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Physical Review Letters

Optical “Multiexcitons”: Quantum Gap Solitons in Nonlinear Bragg Reflectors

Ze Cheng, Gershon Kurizki

Published Nov 6, 1995• 25 citations
Publisher

Abstract

We find a Bethe-ansatz solution for pairwise interacting quanta within the effective-mass regime of band-gap propagation in nonlinear Bragg reflectors. Our theory predicts a new kind of collective excitation of the electromagnetic field dressed by such media, namely, optical multiexciton (OME) complexes (or condensates), which are quantum states associated with gap solitary waves. Their existence should be manifested by the discrete spectrum of band-gap transmission as a function of the transmitted photon number and by the multiexponential falloff of intensity-intensity correlations on a 0.1 mm scale. OMEs should have advantageous stability properties.

DOI
10.1103/physrevlett.75.3430

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We find a Bethe-ansatz solution for pairwise interacting quanta within the effective-mass regime of band-gap propagation in nonlinear Bragg reflectors. Our theory predicts a new kind of collective excitation of the electromagnetic field dressed by such media, namely, optical multiexciton (OME) complexes (or condensates), which are quantum states associated with gap solitary waves. Their existence should be manifested by the discrete spectrum of band-gap transmission as a function of the transmitted photon number and by the multiexponential falloff of intensity-intensity correlations on a 0.1 mm scale. OMEs should have advantageous stability properties.
We establish a quantum theory of gap solitons in a one-dimensional periodic dielectric structure [distributed Bragg reflector (DBR)] of a Kerr nonlinearity. The electromagnetic field in the structure is quantized within the two-band approximation. The basic idea for this quantization is that incident photons with frequencies in the band gap of the DBR are scattered into the upper ``conduction'' and lower ``valence'' bands by the nonlinearity. The effective Hamiltonian of quantum gap solitons is derived within the effective-mass regime. The eigenstates of the Hamiltonian are constructed exactly by Bethe's ansatz method. We find that in certain band gaps of the DBR these eigenstates can be bound, consisting of one or more photon pairs from the conduction and valence bands. These bound multiphoton states are optical analogs of exciton molecules [optical multiexcitons (OMEs)]. Their existence should be manifested by the discrete spectrum of band-gap transmission as a function of the transmitted photon number and by the multiexponential falloff of intensity-intensity correlations on a 0.1-mm scale. Quantum gap solitons are shown to arise as superpositions of OMEs whenever the nonlinear binding exceeds phonon scattering. \textcopyright{} 1996 The American Physical Society.
Three-dimensional Kerr-nonlinear photonic crystals support a new kind of quantum gap solitons. Such 3D-quantum gap solitons are described by an approximate Bethe-ansatz solution of the quantized nonlinear-field Hamiltonian under the effective mass approximation. Their main manifestations are predicted: (i) a series of discrete transmission peaks in the band gap, which progresses linearly with the diphoton number; (ii) Bessel-function dependence of the intensity correlation function on the detector separation.
Summary form only given. In recent years, there has been considerable interest in nonlinear and quantum optics of photonic bandgap structures. Some of this attention has centered on the properties of gap solitary waves, which are light pulses tuned at a Bragg frequency within a forbidden bandgap of the periodic structure. These solitary waves may occur in a periodically modulated medium with a Kerr-like nonlinearity, and in the resonance grating as a two-wave soliton of self-induced transparency. In the later case, the coupled-mode Maxwell-Bloch equations which describe the on-resonance coherent interaction of the intense field with a periodic structure of thin layers of two-level atoms in the ground state, lead to an integrable sine-Gordon equation. In our study, we concentrate on the nonintegrable case, that is, amplification in a resonant Bragg structure by means of a comprehensive analysis that includes and numerical modelling of Dicke superradiance and coherent amplification.
Quantum electrodynamics of a single two-level atom placed within a frequency dispersive medium whose polariton spectrum has a gap due to photon coupling to a medium excitation (exciton, optical phonon, etc.) is studied. Despite a nonlocal effective polariton-polariton coupling, the system is proven to be integrable and is diagonalized exactly by means of the Bethe-ansatz technique. Its spectrum consists of bound many-polariton complexes (quantum solitons) and exhibits some unusual features due to the existence of the polaritonic gap. Only solitons containing an even number of polaritons propagate within the gap, while a soliton with an odd number of polaritons is pinned to the atom and forms a many-polariton-atom bound state, in which the radiation and the medium polarization are localized in the vicinity of the atom. The model under consideration has a quite general structure and can also be applied to the case of photonic-band-gap materials. \textcopyright{} 1996 The American Physical Society.
A system of polaritons interacting with a two-level atom placed within a frequency dispersive medium is proven to be integrable and diagonalized exactly by the Bethe ansatz method, despite a nonlocal effective polariton-polariton coupling. Its spectrum consists of bound many-polariton complexes (quantum solitons) and exhibits unusual features due to the existence of the polaritonic gap. Only solitons containing an even number of polaritons (``even'' solitons) propagate within the gap, while an ``odd'' soliton is pinned to the atom and forms a many-polariton--atom bound state.
A one-band effective-mass (EFM) theory was developed to study the properties of the localized states of a Bose-Einstein condensate (BEC) in a periodic optical potential with either attractive or repulsive atom interactions. The localized states of the BEC are solitons in the gaps or gap solitons. The analytic solutions of the gap solitons are a Bloch function from periodicity, modulated by a soliton envelope function of the nonlinear Schrödinger equation. The soliton width is determined by the detuning chemical potential from the band edge. The detuning chemical potential in the nonlinear Schrödinger equation indicates that not all the atoms in the condensate are used for forming gap solitons, and that some atoms form the background of nonlinear modes. The background atoms are determined by the chemical potential at the band edge. The gap solitons form on top of the background atoms. PACS numbers: 03.75.Lm, 03.75.Kk, 05.30.Jp I.