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AIP conference proceedings

Extremely high Q-factor mechanical modes in quartz bulk acoustic wave resonators at millikelvin temperature

Maxim Goryachev, Daniel Lloyd Creedon, Eugene N. Ivanov, Serge Galliou, R. Bourquin, Michael Edmund Tobar

Published Jan 1, 2014• 2 citations
Publisher

Abstract

We demonstrate that Bulk Acoustic Wave (BAW) quartz resonator cooled down to millikelvin temperatures are excellent building blocks for hybrid quantum systems with extremely long coherence times. Two overtones of the longitudinal mode at frequencies of 15.6 and 65.4 MHz demonstrate a maximum f.Q product of 7.8×1016 Hz. With this result, the Q-factor in such devices near the quantum ground state can be four orders of magnitude better than previously attained in other mechanical systems. Tested quartz resonators possess the ultra low acoustic losses crucial for electromagnetic cooling to the phonon ground state.

DOI
10.1063/1.4903104

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A quartz Bulk Acoustic Wave resonator is designed to coherently trap phonons in such a way that they are well confined and immune to suspension losses so they exhibit extremely high acoustic Q-factors at low temperature, with Q × f products of order 10¹⁸ Hz. In this work we couple such a resonator to a Superconducting Quantum Interference Device (SQUID) amplifier and investigate effects in the strong signal regime. Both parallel and series connection topologies of the system are investigated. The study reveals significant non-Duffing response that is associated with the nonlinear characteristics of Josephson junctions. The nonlinearity provides quasi-periodic structure of the spectrum in both incident power and frequency. The result gives an insight into the open loop behaviour of a future Cryogenic Quartz Oscillator in the strong signal regime.

