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Physical Review Letters

Anomalous Resonance Fluorescence Spectra in a Squeezed Vacuum

S. Swain

Published Sep 12, 1994• 62 citations
Publisher

Abstract

We show that the resonance fluorescence of a two-level atom interacting with a squeezed vacuum can show a wide variety of anomalous features (including hole burning at line center) over a continuous but very narrow range of parameter values. The spectra have a variety of profiles, all of which are qualitatively different from those observed in normal resonance fluorescence and are a distinctive manifestation of the presence of the nonclassical field. The anomalous features persist in a cavity environment, which provides the best means for their experimental observation.

DOI
10.1103/physrevlett.73.1493

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We show that the resonance fluorescence of a two-level atom interacting with a squeezed vacuum can show a wide variety of anomalous features (including hole burning at line center) over a continuous but very narrow range of parameter values. The spectra have a variety of profiles, all of which are qualitatively different from those observed in normal resonance fluorescence and are a distinctive manifestation of the presence of the nonclassical field. The anomalous features persist in a cavity environment, which provides the best means for their experimental observation.
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The steady-state resonance fluorescence spectrum of a two-level atom driven by a bichromatic field in a broadband squeezed vacuum is studied. When the carrier frequency of the squeezed vacuum is tuned to the frequency of the central spectral line, anomalous spectral features, such as hole burning and dispersive profiles, can occur at the central line. We show that these features appear for wider, and experimentally more convenient, ranges of the parameters than in the case of monochromatic excitation. The absence of a coherent spectral component at the central line makes any experimental attempt to observe these features much easier. We also discuss the general features of the spectrum. When the carrier frequency of the squeezed vacuum is tuned to the first odd or even sidebands, the spectrum is asymmetric and only the sidebands are sensitive to phase. For appropriate choices of the phase the linewidths of only the odd or even sidebands can be reduced. A dressed-state interpretation is provided.
We report unusual profiles in the resonance fluorescence spectrum of a two-level atom interacting with a resonant classical field of intermediate intensity and a squeezed vacuum. These have a dispersive profile, quite unlike any previously described, and are a distinctive feature of the interaction of atomic systems with nonclassical fields. An approximate analytic expression is obtained which explains these features, and it is shown that they arise from atomic correlations not probed in normal resonance fluorescence.
It has been suggested that phased atomic decay in a squeezed vacuum could be detected in the fluorescence spectrum emitted from a driven two-level atom in a cavity. Recently, the existence of other very distinctive features in the fluorescence spectra arising from the nonclassical features of the squeezed vacuum has been reported. In this paper, we investigate the possibility of experimental observation of these spectra. The main obstacle to the experimentalist is ensuring an effective squeezed-vacuum-atom coupling. To overcome this problem we propose the use of a Fabry-P\'erot microcavity. The analysis involves a consideration of the three-dimensional nature of the electromagnetic field, and the possibility of a mismatch between the squeezed and cavity modes. The problem of squeezing bandwidths is also addressed. We show that under experimentally realistic circumstances many of the spectral anomalies predicted in free space also occur in this environment. In addition, we report large population inversions in the dressed states of the two-level atom.
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Using the coupled-system approach we calculate the optical spectra of the fluorescence and transmitted fields of a two-level atom driven by a squeezed vacuum of bandwidths smaller than the natural atomic linewidth. We find that in this regime of squeezing bandwidths the spectra exhibit unique features, such as a hole burning and a three-peak structure, which do not appear for a broadband excitation. We show that the features are unique to the quantum nature of the driving squeezed vacuum field and do not appear when the atom is driven by a classically squeezed field. We find that a quantum squeezed-vacuum field produces squeezing in the emitted fluorescence field which appears only in the squeezing spectrum while there is no squeezing in the total field. We also discuss a nonresonant excitation and find that depending on the squeezing bandwidth there is a peak or a hole in the spectrum at a frequency corresponding to a three-wave-mixing process. The hole appears only for a broadband excitation and results from the strong correlations between squeezed-vacuum photons.