We give a general nonperturbative treatment of cooperative emission in systems of
N two-level atoms, starting from first principles and including inhomogeneous broadening. In particular, we study superfluorescence, which is defined as the cooperative spontaneous emission, i.e., radiation rate proportional to
N2, from an atomic system initially excited with zero macroscopic dipole moment and a uniform population difference between the excited and the fundamental states. The atomic system is described by means of collective dipole operators. A fundamental justification is given for the existence of damped "quasimodes" of the mirrorless active volume. The damping of such modes is simply due to the propagation of the Maxwell field, which escapes from the active volume. A general atom-field master equation is derived for the system atoms plus field inside the active volume, described, respectively, in terms of collective dipole operators and quasimode operators. An important feature of this equation is that inhomogeneous broadening simply appears via a time-dependent atom-field coupling constant. In this paper we give a semiclassical treatment of such a master equation. For a pencil-shaped geometry of the active volume, generalized Maxwell-Bloch equations are derived for the envelopes of the radiation inside the active volume and polarization. Such equations take into account the two directions of propagation of the radiation and the inhomogeneous broadening. Suitably phrasing our initial condition in semiclassical terms, we find that propagation effects can be neglected at all times and the generalized Maxwell-Bloch equations reduce to a simple pendulum equation. On the basis of the discussion of the pendulum equation, we conclude that superfluorescence occurs when (i) the length
L of the active volume is much larger than a suitable threshold length
LT (this condition ensures that the dephasing atomic processes occur on a time scale much larger than the times characteristic of the cooperative emission); (ii) the length
L is smaller or of the same order of a suitable cooperation length
Lc (this condition ensures that cooperative spontaneous emission dominates stimulated processes, which give radiation proportional to
N). For $L\ensuremath{\ll}{L}_{c}$, one has a hyperbolic-secant superfluorescent pulse; for $L\ensuremath{\approx}{L}_{c}$, as one has in the recent experiments of Skribanowitz et al., one finds oscillations in the cooperative decay and in the radiation emission. Such oscillations are due to the contribution of stimulated processes. For $L\ensuremath{\gg}{L}_{c}$, this contribution increases. As a consequence one gets more oscillations in the radiated intensity, which becomes proportional to
N, so that superfluorescence effects disappear.
We discuss from first principles the cooperative decay of a system of two-level atoms, initially prepared in an uncorrelated excited state with population inversion
N, and we give the conditions under which the superfluorescence effect occurs. Describing the atomic system in terms of collective variables, we derive a master equation for the reduced atomic density operator, which gives rise both to a damping and to a time-dependent frequency shift in the dynamics of collective modes. The coupled equations of motion are solved with a self-consistent approach. It is found that the system goes through a nonexponential decay if the maximum length of the active volume is smaller than a "cooperation range" and larger than a "threshold length," in agreement with the one-mode theory. The radiation burst has a time width proportional to ${N}^{\ensuremath{-}1}$, and its intensity is proportional to
N2. Specializing to a pencil-shaped volume, we find that only two atomic modes need to be considered; in this case, the average emitted radiation is all condensed in the two diffraction patterns of the opposite axial modes.
The dynamics of the pulse shape and spectra of superfluorescence, stimulated superradiance, and coherent amplification of ultrashort light pulses is studied for a system of four-level atoms under incoherent cw pumping taking into account homogeneous and inhomogeneous broadening of the luminescence lines. It is found that incoherent pumping at a high level of excitation may significantly change the shape of the emission pulse in cooperative coherent processes. Also, it is found that, depending on the ratio of parameters of the pump, nonradiative transitions, and relaxation, different regimes of superfluorescence and stimulated superradiance may be realized.
The fully quantum mechanical treatment of superfluorescence buildup in the linearized regime of superfluorescence is presented for coherently, optically pumped three-level systems. It is shown that to order $\frac{{\ensuremath{\tau}}_{p}}{{\ensuremath{\tau}}_{R}}$, where ${\ensuremath{\tau}}_{p}$ is the pump time duration and ${\ensuremath{\tau}}_{R}$ the characteristic superfluorescence time, fluorescence buildup during the dynamical pumping process contributes significantly to quantum initiation of superfluorescence.
Numerical researches of the three-level atomic system on supervision of pulse and spectrum dynamics of superfluorescence are carried out at incoherent pumping depending on nonradiation relaxations, on influence of phase relaxations are shown. Pulse and spectrum dynamics of induced superradiation depending on the area and duration of input pulse at incoherent pumping, with and without taking into account phase relaxations, are investigated. Depending on media parameters different modes of induced superradiation are researched.
We discuss various aspects of the incoherent spontaneous emission in atomic few-level systems arising from the coupling of the atom to the surrounding vacuum. First, we consider systems where the decoherence due to spontaneous emission acts as a limiting factor. Here, we combine collective effects in larger samples of atoms with control mechanisms known from single-atom schemes, or modify the system dynamics by externally inducing multiphoton quantum interference effects. In the second part, we discuss ground-state laser cooling of trapped atoms and ions. Here, the momentum transfer in the spontaneous emission events is required to cool the particles, but needs to be controlled in order to achieve a low cooling limit. In our scheme, we make use of double electromagnetically induced transparency in order to design the absorption spectrum of the trapped particle. In the final part, we show that the incoherent part of the resonance fluorescence spectrum of a two-level system may serve as an interesting candidate for high-precision spectroscopy. For this, we discuss relativistic and radiative corrections to the resonance fluorescence spectra of laser-driven few-level systems.