytte's work is not still complete even in the framework of the Hartree-Fock theory since a term was left out there which gave a quantitative difference between the Heisenberg model and the X Y model. We find the softening of phonons in the antiferromagnetic state which has overcome the spin-Peierls state.