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Physical review. B, Condensed matter

Thermodynamic properties of the random-field spherical model

Richard M. Hornreich, H. G. Schuster

Published Oct 1, 1982• 35 citations
Publisher

Abstract

The thermodynamic properties of a $d$-dimensional classical vector-spin system in a random magnetic field are calculated explicitly in the spherical-model limit. The system is characterized by significant spin-glass order of the Edwards-Anderson type even when no transition to a state with spontaneous magnetization occurs. This spin-glass order should result in observable effects in the magnetic susceptibility and specific heat. The properties of the random-field spherical model are compared with those reported for the corresponding Ising model. The behavior of the coherence length is identical in both models at their respective lower critical dimensionalities.

DOI
10.1103/physrevb.26.3929

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The thermodynamic properties of a ddd-dimensional classical vector-spin system in a random magnetic field are calculated explicitly in the spherical-model limit. The system is characterized by significant spin-glass order of the Edwards-Anderson type even when no transition to a state with spontaneous magnetization occurs. This spin-glass order should result in observable effects in the magnetic susceptibility and specific heat. The properties of the random-field spherical model are compared with those reported for the corresponding Ising model. The behavior of the coherence length is identical in both models at their respective lower critical dimensionalities.
Critical behavior of Ising spin-glass with $\ifmmode\pm\else\textpm\fi{}J$ distribution is discussed. The results are based on the high-temperature series expansion of Edwards-Anderson susceptibility in powers of w(=tanh2JkT)w (=\frac{{tanh}^{2}J}{\mathrm{kT}})w(=kTtanh2J​) for 2D, 3D, and 4D "cubic" lattices to orders 19, 17, and 15, respectively. The lengths of the series are comparable to the best available for the pure Ising model. While 3D and 4D systems exhibit transitions at finite temperatures, in 2D a zero-temperature transition with a power-law divergence (in inverse temperature) for the susceptibility is found. The estimates of critical temperatures and exponents are presented.
We present an alternative treatment to the quantum spherical spin model on $(d\ensuremath{\ge}2)$-dimensional hypercubic lattices, focusing on the effects of quantum (g)(g)(g) and thermal (T)(T)(T) fluctuations, under a uniform magnetic field hhh, on the correlation function, correlation length, entropy, specific heat, and energy gap in the excitation spectrum. Explicit expressions for such quantities are provided close to the $d\ensuremath{\ge}2$ quantum (g=gcg={g}_{c}g=gc​, T=0T=0T=0) and $d\ensuremath{\ge}3$ thermal [T=Tc(g)][T={T}_{c}(g)][T=Tc​(g)] phase transitions in h=0h=0h=0, including the low-TTT quantum regimes near the quantum critical point. In particular, the calculation of the correlation function and correlation length generalizes the results on the g=0g=0g=0 classical spherical model. At T=0T=0T=0, the zero-field system is gapless at and below gc{g}_{c}gc​; however, a gap opens in the quantum-disordered ground state, g>gcg>{g}_{c}g>gc​. Conversely, the null gap for $T\ensuremath{\le}{T}_{c}(g\ensuremath{\ne}0)$ becomes finite as $T\ensuremath{\rightarrow}{T}_{c}(g\ensuremath{\ne}0{)}^{+}$; thus, quantum fluctuations suppress the critical prefactors of observables near ${T}_{c}(g\ensuremath{\ne}0)$, though they are irrelevant to the universality class shared with the gapless classical spherical model. The results on the entropy and specific heat in $g\ensuremath{\ne}0$ circumvent the drawback in classical spherical models concerning the third law of thermodynamics, as $T\ensuremath{\rightarrow}0$.
We study a quantum extension of the spherical p-spin-glass model using the imaginary-time replica formalism. We solve the model numerically and we discuss two analytical approximation schemes that capture most of the features of the solution. The phase diagram and the physical properties of the system are determined in thermodynamic equilibrium and under conditions of marginal stability. In both cases, the phase diagram consists of two qualitatively different regions. If the transition temperature is higher than a certain value T∗,{T}^{*},T∗, quantum effects are qualitatively irrelevant and the phase transition is second order, as in the classical case. When quantum fluctuations depress the transition temperature below T∗,{T}^{*},T∗, the transition becomes first order. The susceptibility is discontinuous and shows hysteresis across the first-order line. This behavior is reminiscent of that observed in the dipolar Ising spin-glass ${\mathrm{LiHo}}_{x}{\mathrm{Y}}_{1\ensuremath{-}x}{\mathrm{F}}_{4}$ in an external transverse magnetic field. We discuss the thermodynamics and the stationary dynamics of both states. The spectrum of magnetic excitations of the equilibrium spin-glass state is gapped, leading to an exponentially small specific heat at low temperatures. That of the marginally stable state is gapless and its specific heat varies linearly with temperature, as generally observed in glasses at low temperature. We show that the properties of the marginally stable state are closely related to those obtained in studies of the real-time dynamics of the system weakly coupled to a quantum thermal bath. Finally, we discuss a possible application of our results to the problem of polymers in random media.
A mean-field spherical model with random couplings between pairs, quartets, and possibly higher multiplets of spins is considered. It has the same critical behavior as the Sherrington-Kirkpatrick model. It thus exhibits replica symmetry breaking. The order parameter function is solved exactly in the whole low temperature phase. The zero-field-cooled susceptibility remains finite at low TTT. Next a quantum version of the system is considered. Whereas the magnetic properties are not altered qualitatively, the thermodynamics is now regular at small temperatures.
We study analytically the equilibrium properties of the spherical hierarchical model in the presence of random fields. The expression for the critical line separating a paramagnetic from a ferromagnetic phase is derived. The critical exponents characterising this phase transition are computed analytically and compared with those of the corresponding D -dimensional short-range model, leading to conclude that the usual mapping between one dimensional long-range models and D -dimensional short-range models holds exactly for this system, in contrast to models with Ising spins. Moreover, the critical exponents of the pure model and those of the random field model satisfy a relationship that mimics the dimensional reduction rule. The absence of a spin-glass phase is strongly supported by the local stability analysis of the replica symmetric saddle-point as well as by an independent computation of the free-energy using a renormalization-like approach. This latter result enlarges the class of random field models for which the spin-glass phase has been recently ruled out.
A general phenomenological theory of spin-glasses is presented, which predicts the weak singularities (like cusps) of susceptibilities and specific heat near the transition point TSG and also predicts generally the divergence of the second derivative of the nonlinear susceptibility with respect to a magnetic field in zero field at TSG. A similar second derivative of specific heat is also shown to diverge at TSG except for the molecular field theory. Scaling equations of state for magnetization m and spin-glass order-parameter q are derived, which yield new scaling relations of critical exponents for m(T), q(T), χ0(T), C0(T) and the corresponding nonlinear quantities. These general results explain qualitatively very well the magnetic field dependence of magnetization and specific heat observed experimentally. A non-uniform phenomenological Hamiltonian is also proposed for the renormalization group approach, which yields the critical dimensionality dc = 6, as usual. Intermediate random statistics and real replica method are proposed. There is also presented an exactly soluble model showing a spin-glass like phase transition.