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Physical Review A

Diffraction of atoms moving through a standing light wave

Peter J. Martin, P. L. Gould, Bruce G. Oldaker, A. H. Miklich, David E. Pritchard

Published Sep 1, 1987• 106 citations
Publisher

Abstract

The diffraction of sodium atoms from a standing wave of near-resonant light is studied as a function of the atomic velocity component along the k vector of the wave. A simple theory is presented which quantitatively predicts the observed diffraction patterns and the decrease of the rms momentum transfer to the atoms with increasing velocity. This decrease results from the dephasing between the two counterpropagating traveling waves due to the first-order Doppler shift. In addition, these measurements have resolved the previous discrepancy between theory and experiment concerning the overall momentum transferred by a standing wave.

DOI
10.1103/physreva.36.2495

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Annual Meeting Optical Society of America•Jan 1, 1990•0 citations
The diffraction of sodium atoms from a standing wave of near-resonant light is studied as a function of the atomic velocity component along the k vector of the wave. A simple theory is presented which quantitatively predicts the observed diffraction patterns and the decrease of the rms momentum transfer to the atoms with increasing velocity. This decrease results from the dephasing between the two counterpropagating traveling waves due to the first-order Doppler shift. In addition, these measurements have resolved the previous discrepancy between theory and experiment concerning the overall momentum transferred by a standing wave.
We have observed both diffractive and diffusive regimes in the transfer of momentum to an atomic beam by a standing-wave radiation field. The momentum transfer was measured by passing a well-collimated beam of sodium atoms through a focused standing-wave laser waist. A narrow velocity distribution beam was obtained by utilizing a supersonic expansion and a two-state system was realized by optically pumping the beam prior to the interaction. The transverse momentum transferred to the atomic beam by the radiation field was measured by scanning a detector downstream from the interaction. The overall momentum resolution of the apparatus is less than the momentum of a single photon. The transition from diffractive to diffusive behavior is associated with an increase in the average number of spontaneous decays occurring during the interaction. In the diffractive regime, spontaneous decay is insignificant and momentum transfer proceeds by pairs of absorption/stimulated emission processes. This produces momentum exchange quantized in even multiples of photon momentum, the so-called Kapitza-Dirac effect; the deflection patterns show oscillatory structure. In the diffusive regime, spontaneous decay is important and causes fluctuations in the radiative forces. In addition, the recoil distribution associated with spontaneous decay results in a washing out of the diffraction peaks associated with stimulated processes, resulting in a smooth deflection pattern.
Momentum transfer to atoms by a standing light wave is measured in the presence of spontaneous decay. As the number of spontaneous decays is increased, the well-known Kapitza-Dirac diffractive structure observed in the absence of spontaneous decay evolves into a smooth diffusive pattern. Theoretical treatments based on a diffusive model adequately describe the rms momentum transfers and the envelopes of the momentum distributions. However, we observe significant persistence of diffractive structure at our long interaction times and find that details of the deflection profiles are accurately predicted only when several spontaneous decays occur during the interaction.
We investigate the diffraction of a three-level atom from a "walking" light wave composed of counterpropagating traveling waves of different frequencies. The coupling of the two nondegenerate internal ground states by means of an off-resonant Raman transition resonantly couples the initial external momentum state to only one other momentum state. This happens even in the Raman-Nath regime, where the interaction time is short enough that momentum transfer is not constrained by phase-matching conditions. The final momentum state depends on the initial internal state of the atom and the relative directions of the two traveling waves. By using multiple diffraction regions, this process can be used to coherently split a beam of atoms into two beams that are widely separated in momentum space. This type of beam splitter would be useful in the building an atom interferometer.
Atoms undergo two types of momentum changes as they pass across a near-resonant standing wave. First, their transverse momentum spreads. Second, if the atoms cross the field at an angle, they undergo Bragg scattering from the periodic structure provided by the wave. Classically, this behavior can be understood in terms of traveling waves: the atom catalyzes the transfer of momentum from one traveling wave to the other, thereby changing its own transverse momentum. In the quantum regime, however, there is an essential difference between scattering by two running waves and by a standing wave. With running waves, we can in principle know which of the two waves has exchanged a unit of momentum with the atom. In contrast, a standing wave is an inseparable quantum unit whose average momentum remains zero at all times. This unity is imposed by the fixed mirrors that establish the standing wave. These act as infinite sinks of momentum. Quantum mechanics forbids one even in principle to determine, via a field measurement from which traveling wave the atom picked up its momentum. To demonstrate this point, we discuss the diffraction and deflection of an atom in both a standing wave and a superposition of two counter-propagating running waves.