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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Collective spontaneous emission from small assemblies of atoms

James Clemens, Levente Horvath, Barry C. Sanders, H. J. Carmichael

Published May 16, 2003• 0 citations
Publisher

Abstract

We study collective spontaneous emission from arbitrary distributions of N two-state atoms using quantum trajectory theory and without an a priori single-mode assumption. Assuming a fully excited initial state, we calculate the angular distribution of the average integrated intensity. We investigate the dependence of the angular distribution of emission on the geometry of the atomic distribution. The formalism is developed around an unravelling of the master equation in terms of source mode quantum jumps. A modified boson approximation is made to treat the many-atom case, where it is found that strong directional superradiance occurs for a few hundred to a few thousand atoms. In order to illustrate important differences between our model and single-mode models we consider shot-to-shot intensity fluctuations and angular correlations in the emitted intensity.

DOI
10.1117/12.490148

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We study collective spontaneous emission from arbitrary distributions of N two-state atoms using quantum trajectory theory and without an a priori single-mode assumption. Assuming a fully excited initial state, we calculate the angular distribution of the average integrated intensity. We investigate the dependence of the angular distribution of emission on the geometry of the atomic distribution. The formalism is developed around an unravelling of the master equation in terms of source mode quantum jumps. A modified boson approximation is made to treat the many-atom case, where it is found that strong directional superradiance occurs for a few hundred to a few thousand atoms. In order to illustrate important differences between our model and single-mode models we consider shot-to-shot intensity fluctuations and angular correlations in the emitted intensity.
We study collective spontaneous emission from a linear array of N two-state atoms using quantum trajectory theory and without an a priori single-mode assumption. Assuming a fully excited initial state, we calculate the angular distribution of the kthk\mathrm{th}kth emitted photon, k=1,…,N.k=1,\dots{},N.k=1,…,N. We investigate the evolution of the distribution from a dipole radiation pattern for the first photon emission to a distribution characteristic of directional superradiance. The formalism is developed around an unravelling of the master equation in terms of source-mode quantum jumps. Exact calculations for 11 and fewer atoms do not show directional superradiance, but are characterized by delayed (subradiant) photon emissions directed along the axis of the linear array. A modified boson approximation is made to treat the many-atom case, where it is found that strong directional superradiance occurs for a few hundred atoms; the decay of subradiant excitations is preserved in the tail of the superradiant pulse.
We study collective spontaneous emission from arbitrary distributions of N two-state atoms using quantum trajectory theory and without an a priori single-mode assumption. Assuming a fully excited initial state, we calculate the angular distribution of the average intensity, focusing on pencil- and disc-shaped samples. The formalism is developed around an unravelling of the master equation in terms of source mode quantum jumps. A modified boson approximation is made to treat the many-atom case, where it is found that strong directional superradiance with shot-to-shot fluctuations occurs for a few hundred to a few thousand atoms.
We consider the directed superradiant emission from a collection of N two-state atoms with arbitrary spatial locations within the framework of quantum trajectory theory and without a single-mode assumption. The formalism is developed around an unravelling of the master equation in terms of source mode quantum jumps. A modified boson approximation is made to treat the many-atom case, where it is found that strong directional superradiance occurs for a few thousand atoms, even with randomized atomic positions.
Spontaneous emission from a system of NNN identical two-level atoms is considered using a master equation recently derived by the author. The master equation describing the time evolution of the phase-space distribution function associated with the reduced density operator of the atomic system is obtained. This master equation, which is of the type of a Fokker-Planck equation, is used to derive the equation of motion for the mean values of various atomic operators characterizing the physical properties of the system. This leads to a hierarchy of equations, which is decoupled by making a suitable approximation. The intensity of the spontaneously emitted radiation is then calculated. Next, the spontaneous emission from geometrically small systems is considered. For this case, the master equation is solved exactly, and an exact expression for the radiation rate is obtained. The exact solution of the master equation is also used to calculate the normally ordered correlation functions for the electric field. Section V deals with the spontaneous emission from a system of harmonic oscillators, the size of the system being small compared to a wavelength. The master equation for this problem is also solved exactly, and it is shown that this system also leads to superradiant emission in some cases, e.g., if all the oscillstors are excited initially to some coherent state ∣z0〉|{z}_{0}〉∣z0​〉.
We investigate the stochastic initiation of superradiant emission from a collection of excited two-state atoms coupled through a low-Q cavity mode. Noncollective emission into other modes of the electromagnetic field is included, allowing us to describe the transition from predominantly noncollective to collective behavior as the number of atoms is increased. We examine the dependence of the photon statistics on the number of atoms and the ratio of collective to noncollective decay rates. Numerical results for a few to 106{10}^{6}106 atoms are obtained using an approximation scheme developed within the framework of quantum trajectory theory. Results are compared with those for a pure collective emission process and an earlier treatment of noncollective effects.
Interaction with a multimode quantized radiation field of an assembly of NNN two-level atoms contained in a small volume is considered for the special cases of (i) highly excited, (ii) weakly excited, and (iii) superradiant atomic assemblies, and solutions of equations of motion are obtained in closed form. For (i) and (ii) we show that, if the atomic assembly is in the Dicke state ∣r,m>|r,m>∣r,m>, the spontaneously emitted radiation is Lorentzian, and its spectral width and the numerical value of the Lamb shift are r+∣m∣r+|m|r+∣m∣ times that for a single excited atom. For (i) the sign of Lamb shift is opposite to that for (ii) and for a single excited atom. Change in the frequency shift gives chirping in the pulse radiation emitted spontaneously by an assembly of atoms. We obtain the reduced density operator for a single mode and for the complete spontaneous emitted radiation, and discuss its characteristic function, weight function in diagonal representation, coherence functions, and normalized variance. We find that the emitted radiation is chaotic if all atoms are excited or if the assembly is weakly excited and is in thermal equilibrium. For a superradiant assembly, the radiation is coherent; it is only amplitude coherent if the initial atomic density operator is nondiagonal. We also study stimulated emission and scattering for the cases (i) and (ii). For case (iii) these phenomena do not take place.