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Physical Review A

Electromagnetically induced absorption via incoherent collisions

Xihua Yang, Jiteng Sheng, Min Xiao

Published Oct 21, 2011• 19 citations
Publisher

Abstract

We conduct theoretical studies on electromagnetically induced absorption via incoherent collisions in an inhomogeneously broadened ladder-type three-level system with the density-matrix approach. The effects of the collision-induced coherence decay rates as well as the probe laser field intensity on the probe field absorption are examined. It is shown that with the increase of the collisional decay rates in a moderate range, a narrow dip due to electromagnetically induced transparency superimposed on the Doppler-broadened absorption background can be turned into a narrow peak under the conditions that the probe field intensity is not very weak as compared to the pump field, which results from the enhancement of constructive interference and suppression of destructive interference between one-photon and multiphoton transition pathways. The physical origin of the collision-assisted electromagnetically induced absorption is analyzed with a power-series solution of the density-matrix equations.

DOI
10.1103/physreva.84.043837

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International Journal of Modern Physics B•Mar 2, 2024•2 citations
We conduct theoretical studies on electromagnetically induced absorption via incoherent collisions in an inhomogeneously broadened ladder-type three-level system with the density-matrix approach. The effects of the collision-induced coherence decay rates as well as the probe laser field intensity on the probe field absorption are examined. It is shown that with the increase of the collisional decay rates in a moderate range, a narrow dip due to electromagnetically induced transparency superimposed on the Doppler-broadened absorption background can be turned into a narrow peak under the conditions that the probe field intensity is not very weak as compared to the pump field, which results from the enhancement of constructive interference and suppression of destructive interference between one-photon and multiphoton transition pathways. The physical origin of the collision-assisted electromagnetically induced absorption is analyzed with a power-series solution of the density-matrix equations.
In contrast to the general thought that the collisions are intrinsically dephasing in nature and detrimental to quantum entanglement at room or higher temperatures, here, we show that in the conventional ladder-type electromagnetically induced transparency (EIT) configuration, when the probe field intensity is not very weak as compared to the pump field, the entanglement between the bright pump and probe fields can be remarkably enhanced with the increase of the collisional decay rates in a moderate range in an inhomogeneously broadened atomic system. The strengthened entanglement results from the enhancement of constructive interference and suppression of destructive interference between one-photon and multiphoton transition pathways. Our results clearly indicate that the collisions offer a promising alternative to enhance entanglement at room or higher temperatures despite of the dephasing nature, which provides great convenience for experimental implementation, and opens new prospects and applications in realistic quantum computation and quantum information processing.
We study the response of an inhomogeneously broadened atomic three-level ladder system to a strong probe beam under conditions in which electromagnetically induced transparency would be induced on a weak probe beam. Theoretical analysis and experimental data show that saturation effects associated with the strong probe can substantially alter the behavior of the system and can result in enhanced probe absorption under exactly the same circumstances in which a weak probe would experience enhanced transparency. Strong probe effects are also shown to lead to a breakdown of the correspondence between population inversion and gain. A power-series solution of the density-matrix equations describing the ladder system provides a physical picture for strong probe effects in terms of interfering multiphoton transition pathways.
The effect of the collisions on the control of coherent population transfer in a closed inverse YYY-type four-level system driven by three laser fields is investigated with the stimulated Raman adiabatic passage technique. An arbitrary coherent superposition between the initial state and target state can be created either by varying the Rabi frequency of the control laser field or by tuning the one-photon detunings of the pump and Stokes laser fields. When the three laser fields with nearly equal peak Rabi frequencies are each tuned to resonance with the respective transitions, the low transfer efficiency due to the nonadiabatic coupling between two degenerate adiabatic states could be enhanced dramatically with the increase of the collision-induced coherence decay rates to the value nearly comparable to the Rabi frequency of the control field. The enhanced transfer efficiency results from the collision-controlled electromagnetically induced transparency in the $\ensuremath{\Lambda}$-type three-level subsystem and electromagnetically induced absorption in the ladder-type three-level subsystem of the four-level system.
We present a theory of electromagnetically induced transparency (EIT) and slow light in a Doppler broadened three-level ladder (cascade) system incorporating residual Doppler broadening of two-photon coherence and velocity-changing and dephasing collision effects of a buffer gas. Both regimes of wave-vector mismatch occurring when either the probe frequency is higher than that of the (strong) control field or vice versa are considered. It is found that the velocity-changing collisions in general cause narrowing of EIT resonance linewidths which, in a particular wave-vector mismatch regime, can lead to large transparency and slow light generation at relatively low control field intensities. Large collisional dephasing of two-photon coherence in a ladder system, however, tends to mask these effects. A reduction in group velocity by more than 3 orders of magnitude is predicted in the regime where the probe frequency is lesser than that of the control field and in the absence of collisions.
This investigation clarifies the transition phenomenon between the electromagnetically induced transparency (EIT) and Raman absorption in a ladder-type system of Doppler-broadened cesium vapor. A competition window of this transition was found to be as narrow as 2 MHz defined by the probe Rabi frequency. For a weak probe, the spectrum of EIT associated with quantum interference suggests that the effect of the Doppler velocity on the spectrum is negligible. When the Rabi frequency of the probe becomes comparable with the effective decay rate, an electromagnetically induced absorption (EIA) dip emerges at the center of the power broadened EIT peak. While the Rabi frequency of the probe exceeds the effective decay rate, decoherence that is generated by the intensified probe field occurs and Raman absorption dominates the interaction process, yielding a pure absorption spectrum; the Doppler velocity plays an important role in the interaction. A theory that is based on density matrix simulation, with or without the Doppler effect, can qualitatively fit the experimental data. In this work, the coherence of atom-photon interactions is created or destroyed using the probe Rabi frequency as a decoherence source.
In a Doppler-broadened ladder-type Rubidium atomic system [Formula: see text]–[Formula: see text]–[Formula: see text], three-photon electromagnetically induced absorption (EIA) and transparency (EIT) in two schemes of two coupling lasers with different propagation directions are comprehensively studied. Two coupling fields are entangled tightly with each other and induce constructive interference such that we observe EIA as two coupling fields are counter-propagating. Two coupling fields are independent and cause destructive interference such that only enhanced EIT occurs when two coupling fields are co-propagating, although all of the Doppler-broadened atoms satisfy the condition for three-photon resonance. The experimental results are coincided with the numerically calculated spectra using the dressed perturbation method. The mechanisms of EIT and EIA could also be understood by the dressed-state pictures.