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Physical Review A

Teardrop bifurcation for Rydberg atoms in parallel electric and magnetic fields

André Deprit, Victor Lanchares, Manuel Iñarrea, J. Pablo Salas, J. D. Sierra

Published Nov 1, 1996• 16 citations
Publisher

Abstract

In the classical model for Rydberg atoms, the transition from a pure Zeeman effect to a pure Stark effect passes through a teardrop bifurcation when the magnetic quantum number is not zero. \textcopyright{} 1996 The American Physical Society.
DOI
10.1103/physreva.54.3885

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I have calculated the energy spectrum of a highly excited atom which lies in parallel, static electric and magnetic fields. In parallel fields the Coulomb quantum numbers n and m are still "good" quantum numbers but 1 is not: the calculation is for n = 30, m = 1 atoms.;The eigenvalues were obtained by semi-classical quantisation of first-order classical perturbation theory and have been calculated for a large range of electric and magnetic field strengths. The results are in good agreement with those found from first-order degenerate quantum perturbation theory.;The semi-classical analysis provides a correlation diagram connecting the Stark effect states to those of the diamagnetic effect.
The quadratic Zeeman effect of Rydberg atoms is treated with the help of first-order perturbation theory and a special WKB approximation. The Bohr-Sommerfeld quantization leads to complete elliptic integrals. As a result we found that the spectrum is doubly degenerate if n2m2>5\frac{{n}^{2}}{{m}^{2}>5}m2>5n2​, this part exhibiting a linear Stark effect in an additional weak electric field; the rest of the spectrum (n2m2<5\frac{{n}^{2}}{{m}^{2}<5}m2<5n2​) is nondegenerate, exhibiting a quadratic Stark effect in an additional weak electric field.
A Rydberg atom has a highly excited valence electron which is weakly bound and far from the nucleus. These atoms have exaggerated properties that make them attractive candidates for quantum computation and studies of fundamental quantum mechanics. The discrete energy levels of Rydberg atoms are shifted in the presence of an electric field by the Stark effect and are similarly shifted due to a magnetic field by the Zeeman effect. These effects couple the energy levels together, creating avoiding crossings. At these avoided crossings, an electron in one energy level can jump to the other. Our goal is to be able to use these avoided crossings to put the electron in a superposition state of both energy levels. In order to achieve this we created new software that enables us to calculate the energy levels of an electron in both a magnetic and an electric field. We present energy level maps visualizing the results of the Stark and Zeeman effects.
The problem of Rydberg atomic spectra in crossed electric F and magnetic B fields (combined Stark–Zeeman effects), as well as an oscillating electric field are under consideration. The main problem is the great array of radiative transitions between the Rydberg atomic states. The different versions of semiclassical approaches are applied for the solution of the problem. New approximate selection rules are established to simplify the matrix elements of radiative transitions, making it possible to reduce the complex expressions of Gordon’s hypergeometric series to the trivial trigonometric functions. Simple analytical formulas for the dipole matrix elements of a Rydberg hydrogen-like atom in external crossed electric and magnetic fields for Hnα are obtained. The specific calculations are presented for n = 10 to 9 transition both for parallel and perpendicular orientations of F–B fields. The result of Blokhintsev for a single Stark component in oscillating field is generalized for the array of radiative transitions between Rydberg atomic states. Such spectra with large values of modulation index are compared with static ones.
We report the observation of a controlled Landau-Zener transition (LZT) in Rydberg atoms by breaking the symmetry of the underlying Hamiltonian. For a nonhydrogenic Rydberg atom inside a changing electric (F) field, a LZT occurs between the avoided crossing energy levels of neighboring Rydberg states only for a sufficiently high changing rate. If a transverse magnetic (B) field is applied as we implement, the atomic level symmetry is broken, which causes the Stark manifolds denoted by a different |m| (m is the magnetic quantum number) to interact with each other. The mixed state levels end up pushing the adiabatically repelled target states closer and additionally they serve as stepping stones for the sequential LZTs between the neighboring sublevels. Such a feature significantly decreases the changing rate required for an efficient LZT inside a pure electric field. We report experimental observations that support the above scenario. It opens a versatile approach for engineering a controlled LZT in more general systems.