•Jan 1, 2018•0 citations
We demonstrate that Bulk Acoustic Wave (BAW) quartz resonator cooled down to millikelvin temperatures are excellent building blocks for hybrid quantum systems with extremely long coherence times. Two overtones of the longitudinal mode at frequencies of 15.6 and 65.4 MHz demonstrate a maximum f.Q product of 7.8×1016 Hz. With this result, the Q-factor in such devices near the quantum ground state can be four orders of magnitude better than previously attained in other mechanical systems. Tested quartz resonators possess the ultra low acoustic losses crucial for electromagnetic cooling to the phonon ground state.
Low-loss, high frequency acoustic resonators cooled to millikelvin temperatures are a topic of great interest for application to hybrid quantum systems. When cooled to 20 mK, we show that resonant acoustic phonon modes in a bulk acoustic wave quartz resonator demonstrate exceptionally low loss (with Q-factors of order billions) at frequencies of 15.6 and 65.4 MHz, with a maximum f · Q product of 7.8 × 1016 Hz. Given this result, we show that the Q-factor in such devices near the quantum ground state can be four orders of magnitude better than previously attained. Such resonators possess the low losses crucial for electromagnetic cooling to the phonon ground state, and the possibility of long coherence and interaction times of a few seconds, allowing multiple quantum gate operations.
High-frequency mechanical oscillators with long coherence times are essential for realizing a variety of high-fidelity quantum sensors, transducers and memories. However, the coherence times needed for quantum applications require advances in probing and mitigating the origins of phonon decoherence in the materials used for mechanical oscillators. Here we identify key sources of phonon decoherence in crystalline media by combining non-invasive laser spectroscopy with materials analysis. Using micro-fabricated high-overtone bulk acoustic-wave resonators as an experimental test bed, we find that phonon–surface interactions are the dominant source of phonon decoherence in crystalline quartz. The probable causes are lattice distortion, subsurface damage and a high concentration of elemental impurities. We use an optimized polishing process to remove the compromised surface layer and produce resonators with quality factors exceeding 240 million at 12 GHz, corresponding to phonon coherence times of over 6 ms. We verify that these mechanical oscillators have negligible dephasing. Building on these results, we propose a path that could reach coherence times beyond 100 ms as the basis for high-frequency quantum memories. These findings demonstrate that enhanced control over surfaces enables a substantial reduction in dissipation and noise. Phonon decoherence in quantum high-overtone bulk acoustic-wave resonators is dominated by imperfections under the material surface. Removing the damaged subsurface layer substantially increases the performance of these devices.
Hybrid systems that couple superconducting qubits to mechanical oscillators facilitate quantum control of individual phonons and have the potential to enable compact, highly coherent quantum memories and processors. To date, however, the utility of hybrid quantum acoustic devices has been limited by poor qubit and mechanical coherence times that are far shorter than those exhibited by their unhybridized counterparts. A primary challenge lies in the intrinsic nature of elastic waves in solids: the slow speed of sound results in a dense spectrum of acoustic modes, making it difficult to prevent spontaneous emission of the qubit into phononic degrees of freedom. In this thesis, I will present a systematic effort to suppress loss mechanisms in superconducting qubits and mechanical resonators in the context of circuit quantum acoustics. I begin by demonstrating the use of crystallographic orientation optimization to passively suppress diffraction losses in narrow-aperture quartz surface acoustic wave (SAW) resonators. We then study the coupling of SAW resonators to a quasi-continuum of bulk acoustic modes; this motivates us to abandon bulk piezoelectric media in favor of bandgap-protected thin-film devices. By fabricating suspended phononic crystal resonators from thin-film quartz, we demonstrate an order-of-magnitude improvement in the coherence of this class of devices. I conclude by presenting preliminary measurements of a new flip-chip architecture for circuit quantum acoustics -- the `acoustic trampoline' -- that is designed to maximize qubit-mechanical coupling while simultaneously suppressing spontaneous acoustic emission.
Acoustic modes—in the form of collective vibrations trapped between the parallel and polished surfaces of a crystalline cavity—provide an intriguing opportunity for probing the quantum-mechanical regime of macroscopical mechanical resonators. Moreover, the exceptional quality factors in a compact size from mm to μm motivate the integration of acoustic resonators into quantum circuits to explore the applications of a quantum hybrid system.While the acoustic modes of a crystal are commonly isolated from electrical dynamics, piezoelectricityis employed to transduce energy between the two domains. In the first part of this thesis, we investigate the means to improve the quality factor of a low frequency plano-convex monolithic quartz resonator. The resonator is 7mm indiameter and 250 μm in thickness, made only of only piezoelectric crystalline material. By the removal of clamping losses and incorporating a distant non-contact measurement setup,we demonstrate quality factors as high as 108 at cryogenic temperatures close to the quantumground state. Additionally, we model the electromechanical clamping losses of a particular grounding setup using temperature-dependent data and the acoustic transmission line based Mason’s model. In the latter part of this thesis, we couple a bulk acoustic high-overtone resonator (HBAR) with a transmon qubit. The electrical actuation of GHz-frequency sound in a HBAR is based on a μm-thin piezo film grown on a low-loss crystalline non-piezo bulk substrate. With an analogy to an acoustic musical instrument, the driven oscillations are amplified at the resonant frequencies of the acoustic cavity, with the addition that a small subset of such modes are selectively listened by the qubit. By the introduction of the acoustic overtones, high quality factors are accessible at the high frequencies of a transmon qubit,while the coupling between the two systems is distributed over the multitude of modes. I model this coupling in detail with respect to the system parameters for guiding the design of related quantum acoustic devices. I cover several different parameter regimes and explore the rich physics taking place in the multimodal hybrid system: Landau-Zener Stuckelberg interference, photon assisted sideband transitions and parametrically modulated coupling that involve the resonant periodical exchange of energy quanta known as vacuum Rabi oscillations, and drive-dependent multiphonon transitions. Despite the otherwise common difficulty to observe quantum mechanics in a harmonic oscillator, we observe purely quantum mechanical effects in the macroscopic resonator, such as a specific square root dependence of the transition energies on the quantum number.
Circuit quantum acoustodynamics (cQAD) devices have a wide range of applications in quantum science, all of which depend crucially on the quantum coherence of the mechanical subsystem. In this context, high-overtone bulk acoustic-wave resonators (HBARs) are particularly promising, since they have shown very high quality factors with negligible dephasing. However, the introduction of piezoelectric films, which are necessary for coupling to a superconducting circuit, can lead to additional loss channels, such as surface scattering and two-level systems (TLS). Here, we study the acoustic dissipation of HBAR resonators in cQAD systems and find that the defect density of the piezoelectric material and its interface with the bulk are limiting factors for the coherence. We measure acoustic modes with phonon lifetimes up to 400 μμμs and lifetime-limited coherence times approaching one millisecond in the quantum regime. When coupled to a superconducting qubit, this leads to a hybrid system with a large quantum coherence cooperativity of CT2=1.1×105C_{T_2}=1.1\times10^5CT2​​=1.1×105. These results represent a new milestone for the performance of cQAD devices and offer concrete paths forward for further improvements.
A quartz Bulk Acoustic Wave resonator is designed to coherently trap phonons in such a way that they are well confined and immune to suspension losses so they exhibit extremely high acoustic Q-factors at low temperature, with Q × f products of order 10¹⁸ Hz. In this work we couple such a resonator to a Superconducting Quantum Interference Device (SQUID) amplifier and investigate effects in the strong signal regime. Both parallel and series connection topologies of the system are investigated. The study reveals significant non-Duffing response that is associated with the nonlinear characteristics of Josephson junctions. The nonlinearity provides quasi-periodic structure of the spectrum in both incident power and frequency. The result gives an insight into the open loop behaviour of a future Cryogenic Quartz Oscillator in the strong signal regime.