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Physical Review A

Lasers without inversion: Raman transitions using autoionizing resonances

G. S. Agarwal, Seenipandian Ravi, J. Cooper

Published May 1, 1990• 75 citations
Publisher

Abstract

We consider laser action on a transition involving an autoionizing state \ensuremath{\Vert}a〉 and an initially unpopulated state \ensuremath{\Vert}f〉, the population of which builds up because of spontaneous emission and Raman processes. The autoionizing state is pumped by a coherent field. We discuss the transient amplification of the probe field on the lasing transition for a range of parameters. The coherent field on the pumping transition leads to minima in the absorption spectra if the atomic population were in the state \ensuremath{\Vert}f〉. Such regions of minima can be used for obtaining gain even for long times.

DOI
10.1103/physreva.41.4727

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We consider a four-level atomic system with a degenerate or quasidegenerate ground-state doublet and two excited states. One of the upper levels is coupled to the ground doublet by a coherent field of variable strength, which we refer to as the Raman field, whose role is to create atomic coherence between the driven atomic states. The other higher lying state is coupled to the ground states when laser action develops. This model includes an incoherent pump mechanism to create some population in the top lasing state. In appropriate conditions, for the incoherent pump rate and the Raman field strength, the absorption profile of the laser transition develops gain features. We discuss the physical origin of this gain which we find to be the consequence of a population inversion between dressed atomic states. It is interesting to compare the results of this analysis with a similar study of a three-level lambda system which was previously recognized to yield lasing without inversion.1 In this case the appearance of gain can be attributed to the induced atomic coherence.

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The emergence of laser action from an atomic system without population inversion is beginning to attract theoretical and experimental attention as a possible way of generating useful coherent radiation at unusual wavelengths. The goal of this communication is to clarify the physical origin of this phenomenon using a four-level system whose ground state consists of two quasidegenerate levels that are coupled to a higher-lying state by a Raman-like transition. In the presence of the ground-state coherence induced by the Raman field, we calculate the absorption spectrum of a weak probe whose tunable frequency scans across the transition frequencies between the two ground-state levels and another higher-lying state that may or may not be weakly excited by an incoherent pump mechanism. Our calculation, based on a dressed atomic state approach, clarifies the conditions that must be satisfied to produce gain, identifies the frequency (or frequencies) at which the gain is maximum, and elucidates the functions of the incoherent pump, the Raman field, and the coherence between the ground-state levels in this process. An appropriate set of Maxwell- Bloch equations for a ring-cavity model of this system confirms the appearance of laser action when the small-signal gain conditions are satisfied.

Annual Meeting Optical Society of America•Jan 1, 1990•0 citations

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Considerable attention has been directed recently to the study of lasing without the need of population inversion. The optical coherence and quantum interference associated with the light amplification may lead to interesting statistical properties in inversionless lasers. Here we analyze a laser model that consists of an ensemble of closed multi-level (three or four levels) atoms driven by a single coherent field. Unlike conventional lasers where population inversion is maintained and kept at the threshold value for arbitrary laser output, the multi-level laser analyzed here can start lasing from population inversion and evolves from population inversion into non-inversion with the increasing atomic pumping. In other words, the system makes transition from light amplification by population inversion into light amplification by coherence. On the other hand, the system can be also made to start lasing without population inversion in any state basis. In both cases, initial inversion and non-inversion, which are controlled by the ratio of spontaneous decay rates, the laser well above threshold is always maintained by lasing without inversion (light amplification by coherence), and the laser intensity fluctuations may drop below the shot noise limit. Two factors contribute to the noise reduction: first, the disappearance of the population inversion leads to the depleted atomic population in the upper lasing state, which reduces the spontaneous emission noises; second, the fast coherent cycling of electrons between excited states leads to the highly regulated absorption and emission processes. We found that the combination of these two mechanisms can lead to the noise reduction in the laser output more than 50% below the shot-noise limit.

