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Optics Communications

Coherent control of spectra effects with chirped femtosecond laser pulse

Xiaohong Song, Shangqing Gong, Weifeng Yang, Shiqi Jin, Xun‐Li Feng, Zhizhan Xu

Published Mar 21, 2004• 12 citations
Publisher
DOI
10.1016/j.optcom.2004.03.029

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We have studied the effects of chirped femtosecond laser pulses on the formation of ultracold molecules in a Rb magneto-optical trap. We have found that application of chirped femtosecond pulses suppressed the formation of (85)Rb and (87)Rb(2) a(3)sigma(+)(u) molecules in contrast to comparable nonchirped pulses, cw illumination, and background formation rates. Variation of the amount of chirp indicated that this suppression is coherent in nature, suggesting that coherent control is likely to be useful for manipulating the dynamics of ultracold quantum molecular gases.