Annual Meeting Optical Society of America•Jan 1, 1993•0 citations
We consider laser action on a transition involving an autoionizing state \ensuremath{\Vert}a〉 and an initially unpopulated state \ensuremath{\Vert}f〉, the population of which builds up because of spontaneous emission and Raman processes. The autoionizing state is pumped by a coherent field. We discuss the transient amplification of the probe field on the lasing transition for a range of parameters. The coherent field on the pumping transition leads to minima in the absorption spectra if the atomic population were in the state \ensuremath{\Vert}f〉. Such regions of minima can be used for obtaining gain even for long times.
We consider how externally coupled (e.g., dc-field-coupled) autoionizing states can be useful in producing gain without population inversion. The dc fields produce new absorption minima that enable one to obtain laser action in different frequency regions depending on the strength of the coupling. We calculate absorption and emission profiles assuming that one of the autoionizing states is incoherently pumped as in most conventional laser models. We present numerical results that demonstrate gain regions without population inversion.
We explore a three-level Lambda scheme to demonstrate that the phenomenon of lasing without inversion (LWI) can be observed in the transient regime. We demonstrate that the pure LWI contribution to the gain of a probe field is distinct from both the resonant absorption (or gain) and the coherent Raman gain (or absorption) by choosing specific initial populations in the dressed-state basis. The suppression of the non-LWI (resonant and Raman) processes is followed by the "rich get richer" (capitalistic) effect for the ground-state population dynamics: Initially, the more populated ground state becomes even more populated. The conditions for the observation of the effect are specified.
The absorption and stimulated emission of coherent electromagnetic radiation tuned close to an autoionizing state is investigated with the aim of clarifying some of the aspects behind the proposals of inversionless gain involving such atomic configurations. This is carried out within the framework of individual atomic evolution rather than by the use of density matrix equations, thus providing better insight into the fundamental processes of absorption and emission. In particular, we find that stimulated emission does not overcome absorption in spite of quantum interference of the Fano type being present. It is also shown that gain, in this configuration, although it can take place without population inversion between the involved levels, requires in any case a strong departure from thermal equilibrium conditions. Thereby a strong pumping mechanism, or equivalently a strong excitation power, is needed to reach the lasing threshold. This raises some questions on the relevance of the population inversion indicator of efficient gain implicitly assumed in similar configurations and in many related works.
We consider a four-level atomic system with a degenerate or quasidegenerate ground-state doublet and two excited states. One of the upper levels is coupled to the ground doublet by a coherent field of variable strength, which we refer to as the Raman field, whose role is to create atomic coherence between the driven atomic states. The other higher lying state is coupled to the ground states when laser action develops. This model includes an incoherent pump mechanism to create some population in the top lasing state. In appropriate conditions, for the incoherent pump rate and the Raman field strength, the absorption profile of the laser transition develops gain features. We discuss the physical origin of this gain which we find to be the consequence of a population inversion between dressed atomic states. It is interesting to compare the results of this analysis with a similar study of a three-level lambda system which was previously recognized to yield lasing without inversion.1 In this case the appearance of gain can be attributed to the induced atomic coherence.
The emergence of laser action from an atomic system without population inversion is beginning to attract theoretical and experimental attention as a possible way of generating useful coherent radiation at unusual wavelengths. The goal of this communication is to clarify the physical origin of this phenomenon using a four-level system whose ground state consists of two quasidegenerate levels that are coupled to a higher-lying state by a Raman-like transition. In the presence of the ground-state coherence induced by the Raman field, we calculate the absorption spectrum of a weak probe whose tunable frequency scans across the transition frequencies between the two ground-state levels and another higher-lying state that may or may not be weakly excited by an incoherent pump mechanism. Our calculation, based on a dressed atomic state approach, clarifies the conditions that must be satisfied to produce gain, identifies the frequency (or frequencies) at which the gain is maximum, and elucidates the functions of the incoherent pump, the Raman field, and the coherence between the ground-state levels in this process. An appropriate set of Maxwell- Bloch equations for a ring-cavity model of this system confirms the appearance of laser action when the small-signal gain conditions are satisfied.
Considerable attention has been directed recently to the study of lasing without the need of population inversion. The optical coherence and quantum interference associated with the light amplification may lead to interesting statistical properties in inversionless lasers. Here we analyze a laser model that consists of an ensemble of closed multi-level (three or four levels) atoms driven by a single coherent field. Unlike conventional lasers where population inversion is maintained and kept at the threshold value for arbitrary laser output, the multi-level laser analyzed here can start lasing from population inversion and evolves from population inversion into non-inversion with the increasing atomic pumping. In other words, the system makes transition from light amplification by population inversion into light amplification by coherence. On the other hand, the system can be also made to start lasing without population inversion in any state basis. In both cases, initial inversion and non-inversion, which are controlled by the ratio of spontaneous decay rates, the laser well above threshold is always maintained by lasing without inversion (light amplification by coherence), and the laser intensity fluctuations may drop below the shot noise limit. Two factors contribute to the noise reduction: first, the disappearance of the population inversion leads to the depleted atomic population in the upper lasing state, which reduces the spontaneous emission noises; second, the fast coherent cycling of electrons between excited states leads to the highly regulated absorption and emission processes. We found that the combination of these two mechanisms can lead to the noise reduction in the laser output more than 50% below the shot-noise limit.